Heterodyne detected transient gratings in supercooled molecular liquids

Abstract. We present an analysis, based on a phenomenological set of Generalised Navier-Stokes equations, of Heterodyne Detected Transient Gratings on supercooled molecular liquids of anisotropic molecules. This set of equations generalises equations proven in Franosch, Latz and Pick [24] for the sa...
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Autor*in:	Pick, R. M. [verfasserIn] Dreyfus, C. Azzimani, A. Gupta, R. Torre, R. Taschin, A. Franosch, T.

Format:	Artikel
Sprache:	Englisch

Erschienen:	2004

Schlagwörter:	Response Function Temperature Evolution Elementary Response Temperature Behaviour Laplace Transform

Systematik:	UA 3858.B

Anmerkung:	© Springer-Verlag Berlin/Heidelberg 2004

Übergeordnetes Werk:	Enthalten in: The European physical journal / B - Springer-Verlag, 1998, 39(2004), 2 vom: Mai, Seite 169-197
Übergeordnetes Werk:	volume:39 ; year:2004 ; number:2 ; month:05 ; pages:169-197

Links:	Volltext

DOI / URN:	10.1140/epjb/e2004-00181-2

Katalog-ID:	OLC2065646594

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spelling	10.1140/epjb/e2004-00181-2 doi (DE-627)OLC2065646594 (DE-He213)e2004-00181-2-p DE-627 ger DE-627 rakwb eng 530 VZ 530 VZ UA 3858.B VZ rvk Pick, R. M. verfasserin aut Heterodyne detected transient gratings in supercooled molecular liquids 2004 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin/Heidelberg 2004 Abstract. We present an analysis, based on a phenomenological set of Generalised Navier-Stokes equations, of Heterodyne Detected Transient Gratings on supercooled molecular liquids of anisotropic molecules. This set of equations generalises equations proven in Franosch, Latz and Pick [24] for the same type of liquids. It also takes into account the three different sources generated by the laser pumping process pertinent for these experiments. We give analytical expressions for the response functions that can be measured using the different polarisation of the experimental set-up. Specialising to the case of parallel polarisation (where longitudinal phonons are launched), we show that each response function is a sum of the same seven “elementary response functions” (ERFs) whose time and temperature evolutions are individually analysed. We also show that the response functions corresponding to two of the sources can be directly connected to the Laplace Transform of a light scattering signal. The ERFs generated by the heat-absorption process, which is the third source, are of a different nature. They do not have the same time and temperature behaviours and they can provide, inter alia, unique information on the rotation-translation coupling function characteristic of these liquids. Response Function Temperature Evolution Elementary Response Temperature Behaviour Laplace Transform Dreyfus, C. aut Azzimani, A. aut Gupta, R. aut Torre, R. aut Taschin, A. aut Franosch, T. aut Enthalten in The European physical journal / B Springer-Verlag, 1998 39(2004), 2 vom: Mai, Seite 169-197 (DE-627)235469769 (DE-600)1397768-4 (DE-576)061879142 1434-6028 nnns volume:39 year:2004 number:2 month:05 pages:169-197 https://doi.org/10.1140/epjb/e2004-00181-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_30 GBV_ILN_31 GBV_ILN_40 GBV_ILN_62 GBV_ILN_65 GBV_ILN_70 GBV_ILN_100 GBV_ILN_105 GBV_ILN_120 GBV_ILN_130 GBV_ILN_170 GBV_ILN_267 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2010 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2185 GBV_ILN_4029 GBV_ILN_4116 GBV_ILN_4126 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4317 GBV_ILN_4700 UA 3858.B AR 39 2004 2 05 169-197
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author	Pick, R. M.
spellingShingle	Pick, R. M. ddc 530 rvk UA 3858.B misc Response Function misc Temperature Evolution misc Elementary Response misc Temperature Behaviour misc Laplace Transform Heterodyne detected transient gratings in supercooled molecular liquids
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title	Heterodyne detected transient gratings in supercooled molecular liquids
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title_full	Heterodyne detected transient gratings in supercooled molecular liquids
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title_sort	heterodyne detected transient gratings in supercooled molecular liquids
title_auth	Heterodyne detected transient gratings in supercooled molecular liquids
abstract	Abstract. We present an analysis, based on a phenomenological set of Generalised Navier-Stokes equations, of Heterodyne Detected Transient Gratings on supercooled molecular liquids of anisotropic molecules. This set of equations generalises equations proven in Franosch, Latz and Pick [24] for the same type of liquids. It also takes into account the three different sources generated by the laser pumping process pertinent for these experiments. We give analytical expressions for the response functions that can be measured using the different polarisation of the experimental set-up. Specialising to the case of parallel polarisation (where longitudinal phonons are launched), we show that each response function is a sum of the same seven “elementary response functions” (ERFs) whose time and temperature evolutions are individually analysed. We also show that the response functions corresponding to two of the sources can be directly connected to the Laplace Transform of a light scattering signal. The ERFs generated by the heat-absorption process, which is the third source, are of a different nature. They do not have the same time and temperature behaviours and they can provide, inter alia, unique information on the rotation-translation coupling function characteristic of these liquids. © Springer-Verlag Berlin/Heidelberg 2004
abstractGer	Abstract. We present an analysis, based on a phenomenological set of Generalised Navier-Stokes equations, of Heterodyne Detected Transient Gratings on supercooled molecular liquids of anisotropic molecules. This set of equations generalises equations proven in Franosch, Latz and Pick [24] for the same type of liquids. It also takes into account the three different sources generated by the laser pumping process pertinent for these experiments. We give analytical expressions for the response functions that can be measured using the different polarisation of the experimental set-up. Specialising to the case of parallel polarisation (where longitudinal phonons are launched), we show that each response function is a sum of the same seven “elementary response functions” (ERFs) whose time and temperature evolutions are individually analysed. We also show that the response functions corresponding to two of the sources can be directly connected to the Laplace Transform of a light scattering signal. The ERFs generated by the heat-absorption process, which is the third source, are of a different nature. They do not have the same time and temperature behaviours and they can provide, inter alia, unique information on the rotation-translation coupling function characteristic of these liquids. © Springer-Verlag Berlin/Heidelberg 2004
abstract_unstemmed	Abstract. We present an analysis, based on a phenomenological set of Generalised Navier-Stokes equations, of Heterodyne Detected Transient Gratings on supercooled molecular liquids of anisotropic molecules. This set of equations generalises equations proven in Franosch, Latz and Pick [24] for the same type of liquids. It also takes into account the three different sources generated by the laser pumping process pertinent for these experiments. We give analytical expressions for the response functions that can be measured using the different polarisation of the experimental set-up. Specialising to the case of parallel polarisation (where longitudinal phonons are launched), we show that each response function is a sum of the same seven “elementary response functions” (ERFs) whose time and temperature evolutions are individually analysed. We also show that the response functions corresponding to two of the sources can be directly connected to the Laplace Transform of a light scattering signal. The ERFs generated by the heat-absorption process, which is the third source, are of a different nature. They do not have the same time and temperature behaviours and they can provide, inter alia, unique information on the rotation-translation coupling function characteristic of these liquids. © Springer-Verlag Berlin/Heidelberg 2004
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title_short	Heterodyne detected transient gratings in supercooled molecular liquids
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