Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas
Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi...
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| Autor*in: |
Lester, G. W. [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2013 |
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| Anmerkung: |
© Springer-Verlag Berlin Heidelberg 2013 |
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| Übergeordnetes Werk: |
Enthalten in: Contributions to mineralogy and petrology - Springer-Verlag, 1966, 166(2013), 1 vom: 16. Mai, Seite 329-349 |
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| Übergeordnetes Werk: |
volume:166 ; year:2013 ; number:1 ; day:16 ; month:05 ; pages:329-349 |
| Links: |
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| DOI / URN: |
10.1007/s00410-013-0878-1 |
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| Katalog-ID: |
OLC2070532372 |
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| 245 | 1 | 0 | |a Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas |
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| 520 | |a Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. | ||
| 650 | 4 | |a Immiscible oxide melts | |
| 650 | 4 | |a Immiscible magma | |
| 650 | 4 | |a Two-liquid partitioning | |
| 650 | 4 | |a Immiscible | |
| 700 | 1 | |a Clark, A. H. |4 aut | |
| 700 | 1 | |a Kyser, T. K. |4 aut | |
| 700 | 1 | |a Naslund, H. R. |4 aut | |
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10.1007/s00410-013-0878-1 doi (DE-627)OLC2070532372 (DE-He213)s00410-013-0878-1-p DE-627 ger DE-627 rakwb eng 550 VZ 13 ssgn TE 1000 VZ rvk Lester, G. W. verfasserin aut Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas 2013 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2013 Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. Immiscible oxide melts Immiscible magma Two-liquid partitioning Immiscible Clark, A. H. aut Kyser, T. K. aut Naslund, H. R. aut Enthalten in Contributions to mineralogy and petrology Springer-Verlag, 1966 166(2013), 1 vom: 16. Mai, Seite 329-349 (DE-627)129068721 (DE-600)1616-0 (DE-576)014400367 0010-7999 nnns volume:166 year:2013 number:1 day:16 month:05 pages:329-349 https://doi.org/10.1007/s00410-013-0878-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-GEO SSG-OPC-GGO GBV_ILN_30 GBV_ILN_40 GBV_ILN_70 GBV_ILN_381 GBV_ILN_2018 GBV_ILN_2027 GBV_ILN_4277 GBV_ILN_4323 TE 1000 AR 166 2013 1 16 05 329-349 |
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10.1007/s00410-013-0878-1 doi (DE-627)OLC2070532372 (DE-He213)s00410-013-0878-1-p DE-627 ger DE-627 rakwb eng 550 VZ 13 ssgn TE 1000 VZ rvk Lester, G. W. verfasserin aut Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas 2013 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2013 Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. Immiscible oxide melts Immiscible magma Two-liquid partitioning Immiscible Clark, A. H. aut Kyser, T. K. aut Naslund, H. R. aut Enthalten in Contributions to mineralogy and petrology Springer-Verlag, 1966 166(2013), 1 vom: 16. Mai, Seite 329-349 (DE-627)129068721 (DE-600)1616-0 (DE-576)014400367 0010-7999 nnns volume:166 year:2013 number:1 day:16 month:05 pages:329-349 https://doi.org/10.1007/s00410-013-0878-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-GEO SSG-OPC-GGO GBV_ILN_30 GBV_ILN_40 GBV_ILN_70 GBV_ILN_381 GBV_ILN_2018 GBV_ILN_2027 GBV_ILN_4277 GBV_ILN_4323 TE 1000 AR 166 2013 1 16 05 329-349 |
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10.1007/s00410-013-0878-1 doi (DE-627)OLC2070532372 (DE-He213)s00410-013-0878-1-p DE-627 ger DE-627 rakwb eng 550 VZ 13 ssgn TE 1000 VZ rvk Lester, G. W. verfasserin aut Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas 2013 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2013 Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. Immiscible oxide melts Immiscible magma Two-liquid partitioning Immiscible Clark, A. H. aut Kyser, T. K. aut Naslund, H. R. aut Enthalten in Contributions to mineralogy and petrology Springer-Verlag, 1966 166(2013), 1 vom: 16. Mai, Seite 329-349 (DE-627)129068721 (DE-600)1616-0 (DE-576)014400367 0010-7999 nnns volume:166 year:2013 number:1 day:16 month:05 pages:329-349 https://doi.org/10.1007/s00410-013-0878-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-GEO SSG-OPC-GGO GBV_ILN_30 GBV_ILN_40 GBV_ILN_70 GBV_ILN_381 GBV_ILN_2018 GBV_ILN_2027 GBV_ILN_4277 GBV_ILN_4323 TE 1000 AR 166 2013 1 16 05 329-349 |
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10.1007/s00410-013-0878-1 doi (DE-627)OLC2070532372 (DE-He213)s00410-013-0878-1-p DE-627 ger DE-627 rakwb eng 550 VZ 13 ssgn TE 1000 VZ rvk Lester, G. W. verfasserin aut Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas 2013 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2013 Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. Immiscible oxide melts Immiscible magma Two-liquid partitioning Immiscible Clark, A. H. aut Kyser, T. K. aut Naslund, H. R. aut Enthalten in Contributions to mineralogy and petrology Springer-Verlag, 1966 166(2013), 1 vom: 16. Mai, Seite 329-349 (DE-627)129068721 (DE-600)1616-0 (DE-576)014400367 0010-7999 nnns volume:166 year:2013 number:1 day:16 month:05 pages:329-349 https://doi.org/10.1007/s00410-013-0878-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-GEO SSG-OPC-GGO GBV_ILN_30 GBV_ILN_40 GBV_ILN_70 GBV_ILN_381 GBV_ILN_2018 GBV_ILN_2027 GBV_ILN_4277 GBV_ILN_4323 TE 1000 AR 166 2013 1 16 05 329-349 |
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10.1007/s00410-013-0878-1 doi (DE-627)OLC2070532372 (DE-He213)s00410-013-0878-1-p DE-627 ger DE-627 rakwb eng 550 VZ 13 ssgn TE 1000 VZ rvk Lester, G. W. verfasserin aut Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas 2013 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2013 Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. Immiscible oxide melts Immiscible magma Two-liquid partitioning Immiscible Clark, A. H. aut Kyser, T. K. aut Naslund, H. R. aut Enthalten in Contributions to mineralogy and petrology Springer-Verlag, 1966 166(2013), 1 vom: 16. Mai, Seite 329-349 (DE-627)129068721 (DE-600)1616-0 (DE-576)014400367 0010-7999 nnns volume:166 year:2013 number:1 day:16 month:05 pages:329-349 https://doi.org/10.1007/s00410-013-0878-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-GEO SSG-OPC-GGO GBV_ILN_30 GBV_ILN_40 GBV_ILN_70 GBV_ILN_381 GBV_ILN_2018 GBV_ILN_2027 GBV_ILN_4277 GBV_ILN_4323 TE 1000 AR 166 2013 1 16 05 329-349 |
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Lester, G. W. |
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Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas |
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experiments on liquid immiscibility in silicate melts with $ h_{2} $o, p, s, f and cl: implications for natural magmas |
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Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas |
| abstract |
Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. © Springer-Verlag Berlin Heidelberg 2013 |
| abstractGer |
Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. © Springer-Verlag Berlin Heidelberg 2013 |
| abstract_unstemmed |
Abstract Isobaric (200 MPa) experiments have been performed to investigate the effects of $ H_{2} $O alone or in combination with P, S, F or Cl on liquid-phase separation in melts in the systems $ Fe_{2} $$ SiO_{4} $–$ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $, $ Fe_{3} $$ O_{4} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ and $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ with or without plagioclase ($ An_{50} $). Experiments were heated in a rapid-quench internally heated pressure vessel at 1,075, 1,150 or 1,200 °C for 2 h. Experimental f$ O_{2} $ was maintained at QFM, NNO or MH oxygen buffers. $ H_{2} $O alone or in combination with P, S or F increases the temperature and composition range of two-liquid fields at f$ O_{2} $ = NNO and MH buffers. P, S, F and Cl partition preferentially into the Fe-rich immiscible liquid. Two-liquid partition coefficients for Fe, Si, P and S correlate well with the degree of polymerization of the $ SiO_{2} $-rich liquid and plot on similar but distinct power-law curves compared with equivalent anhydrous or basaltic melts. The addition of 2 wt% S to the system $ Fe_{3} $$ O_{4} $–$ Fe_{2} $$ O_{3} $–$ KAlSi_{2} $$ O_{6} $–$ SiO_{2} $ stabilizes three immiscible melts with Fe-, FeS- and Si-rich compositions. $ H_{2} $O-induced suppression of liquidus temperatures in the experimental systems, considered with the effects of pressure on the temperature and composition ranges of two-liquid fields in silicate melts, suggests that liquid-phase separation may be stable in some $ H_{2} $O-rich silicate magmas at pressures in excess of 200 MPa. © Springer-Verlag Berlin Heidelberg 2013 |
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Experiments on liquid immiscibility in silicate melts with $ H_{2} $O, P, S, F and Cl: implications for natural magmas |
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