Length effect of ceria nanorod on its oxygen vacancy formation and photocatalytic property
Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concent...
Ausführliche Beschreibung
Autor*in: |
Zhang, Junshan [verfasserIn] |
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Englisch |
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2022 |
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Anmerkung: |
© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
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Übergeordnetes Werk: |
Enthalten in: Journal of materials science / Materials in electronics - Springer US, 1990, 33(2022), 7 vom: 12. Jan., Seite 4628-4642 |
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Übergeordnetes Werk: |
volume:33 ; year:2022 ; number:7 ; day:12 ; month:01 ; pages:4628-4642 |
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DOI / URN: |
10.1007/s10854-021-07652-1 |
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OLC2078139971 |
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520 | |a Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. | ||
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10.1007/s10854-021-07652-1 doi (DE-627)OLC2078139971 (DE-He213)s10854-021-07652-1-p DE-627 ger DE-627 rakwb eng 600 670 620 VZ Zhang, Junshan verfasserin aut Length effect of ceria nanorod on its oxygen vacancy formation and photocatalytic property 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. Xia, Xuewen aut Mao, Xisong aut Li, Junqi aut Chen, Chaoyi aut Liu, Fengyuan aut Lan, Yuan-Pei (orcid)0000-0002-3046-5330 aut Enthalten in Journal of materials science / Materials in electronics Springer US, 1990 33(2022), 7 vom: 12. Jan., Seite 4628-4642 (DE-627)130863289 (DE-600)1030929-9 (DE-576)023106719 0957-4522 nnns volume:33 year:2022 number:7 day:12 month:01 pages:4628-4642 https://doi.org/10.1007/s10854-021-07652-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_2004 GBV_ILN_2015 AR 33 2022 7 12 01 4628-4642 |
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10.1007/s10854-021-07652-1 doi (DE-627)OLC2078139971 (DE-He213)s10854-021-07652-1-p DE-627 ger DE-627 rakwb eng 600 670 620 VZ Zhang, Junshan verfasserin aut Length effect of ceria nanorod on its oxygen vacancy formation and photocatalytic property 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. Xia, Xuewen aut Mao, Xisong aut Li, Junqi aut Chen, Chaoyi aut Liu, Fengyuan aut Lan, Yuan-Pei (orcid)0000-0002-3046-5330 aut Enthalten in Journal of materials science / Materials in electronics Springer US, 1990 33(2022), 7 vom: 12. Jan., Seite 4628-4642 (DE-627)130863289 (DE-600)1030929-9 (DE-576)023106719 0957-4522 nnns volume:33 year:2022 number:7 day:12 month:01 pages:4628-4642 https://doi.org/10.1007/s10854-021-07652-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_2004 GBV_ILN_2015 AR 33 2022 7 12 01 4628-4642 |
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10.1007/s10854-021-07652-1 doi (DE-627)OLC2078139971 (DE-He213)s10854-021-07652-1-p DE-627 ger DE-627 rakwb eng 600 670 620 VZ Zhang, Junshan verfasserin aut Length effect of ceria nanorod on its oxygen vacancy formation and photocatalytic property 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. Xia, Xuewen aut Mao, Xisong aut Li, Junqi aut Chen, Chaoyi aut Liu, Fengyuan aut Lan, Yuan-Pei (orcid)0000-0002-3046-5330 aut Enthalten in Journal of materials science / Materials in electronics Springer US, 1990 33(2022), 7 vom: 12. Jan., Seite 4628-4642 (DE-627)130863289 (DE-600)1030929-9 (DE-576)023106719 0957-4522 nnns volume:33 year:2022 number:7 day:12 month:01 pages:4628-4642 https://doi.org/10.1007/s10854-021-07652-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_2004 GBV_ILN_2015 AR 33 2022 7 12 01 4628-4642 |
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10.1007/s10854-021-07652-1 doi (DE-627)OLC2078139971 (DE-He213)s10854-021-07652-1-p DE-627 ger DE-627 rakwb eng 600 670 620 VZ Zhang, Junshan verfasserin aut Length effect of ceria nanorod on its oxygen vacancy formation and photocatalytic property 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. Xia, Xuewen aut Mao, Xisong aut Li, Junqi aut Chen, Chaoyi aut Liu, Fengyuan aut Lan, Yuan-Pei (orcid)0000-0002-3046-5330 aut Enthalten in Journal of materials science / Materials in electronics Springer US, 1990 33(2022), 7 vom: 12. Jan., Seite 4628-4642 (DE-627)130863289 (DE-600)1030929-9 (DE-576)023106719 0957-4522 nnns volume:33 year:2022 number:7 day:12 month:01 pages:4628-4642 https://doi.org/10.1007/s10854-021-07652-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_2004 GBV_ILN_2015 AR 33 2022 7 12 01 4628-4642 |
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Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
abstractGer |
Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
abstract_unstemmed |
Abstract Ceria nanorods (NRs) with an average length of 23, 73, 115, 131, and 192 nm were synthesized separately by a facile hydrothermal method and then were roasted at 600 °C in air, 50% $ H_{2} $, and pure $ H_{2} $ to generate various concentrations of surface oxygen vacancies (OVs). OVs concentration in ceria lattice is firstly increasing and then trends to decrease with the rising of ceria NRs length, while the band gap of ceria NRs expands with length increasing and slightly widens with the elevation of surface OVs concentration. Separation efficiency of photo-excited electrons/holes (e−/h+) and photodegradation ratio of methylene blue (MB) with ceria NRs elevate firstly and then decrease with the length increasing, while the generated OVs promote the photocatalytic activity of ceria. The ceria NRs with an average length of 115 nm and calcined in hydrogen show a better photocatalytic activity with the MB degradation ratio of 86.32%. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
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title_short |
Length effect of ceria nanorod on its oxygen vacancy formation and photocatalytic property |
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https://doi.org/10.1007/s10854-021-07652-1 |
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Xia, Xuewen Mao, Xisong Li, Junqi Chen, Chaoyi Liu, Fengyuan Lan, Yuan-Pei |
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up_date |
2024-07-03T18:59:54.752Z |
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