Absorption-edge calculations of inorganic nonlinear optical crystals
Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wu, Kechen [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
1992 |
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| Systematik: |
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| Anmerkung: |
© Springer-Verlag 1992 |
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| Übergeordnetes Werk: |
Enthalten in: Applied physics. A, Materials science & processing - Springer-Verlag, 1981, 54(1992), 3 vom: März, Seite 209-220 |
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| Übergeordnetes Werk: |
volume:54 ; year:1992 ; number:3 ; month:03 ; pages:209-220 |
| Links: |
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| DOI / URN: |
10.1007/BF00323839 |
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| Katalog-ID: |
OLC2074124392 |
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| 520 | |a Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. | ||
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10.1007/BF00323839 doi (DE-627)OLC2074124392 (DE-He213)BF00323839-p DE-627 ger DE-627 rakwb eng 530 620 VZ 530 VZ UA 9001.A VZ rvk Wu, Kechen verfasserin aut Absorption-edge calculations of inorganic nonlinear optical crystals 1992 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag 1992 Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. Chen, Chuangtian aut Enthalten in Applied physics. A, Materials science & processing Springer-Verlag, 1981 54(1992), 3 vom: März, Seite 209-220 (DE-627)129861340 (DE-600)283365-7 (DE-576)015171930 0947-8396 nnns volume:54 year:1992 number:3 month:03 pages:209-220 https://doi.org/10.1007/BF00323839 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_30 GBV_ILN_31 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_70 GBV_ILN_105 GBV_ILN_121 GBV_ILN_130 GBV_ILN_170 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4126 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4313 GBV_ILN_4315 GBV_ILN_4318 GBV_ILN_4319 GBV_ILN_4323 GBV_ILN_4700 UA 9001.A AR 54 1992 3 03 209-220 |
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10.1007/BF00323839 doi (DE-627)OLC2074124392 (DE-He213)BF00323839-p DE-627 ger DE-627 rakwb eng 530 620 VZ 530 VZ UA 9001.A VZ rvk Wu, Kechen verfasserin aut Absorption-edge calculations of inorganic nonlinear optical crystals 1992 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag 1992 Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. Chen, Chuangtian aut Enthalten in Applied physics. A, Materials science & processing Springer-Verlag, 1981 54(1992), 3 vom: März, Seite 209-220 (DE-627)129861340 (DE-600)283365-7 (DE-576)015171930 0947-8396 nnns volume:54 year:1992 number:3 month:03 pages:209-220 https://doi.org/10.1007/BF00323839 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_30 GBV_ILN_31 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_70 GBV_ILN_105 GBV_ILN_121 GBV_ILN_130 GBV_ILN_170 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4126 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4313 GBV_ILN_4315 GBV_ILN_4318 GBV_ILN_4319 GBV_ILN_4323 GBV_ILN_4700 UA 9001.A AR 54 1992 3 03 209-220 |
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10.1007/BF00323839 doi (DE-627)OLC2074124392 (DE-He213)BF00323839-p DE-627 ger DE-627 rakwb eng 530 620 VZ 530 VZ UA 9001.A VZ rvk Wu, Kechen verfasserin aut Absorption-edge calculations of inorganic nonlinear optical crystals 1992 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag 1992 Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. Chen, Chuangtian aut Enthalten in Applied physics. A, Materials science & processing Springer-Verlag, 1981 54(1992), 3 vom: März, Seite 209-220 (DE-627)129861340 (DE-600)283365-7 (DE-576)015171930 0947-8396 nnns volume:54 year:1992 number:3 month:03 pages:209-220 https://doi.org/10.1007/BF00323839 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_30 GBV_ILN_31 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_70 GBV_ILN_105 GBV_ILN_121 GBV_ILN_130 GBV_ILN_170 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4126 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4313 GBV_ILN_4315 GBV_ILN_4318 GBV_ILN_4319 GBV_ILN_4323 GBV_ILN_4700 UA 9001.A AR 54 1992 3 03 209-220 |
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10.1007/BF00323839 doi (DE-627)OLC2074124392 (DE-He213)BF00323839-p DE-627 ger DE-627 rakwb eng 530 620 VZ 530 VZ UA 9001.A VZ rvk Wu, Kechen verfasserin aut Absorption-edge calculations of inorganic nonlinear optical crystals 1992 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag 1992 Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. Chen, Chuangtian aut Enthalten in Applied physics. A, Materials science & processing Springer-Verlag, 1981 54(1992), 3 vom: März, Seite 209-220 (DE-627)129861340 (DE-600)283365-7 (DE-576)015171930 0947-8396 nnns volume:54 year:1992 number:3 month:03 pages:209-220 https://doi.org/10.1007/BF00323839 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_30 GBV_ILN_31 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_70 GBV_ILN_105 GBV_ILN_121 GBV_ILN_130 GBV_ILN_170 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4126 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4313 GBV_ILN_4315 GBV_ILN_4318 GBV_ILN_4319 GBV_ILN_4323 GBV_ILN_4700 UA 9001.A AR 54 1992 3 03 209-220 |
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10.1007/BF00323839 doi (DE-627)OLC2074124392 (DE-He213)BF00323839-p DE-627 ger DE-627 rakwb eng 530 620 VZ 530 VZ UA 9001.A VZ rvk Wu, Kechen verfasserin aut Absorption-edge calculations of inorganic nonlinear optical crystals 1992 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag 1992 Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. Chen, Chuangtian aut Enthalten in Applied physics. A, Materials science & processing Springer-Verlag, 1981 54(1992), 3 vom: März, Seite 209-220 (DE-627)129861340 (DE-600)283365-7 (DE-576)015171930 0947-8396 nnns volume:54 year:1992 number:3 month:03 pages:209-220 https://doi.org/10.1007/BF00323839 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_30 GBV_ILN_31 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_70 GBV_ILN_105 GBV_ILN_121 GBV_ILN_130 GBV_ILN_170 GBV_ILN_2004 GBV_ILN_2006 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4126 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4313 GBV_ILN_4315 GBV_ILN_4318 GBV_ILN_4319 GBV_ILN_4323 GBV_ILN_4700 UA 9001.A AR 54 1992 3 03 209-220 |
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Enthalten in Applied physics. A, Materials science & processing 54(1992), 3 vom: März, Seite 209-220 volume:54 year:1992 number:3 month:03 pages:209-220 |
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Enthalten in Applied physics. A, Materials science & processing 54(1992), 3 vom: März, Seite 209-220 volume:54 year:1992 number:3 month:03 pages:209-220 |
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absorption-edge calculations of inorganic nonlinear optical crystals |
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Absorption-edge calculations of inorganic nonlinear optical crystals |
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Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. © Springer-Verlag 1992 |
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Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. © Springer-Verlag 1992 |
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Abstract A theoretical model suitable for calculating absorption edges of inorganic nonlinear optical (NLO) crystals is introduced. This model is proved to be useful to elucidate the relationship between electronic structures of NLO-active groups and macroscopic properties of absorption edges on the UV side of most of the inorganic nonlinear optical crystals. A systematic calculation of absorption edges on the UV side for several important inorganic NLO crystals is carried out by means of DV-SCM-$ X_{α} $ method and all calculated results are in good agreement with experimental data. These inorganic NLO crystals include $ LiB_{3} $$ O_{5} $(LBO), β-$ BaB_{2} $$ O_{4} $(BBO), KB5, KDP, $ Na_{2} $$ SbF_{5} $, $ Ba_{2} $$ TiSi_{2} $$ O_{8} $, iodate and $ NaNO_{2} $. The calculated energy level structures of $ LiB_{3} $$ O_{5} $ and β-$ BaB_{2} $$ O_{4} $ crystals are compared with the measured XPS spectra. The unusual transparent spectra of KB5 and KDP crystals are partly explained from the microstructure point of view. The effect of lone electron pair in iodate and $ NaNO_{2} $ crystals on their absorption edges are discussed. All these results show that Anionic Group Theory of Nonlinear Optical Crystals is useful to evaluate the absorption edges of the inorganic nonlinear optical crystal and is a powerful tool in a Molecular Engineering approach to search for new nonlinear optical materials. © Springer-Verlag 1992 |
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