Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy
Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produce...
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| Autor*in: |
Jiménez, J. A. [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2009 |
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| Schlagwörter: |
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| Anmerkung: |
© TMS 2009 |
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| Übergeordnetes Werk: |
Enthalten in: Journal of electronic materials - Springer US, 1972, 39(2009), 1 vom: 29. Sept., Seite 138-143 |
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| Übergeordnetes Werk: |
volume:39 ; year:2009 ; number:1 ; day:29 ; month:09 ; pages:138-143 |
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| DOI / URN: |
10.1007/s11664-009-0961-6 |
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OLC2042311065 |
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| 520 | |a Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. | ||
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10.1007/s11664-009-0961-6 doi (DE-627)OLC2042311065 (DE-He213)s11664-009-0961-6-p DE-627 ger DE-627 rakwb eng 670 VZ Jiménez, J. A. verfasserin aut Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy 2009 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © TMS 2009 Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. Energy transfer nanoparticles phosphate glass silver Lysenko, S. aut Vikhnin, V. S. aut Liu, H. aut Enthalten in Journal of electronic materials Springer US, 1972 39(2009), 1 vom: 29. Sept., Seite 138-143 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:39 year:2009 number:1 day:29 month:09 pages:138-143 https://doi.org/10.1007/s11664-009-0961-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2010 GBV_ILN_2020 GBV_ILN_2021 AR 39 2009 1 29 09 138-143 |
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10.1007/s11664-009-0961-6 doi (DE-627)OLC2042311065 (DE-He213)s11664-009-0961-6-p DE-627 ger DE-627 rakwb eng 670 VZ Jiménez, J. A. verfasserin aut Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy 2009 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © TMS 2009 Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. Energy transfer nanoparticles phosphate glass silver Lysenko, S. aut Vikhnin, V. S. aut Liu, H. aut Enthalten in Journal of electronic materials Springer US, 1972 39(2009), 1 vom: 29. Sept., Seite 138-143 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:39 year:2009 number:1 day:29 month:09 pages:138-143 https://doi.org/10.1007/s11664-009-0961-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2010 GBV_ILN_2020 GBV_ILN_2021 AR 39 2009 1 29 09 138-143 |
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10.1007/s11664-009-0961-6 doi (DE-627)OLC2042311065 (DE-He213)s11664-009-0961-6-p DE-627 ger DE-627 rakwb eng 670 VZ Jiménez, J. A. verfasserin aut Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy 2009 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © TMS 2009 Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. Energy transfer nanoparticles phosphate glass silver Lysenko, S. aut Vikhnin, V. S. aut Liu, H. aut Enthalten in Journal of electronic materials Springer US, 1972 39(2009), 1 vom: 29. Sept., Seite 138-143 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:39 year:2009 number:1 day:29 month:09 pages:138-143 https://doi.org/10.1007/s11664-009-0961-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2010 GBV_ILN_2020 GBV_ILN_2021 AR 39 2009 1 29 09 138-143 |
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10.1007/s11664-009-0961-6 doi (DE-627)OLC2042311065 (DE-He213)s11664-009-0961-6-p DE-627 ger DE-627 rakwb eng 670 VZ Jiménez, J. A. verfasserin aut Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy 2009 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © TMS 2009 Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. Energy transfer nanoparticles phosphate glass silver Lysenko, S. aut Vikhnin, V. S. aut Liu, H. aut Enthalten in Journal of electronic materials Springer US, 1972 39(2009), 1 vom: 29. Sept., Seite 138-143 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:39 year:2009 number:1 day:29 month:09 pages:138-143 https://doi.org/10.1007/s11664-009-0961-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2010 GBV_ILN_2020 GBV_ILN_2021 AR 39 2009 1 29 09 138-143 |
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10.1007/s11664-009-0961-6 doi (DE-627)OLC2042311065 (DE-He213)s11664-009-0961-6-p DE-627 ger DE-627 rakwb eng 670 VZ Jiménez, J. A. verfasserin aut Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy 2009 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © TMS 2009 Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. Energy transfer nanoparticles phosphate glass silver Lysenko, S. aut Vikhnin, V. S. aut Liu, H. aut Enthalten in Journal of electronic materials Springer US, 1972 39(2009), 1 vom: 29. Sept., Seite 138-143 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:39 year:2009 number:1 day:29 month:09 pages:138-143 https://doi.org/10.1007/s11664-009-0961-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2010 GBV_ILN_2020 GBV_ILN_2021 AR 39 2009 1 29 09 138-143 |
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Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy |
| abstract |
Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. © TMS 2009 |
| abstractGer |
Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. © TMS 2009 |
| abstract_unstemmed |
Abstract Relaxation dynamics of silver nanoparticles (NPs) embedded in glass have been studied by picosecond time-resolved transient grating (TG) spectroscopy. Phosphate-based glasses were prepared by melting and heat-treatment processes by which two different nanometal-glass composites were produced. The first is a glass system containing silver and tin in which Ag NPs are embedded in the matrix upon heat treatment. The second is a heat-treated silver-doped glass with spectroscopic indications of $ Ag^{+} $–$ Ag^{0} $ pairs located at or near the surface of the NPs. The time evolution of the light-induced TG for the Ag/Sn-doped glass shows an uncommon relaxation on the nanosecond time scale. Such behavior is explained in terms of energy transfer processes between polaronic and/or excitonic states in the near-interface region of the glass matrix and the NPs. In contrast, a faster monotonic relaxation is observed for the Ag-doped nanocomposite. This result is attributed to Ag NP → $ Ag^{+} $–$ Ag^{0} $ plasmon resonance energy transfer. © TMS 2009 |
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| title_short |
Interfacial Effects in the Relaxation Dynamics of Silver Nanometal-Glass Composites Probed by Transient Grating Spectroscopy |
| url |
https://doi.org/10.1007/s11664-009-0961-6 |
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| author2 |
Lysenko, S. Vikhnin, V. S. Liu, H. |
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Lysenko, S. Vikhnin, V. S. Liu, H. |
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