Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface
Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of speci...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Noiriel, Catherine [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer Nature B.V. 2021 |
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| Übergeordnetes Werk: |
Enthalten in: Transport in porous media - Springer Netherlands, 1986, 140(2021), 1 vom: 21. Mai, Seite 181-213 |
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| Übergeordnetes Werk: |
volume:140 ; year:2021 ; number:1 ; day:21 ; month:05 ; pages:181-213 |
| Links: |
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| DOI / URN: |
10.1007/s11242-021-01613-2 |
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OLC2077197382 |
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| 520 | |a Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of species as well as a strong dependence on the physical, chemical, mineralogical and structural properties of the reacting solid phases. In this article, we review the recent advances in pore-scale imaging and reactive flow modelling applied to interface dynamics. Digital rocks derived from time-lapse X-ray micro-tomography imaging gives unprecedented opportunity to track the interface evolution during reactive flow experiments in porous or fractured media, and evaluate locally mineral reactivity. The recent improvements in pore-scale reactive transport modelling allow for a fine description of flow and transport that integrates moving fluid–mineral interfaces inherent to chemical reactions. Combined with three-dimensional digital images, pore-scale reactive transport modelling complements and augments laboratory experiments. The most advanced multi-scale models integrate sub-voxel porosity and processes which relate to imaging instrument resolution and improve upscaling possibilities. Two example applications based on the solver porousMedia4Foam illustrate the dynamics of the interface for different transport regimes (i.e., diffusive- to advective-dominant) and rock matrix properties (i.e., permeable vs. impermeable, and homogeneous vs. polymineralic). These parameters affect both the interface roughness and its geometry evolution, from sharp front to smeared (i.e., diffuse) interface. The paper concludes by discussing the challenges associated with precipitation processes in porous media, rock texture and composition (i.e., physical and mineralogical heterogeneity), and upscaling to larger scales. | ||
| 650 | 4 | |a Reactive flow | |
| 650 | 4 | |a Mineral reactivity | |
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10.1007/s11242-021-01613-2 doi (DE-627)OLC2077197382 (DE-He213)s11242-021-01613-2-p DE-627 ger DE-627 rakwb eng 530 VZ Noiriel, Catherine verfasserin (orcid)0000-0002-6283-1155 aut Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface 2021 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2021 Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of species as well as a strong dependence on the physical, chemical, mineralogical and structural properties of the reacting solid phases. In this article, we review the recent advances in pore-scale imaging and reactive flow modelling applied to interface dynamics. Digital rocks derived from time-lapse X-ray micro-tomography imaging gives unprecedented opportunity to track the interface evolution during reactive flow experiments in porous or fractured media, and evaluate locally mineral reactivity. The recent improvements in pore-scale reactive transport modelling allow for a fine description of flow and transport that integrates moving fluid–mineral interfaces inherent to chemical reactions. Combined with three-dimensional digital images, pore-scale reactive transport modelling complements and augments laboratory experiments. The most advanced multi-scale models integrate sub-voxel porosity and processes which relate to imaging instrument resolution and improve upscaling possibilities. Two example applications based on the solver porousMedia4Foam illustrate the dynamics of the interface for different transport regimes (i.e., diffusive- to advective-dominant) and rock matrix properties (i.e., permeable vs. impermeable, and homogeneous vs. polymineralic). These parameters affect both the interface roughness and its geometry evolution, from sharp front to smeared (i.e., diffuse) interface. The paper concludes by discussing the challenges associated with precipitation processes in porous media, rock texture and composition (i.e., physical and mineralogical heterogeneity), and upscaling to larger scales. Reactive flow Mineral reactivity X-ray micro-tomography Digital rock physics Fluid–mineral interface Fluid–rock interface Carbonate dissolution Pore-scale imaging Pore-scale modelling Darcy–Brinkman model Soulaine, Cyprien (orcid)0000-0002-6151-3286 aut Enthalten in Transport in porous media Springer Netherlands, 1986 140(2021), 1 vom: 21. Mai, Seite 181-213 (DE-627)129206105 (DE-600)54858-3 (DE-576)014457431 0169-3913 nnns volume:140 year:2021 number:1 day:21 month:05 pages:181-213 https://doi.org/10.1007/s11242-021-01613-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY AR 140 2021 1 21 05 181-213 |
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10.1007/s11242-021-01613-2 doi (DE-627)OLC2077197382 (DE-He213)s11242-021-01613-2-p DE-627 ger DE-627 rakwb eng 530 VZ Noiriel, Catherine verfasserin (orcid)0000-0002-6283-1155 aut Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface 2021 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2021 Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of species as well as a strong dependence on the physical, chemical, mineralogical and structural properties of the reacting solid phases. In this article, we review the recent advances in pore-scale imaging and reactive flow modelling applied to interface dynamics. Digital rocks derived from time-lapse X-ray micro-tomography imaging gives unprecedented opportunity to track the interface evolution during reactive flow experiments in porous or fractured media, and evaluate locally mineral reactivity. The recent improvements in pore-scale reactive transport modelling allow for a fine description of flow and transport that integrates moving fluid–mineral interfaces inherent to chemical reactions. Combined with three-dimensional digital images, pore-scale reactive transport modelling complements and augments laboratory experiments. The most advanced multi-scale models integrate sub-voxel porosity and processes which relate to imaging instrument resolution and improve upscaling possibilities. Two example applications based on the solver porousMedia4Foam illustrate the dynamics of the interface for different transport regimes (i.e., diffusive- to advective-dominant) and rock matrix properties (i.e., permeable vs. impermeable, and homogeneous vs. polymineralic). These parameters affect both the interface roughness and its geometry evolution, from sharp front to smeared (i.e., diffuse) interface. The paper concludes by discussing the challenges associated with precipitation processes in porous media, rock texture and composition (i.e., physical and mineralogical heterogeneity), and upscaling to larger scales. Reactive flow Mineral reactivity X-ray micro-tomography Digital rock physics Fluid–mineral interface Fluid–rock interface Carbonate dissolution Pore-scale imaging Pore-scale modelling Darcy–Brinkman model Soulaine, Cyprien (orcid)0000-0002-6151-3286 aut Enthalten in Transport in porous media Springer Netherlands, 1986 140(2021), 1 vom: 21. Mai, Seite 181-213 (DE-627)129206105 (DE-600)54858-3 (DE-576)014457431 0169-3913 nnns volume:140 year:2021 number:1 day:21 month:05 pages:181-213 https://doi.org/10.1007/s11242-021-01613-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY AR 140 2021 1 21 05 181-213 |
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530 VZ Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface Reactive flow Mineral reactivity X-ray micro-tomography Digital rock physics Fluid–mineral interface Fluid–rock interface Carbonate dissolution Pore-scale imaging Pore-scale modelling Darcy–Brinkman model |
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ddc 530 misc Reactive flow misc Mineral reactivity misc X-ray micro-tomography misc Digital rock physics misc Fluid–mineral interface misc Fluid–rock interface misc Carbonate dissolution misc Pore-scale imaging misc Pore-scale modelling misc Darcy–Brinkman model |
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ddc 530 misc Reactive flow misc Mineral reactivity misc X-ray micro-tomography misc Digital rock physics misc Fluid–mineral interface misc Fluid–rock interface misc Carbonate dissolution misc Pore-scale imaging misc Pore-scale modelling misc Darcy–Brinkman model |
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ddc 530 misc Reactive flow misc Mineral reactivity misc X-ray micro-tomography misc Digital rock physics misc Fluid–mineral interface misc Fluid–rock interface misc Carbonate dissolution misc Pore-scale imaging misc Pore-scale modelling misc Darcy–Brinkman model |
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Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface |
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Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface |
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Noiriel, Catherine |
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Noiriel, Catherine Soulaine, Cyprien |
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pore-scale imaging and modelling of reactive flow in evolving porous media: tracking the dynamics of the fluid–rock interface |
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Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface |
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Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of species as well as a strong dependence on the physical, chemical, mineralogical and structural properties of the reacting solid phases. In this article, we review the recent advances in pore-scale imaging and reactive flow modelling applied to interface dynamics. Digital rocks derived from time-lapse X-ray micro-tomography imaging gives unprecedented opportunity to track the interface evolution during reactive flow experiments in porous or fractured media, and evaluate locally mineral reactivity. The recent improvements in pore-scale reactive transport modelling allow for a fine description of flow and transport that integrates moving fluid–mineral interfaces inherent to chemical reactions. Combined with three-dimensional digital images, pore-scale reactive transport modelling complements and augments laboratory experiments. The most advanced multi-scale models integrate sub-voxel porosity and processes which relate to imaging instrument resolution and improve upscaling possibilities. Two example applications based on the solver porousMedia4Foam illustrate the dynamics of the interface for different transport regimes (i.e., diffusive- to advective-dominant) and rock matrix properties (i.e., permeable vs. impermeable, and homogeneous vs. polymineralic). These parameters affect both the interface roughness and its geometry evolution, from sharp front to smeared (i.e., diffuse) interface. The paper concludes by discussing the challenges associated with precipitation processes in porous media, rock texture and composition (i.e., physical and mineralogical heterogeneity), and upscaling to larger scales. © The Author(s), under exclusive licence to Springer Nature B.V. 2021 |
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Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of species as well as a strong dependence on the physical, chemical, mineralogical and structural properties of the reacting solid phases. In this article, we review the recent advances in pore-scale imaging and reactive flow modelling applied to interface dynamics. Digital rocks derived from time-lapse X-ray micro-tomography imaging gives unprecedented opportunity to track the interface evolution during reactive flow experiments in porous or fractured media, and evaluate locally mineral reactivity. The recent improvements in pore-scale reactive transport modelling allow for a fine description of flow and transport that integrates moving fluid–mineral interfaces inherent to chemical reactions. Combined with three-dimensional digital images, pore-scale reactive transport modelling complements and augments laboratory experiments. The most advanced multi-scale models integrate sub-voxel porosity and processes which relate to imaging instrument resolution and improve upscaling possibilities. Two example applications based on the solver porousMedia4Foam illustrate the dynamics of the interface for different transport regimes (i.e., diffusive- to advective-dominant) and rock matrix properties (i.e., permeable vs. impermeable, and homogeneous vs. polymineralic). These parameters affect both the interface roughness and its geometry evolution, from sharp front to smeared (i.e., diffuse) interface. The paper concludes by discussing the challenges associated with precipitation processes in porous media, rock texture and composition (i.e., physical and mineralogical heterogeneity), and upscaling to larger scales. © The Author(s), under exclusive licence to Springer Nature B.V. 2021 |
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Abstract Fluid–mineral and fluid–rock interfaces are key parameters controlling the reactivity and fate of fluids in reservoir rocks and aquifers. The interface dynamics through space and time results from complex processes involving a tight coupling between chemical reactions and transport of species as well as a strong dependence on the physical, chemical, mineralogical and structural properties of the reacting solid phases. In this article, we review the recent advances in pore-scale imaging and reactive flow modelling applied to interface dynamics. Digital rocks derived from time-lapse X-ray micro-tomography imaging gives unprecedented opportunity to track the interface evolution during reactive flow experiments in porous or fractured media, and evaluate locally mineral reactivity. The recent improvements in pore-scale reactive transport modelling allow for a fine description of flow and transport that integrates moving fluid–mineral interfaces inherent to chemical reactions. Combined with three-dimensional digital images, pore-scale reactive transport modelling complements and augments laboratory experiments. The most advanced multi-scale models integrate sub-voxel porosity and processes which relate to imaging instrument resolution and improve upscaling possibilities. Two example applications based on the solver porousMedia4Foam illustrate the dynamics of the interface for different transport regimes (i.e., diffusive- to advective-dominant) and rock matrix properties (i.e., permeable vs. impermeable, and homogeneous vs. polymineralic). These parameters affect both the interface roughness and its geometry evolution, from sharp front to smeared (i.e., diffuse) interface. The paper concludes by discussing the challenges associated with precipitation processes in porous media, rock texture and composition (i.e., physical and mineralogical heterogeneity), and upscaling to larger scales. © The Author(s), under exclusive licence to Springer Nature B.V. 2021 |
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Pore-Scale Imaging and Modelling of Reactive Flow in Evolving Porous Media: Tracking the Dynamics of the Fluid–Rock Interface |
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