Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China
Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in b...
Ausführliche Beschreibung
Autor*in: |
Liu, Wenhui [verfasserIn] |
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Sprache: |
Englisch |
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2022 |
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Anmerkung: |
© The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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Übergeordnetes Werk: |
Enthalten in: Environmental science and pollution research - Springer Berlin Heidelberg, 1994, 29(2022), 25 vom: 15. Jan., Seite 37115-37128 |
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Übergeordnetes Werk: |
volume:29 ; year:2022 ; number:25 ; day:15 ; month:01 ; pages:37115-37128 |
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DOI / URN: |
10.1007/s11356-021-18478-z |
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OLC207865244X |
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520 | |a Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. | ||
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10.1007/s11356-021-18478-z doi (DE-627)OLC207865244X (DE-He213)s11356-021-18478-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Liu, Wenhui verfasserin aut Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. Le’an River Dissolved organic matter Ecological risk Heavy metals Ma, Teng aut Du, Yao aut Wu, Xiancang aut Chen, Liuzhu aut Li, Junqi aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 25 vom: 15. Jan., Seite 37115-37128 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:25 day:15 month:01 pages:37115-37128 https://doi.org/10.1007/s11356-021-18478-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 25 15 01 37115-37128 |
spelling |
10.1007/s11356-021-18478-z doi (DE-627)OLC207865244X (DE-He213)s11356-021-18478-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Liu, Wenhui verfasserin aut Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. Le’an River Dissolved organic matter Ecological risk Heavy metals Ma, Teng aut Du, Yao aut Wu, Xiancang aut Chen, Liuzhu aut Li, Junqi aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 25 vom: 15. Jan., Seite 37115-37128 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:25 day:15 month:01 pages:37115-37128 https://doi.org/10.1007/s11356-021-18478-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 25 15 01 37115-37128 |
allfields_unstemmed |
10.1007/s11356-021-18478-z doi (DE-627)OLC207865244X (DE-He213)s11356-021-18478-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Liu, Wenhui verfasserin aut Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. Le’an River Dissolved organic matter Ecological risk Heavy metals Ma, Teng aut Du, Yao aut Wu, Xiancang aut Chen, Liuzhu aut Li, Junqi aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 25 vom: 15. Jan., Seite 37115-37128 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:25 day:15 month:01 pages:37115-37128 https://doi.org/10.1007/s11356-021-18478-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 25 15 01 37115-37128 |
allfieldsGer |
10.1007/s11356-021-18478-z doi (DE-627)OLC207865244X (DE-He213)s11356-021-18478-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Liu, Wenhui verfasserin aut Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. Le’an River Dissolved organic matter Ecological risk Heavy metals Ma, Teng aut Du, Yao aut Wu, Xiancang aut Chen, Liuzhu aut Li, Junqi aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 25 vom: 15. Jan., Seite 37115-37128 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:25 day:15 month:01 pages:37115-37128 https://doi.org/10.1007/s11356-021-18478-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 25 15 01 37115-37128 |
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10.1007/s11356-021-18478-z doi (DE-627)OLC207865244X (DE-He213)s11356-021-18478-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Liu, Wenhui verfasserin aut Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. Le’an River Dissolved organic matter Ecological risk Heavy metals Ma, Teng aut Du, Yao aut Wu, Xiancang aut Chen, Liuzhu aut Li, Junqi aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 25 vom: 15. Jan., Seite 37115-37128 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:25 day:15 month:01 pages:37115-37128 https://doi.org/10.1007/s11356-021-18478-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 25 15 01 37115-37128 |
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characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—le’an river, china |
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Characteristics of dissolved organic matter in surface water and sediment and its ecological indication in a typical mining-affected river—Le’an River, China |
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Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
abstract_unstemmed |
Abstract Dissolved organic matter (DOM) plays an important role in the cycling and toxicity of heavy metals in aquatic systems. However, most studies have focused only on DOM in either water or sediments. This study aimed to analyze the source, composition, and structural characteristics of DOM in both surface water and bottom sediments of the Le’an River and its major tributaries. In addition, the potential ecological risks of three typical heavy metals (Cu, Pb, and Zn) were quantitatively evaluated based on the characteristics of DOM and in situ data. The results showed that sediment DOM is more aromatic and hydrophobic than surface water DOM. Although humic-like components dominated the DOM pool in both surface water and sediments, their sources were different. Surface water DOM is mainly autochthonous, while sediment DOM is controlled by both autochthonous and allochthonous sources. Risk prediction results based on DOM characteristics show that surface water has a higher potential risk of heavy metal release than sediments. Comprehensively considering the ecological risk of water and sediments, high-risk areas were found to be mainly distributed in the upper and middle reaches of the Le’an River. This distribution is attributable to the developed mining and smelting industries in these areas and consistent with the risk assessment results of measured concentrations of heavy metals. This study established a new technique for predicting the ecological risk of aquatic systems based on the characteristics of DOM in surface water and sediments. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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