A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction
Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal...
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Gespeichert in:
| Autor*in: |
Le, Hai Viet [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018 |
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| Schlagwörter: |
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| Anmerkung: |
© The Minerals, Metals & Materials Society 2018 |
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| Übergeordnetes Werk: |
Enthalten in: Journal of electronic materials - Springer US, 1972, 47(2018), 11 vom: 31. Aug., Seite 6918-6922 |
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| Übergeordnetes Werk: |
volume:47 ; year:2018 ; number:11 ; day:31 ; month:08 ; pages:6918-6922 |
| Links: |
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| DOI / URN: |
10.1007/s11664-018-6622-x |
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| Katalog-ID: |
OLC2042366048 |
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| 520 | |a Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. | ||
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10.1007/s11664-018-6622-x doi (DE-627)OLC2042366048 (DE-He213)s11664-018-6622-x-p DE-627 ger DE-627 rakwb eng 670 VZ Le, Hai Viet verfasserin aut A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction 2018 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Minerals, Metals & Materials Society 2018 Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. Metal–organic frameworks Pd nanoparticles Pd@MOFs composite hydrogen evolution reaction Nguyen, Quyen Truc Thi aut Co, Thien Thanh aut Nguyen, Phuong Kieu Thi aut Nguyen, Hoang Thai aut Enthalten in Journal of electronic materials Springer US, 1972 47(2018), 11 vom: 31. Aug., Seite 6918-6922 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:47 year:2018 number:11 day:31 month:08 pages:6918-6922 https://doi.org/10.1007/s11664-018-6622-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 AR 47 2018 11 31 08 6918-6922 |
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10.1007/s11664-018-6622-x doi (DE-627)OLC2042366048 (DE-He213)s11664-018-6622-x-p DE-627 ger DE-627 rakwb eng 670 VZ Le, Hai Viet verfasserin aut A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction 2018 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Minerals, Metals & Materials Society 2018 Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. Metal–organic frameworks Pd nanoparticles Pd@MOFs composite hydrogen evolution reaction Nguyen, Quyen Truc Thi aut Co, Thien Thanh aut Nguyen, Phuong Kieu Thi aut Nguyen, Hoang Thai aut Enthalten in Journal of electronic materials Springer US, 1972 47(2018), 11 vom: 31. Aug., Seite 6918-6922 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:47 year:2018 number:11 day:31 month:08 pages:6918-6922 https://doi.org/10.1007/s11664-018-6622-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 AR 47 2018 11 31 08 6918-6922 |
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10.1007/s11664-018-6622-x doi (DE-627)OLC2042366048 (DE-He213)s11664-018-6622-x-p DE-627 ger DE-627 rakwb eng 670 VZ Le, Hai Viet verfasserin aut A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction 2018 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Minerals, Metals & Materials Society 2018 Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. Metal–organic frameworks Pd nanoparticles Pd@MOFs composite hydrogen evolution reaction Nguyen, Quyen Truc Thi aut Co, Thien Thanh aut Nguyen, Phuong Kieu Thi aut Nguyen, Hoang Thai aut Enthalten in Journal of electronic materials Springer US, 1972 47(2018), 11 vom: 31. Aug., Seite 6918-6922 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:47 year:2018 number:11 day:31 month:08 pages:6918-6922 https://doi.org/10.1007/s11664-018-6622-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 AR 47 2018 11 31 08 6918-6922 |
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10.1007/s11664-018-6622-x doi (DE-627)OLC2042366048 (DE-He213)s11664-018-6622-x-p DE-627 ger DE-627 rakwb eng 670 VZ Le, Hai Viet verfasserin aut A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction 2018 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Minerals, Metals & Materials Society 2018 Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. Metal–organic frameworks Pd nanoparticles Pd@MOFs composite hydrogen evolution reaction Nguyen, Quyen Truc Thi aut Co, Thien Thanh aut Nguyen, Phuong Kieu Thi aut Nguyen, Hoang Thai aut Enthalten in Journal of electronic materials Springer US, 1972 47(2018), 11 vom: 31. Aug., Seite 6918-6922 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:47 year:2018 number:11 day:31 month:08 pages:6918-6922 https://doi.org/10.1007/s11664-018-6622-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 AR 47 2018 11 31 08 6918-6922 |
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10.1007/s11664-018-6622-x doi (DE-627)OLC2042366048 (DE-He213)s11664-018-6622-x-p DE-627 ger DE-627 rakwb eng 670 VZ Le, Hai Viet verfasserin aut A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction 2018 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Minerals, Metals & Materials Society 2018 Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. Metal–organic frameworks Pd nanoparticles Pd@MOFs composite hydrogen evolution reaction Nguyen, Quyen Truc Thi aut Co, Thien Thanh aut Nguyen, Phuong Kieu Thi aut Nguyen, Hoang Thai aut Enthalten in Journal of electronic materials Springer US, 1972 47(2018), 11 vom: 31. Aug., Seite 6918-6922 (DE-627)129398233 (DE-600)186069-0 (DE-576)014781387 0361-5235 nnns volume:47 year:2018 number:11 day:31 month:08 pages:6918-6922 https://doi.org/10.1007/s11664-018-6622-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 AR 47 2018 11 31 08 6918-6922 |
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A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction |
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A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction |
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Le, Hai Viet |
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2018 |
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Le, Hai Viet Nguyen, Quyen Truc Thi Co, Thien Thanh Nguyen, Phuong Kieu Thi Nguyen, Hoang Thai |
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Le, Hai Viet |
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a composite based on pd nanoparticles incorporated into a zirconium-based metal–organic frameworks zr–azobdc and its electrocatalytic activity for hydrogen evolution reaction |
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A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction |
| abstract |
Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. © The Minerals, Metals & Materials Society 2018 |
| abstractGer |
Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. © The Minerals, Metals & Materials Society 2018 |
| abstract_unstemmed |
Abstract This work presents the results of the synthesis and characterization of a composite material from a zirconium-based metal–organic framework (Zr–AzoBDC) and Pd nanoparticles. Zr–AzoBDC was synthesized from Zr(IV) salt and azobenzene-4,4′-dicarboxylic acid (AzoBDC) linker by a solvent–thermal method. The PdZr–AzoBDC composite was prepared via two stages (1) absorption of Pd ions into the Zr–AzoBDC, and (2) reduction of the Pd ions by $ NaBH_{4} $. The structure of Zr–AzoBDC and composite were studied by powder x-ray diffraction measurements. The morphology and chemical composition of the composite were analyzed via the FESEM/energy dispersive x-ray method. Electro-catalytic properties of the Zr–AzoBDC support and Pd@Zr–AzoBDC composite were examined by the cyclic voltammetry method in 0.5 M $ Na_{2} $$ SO_{4} $ aqueous solution. The results showed that the amount of Pd in the as-prepared composite was ca. 4.5%. The Pd@Zr–AzoBDC composite was found to be stable in water and showed very good catalytic activity for the hydrogen evolution reaction. The overpotential requirement to achieve a catalytic current density of 1.0 mA $ cm^{2} $ and 10 mA $ cm^{−2} $ was ca. 300 mV and 800 mV versus RHE, respectively. © The Minerals, Metals & Materials Society 2018 |
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A Composite Based on Pd Nanoparticles Incorporated into a Zirconium-Based Metal–Organic Frameworks Zr–AzoBDC and Its Electrocatalytic Activity for Hydrogen Evolution Reaction |
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Nguyen, Quyen Truc Thi Co, Thien Thanh Nguyen, Phuong Kieu Thi Nguyen, Hoang Thai |
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