Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory
Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Result...
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| Autor*in: |
Qin, Guimei [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Environmental science and pollution research - Springer Berlin Heidelberg, 1994, 29(2022), 34 vom: 05. März, Seite 51635-51650 |
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| Übergeordnetes Werk: |
volume:29 ; year:2022 ; number:34 ; day:05 ; month:03 ; pages:51635-51650 |
| Links: |
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| DOI / URN: |
10.1007/s11356-022-19145-7 |
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| Katalog-ID: |
OLC2079169408 |
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| 520 | |a Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. | ||
| 650 | 4 | |a VOC characteristics | |
| 650 | 4 | |a Spatial distribution, Source apportionment | |
| 650 | 4 | |a Emission inventory | |
| 650 | 4 | |a Chemical conversions | |
| 700 | 1 | |a Gao, Song |4 aut | |
| 700 | 1 | |a Fu, Qingyan |4 aut | |
| 700 | 1 | |a Fu, Shuang |4 aut | |
| 700 | 1 | |a Jia, Haohao |4 aut | |
| 700 | 1 | |a Zeng, Qingrui |4 aut | |
| 700 | 1 | |a Fan, Linping |4 aut | |
| 700 | 1 | |a Ren, Huarui |4 aut | |
| 700 | 1 | |a Cheng, Jinping |4 aut | |
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10.1007/s11356-022-19145-7 doi (DE-627)OLC2079169408 (DE-He213)s11356-022-19145-7-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Qin, Guimei verfasserin aut Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. VOC characteristics Spatial distribution, Source apportionment Emission inventory Chemical conversions Gao, Song aut Fu, Qingyan aut Fu, Shuang aut Jia, Haohao aut Zeng, Qingrui aut Fan, Linping aut Ren, Huarui aut Cheng, Jinping aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 34 vom: 05. März, Seite 51635-51650 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:34 day:05 month:03 pages:51635-51650 https://doi.org/10.1007/s11356-022-19145-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 34 05 03 51635-51650 |
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10.1007/s11356-022-19145-7 doi (DE-627)OLC2079169408 (DE-He213)s11356-022-19145-7-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Qin, Guimei verfasserin aut Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. VOC characteristics Spatial distribution, Source apportionment Emission inventory Chemical conversions Gao, Song aut Fu, Qingyan aut Fu, Shuang aut Jia, Haohao aut Zeng, Qingrui aut Fan, Linping aut Ren, Huarui aut Cheng, Jinping aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 34 vom: 05. März, Seite 51635-51650 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:34 day:05 month:03 pages:51635-51650 https://doi.org/10.1007/s11356-022-19145-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 34 05 03 51635-51650 |
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10.1007/s11356-022-19145-7 doi (DE-627)OLC2079169408 (DE-He213)s11356-022-19145-7-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Qin, Guimei verfasserin aut Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. VOC characteristics Spatial distribution, Source apportionment Emission inventory Chemical conversions Gao, Song aut Fu, Qingyan aut Fu, Shuang aut Jia, Haohao aut Zeng, Qingrui aut Fan, Linping aut Ren, Huarui aut Cheng, Jinping aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 34 vom: 05. März, Seite 51635-51650 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:34 day:05 month:03 pages:51635-51650 https://doi.org/10.1007/s11356-022-19145-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 34 05 03 51635-51650 |
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10.1007/s11356-022-19145-7 doi (DE-627)OLC2079169408 (DE-He213)s11356-022-19145-7-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Qin, Guimei verfasserin aut Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. VOC characteristics Spatial distribution, Source apportionment Emission inventory Chemical conversions Gao, Song aut Fu, Qingyan aut Fu, Shuang aut Jia, Haohao aut Zeng, Qingrui aut Fan, Linping aut Ren, Huarui aut Cheng, Jinping aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 34 vom: 05. März, Seite 51635-51650 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:34 day:05 month:03 pages:51635-51650 https://doi.org/10.1007/s11356-022-19145-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 34 05 03 51635-51650 |
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10.1007/s11356-022-19145-7 doi (DE-627)OLC2079169408 (DE-He213)s11356-022-19145-7-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Qin, Guimei verfasserin aut Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. VOC characteristics Spatial distribution, Source apportionment Emission inventory Chemical conversions Gao, Song aut Fu, Qingyan aut Fu, Shuang aut Jia, Haohao aut Zeng, Qingrui aut Fan, Linping aut Ren, Huarui aut Cheng, Jinping aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 29(2022), 34 vom: 05. März, Seite 51635-51650 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:29 year:2022 number:34 day:05 month:03 pages:51635-51650 https://doi.org/10.1007/s11356-022-19145-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 29 2022 34 05 03 51635-51650 |
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The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. 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Investigation of VOC characteristics, source analysis, and chemical conversions in a typical petrochemical area through 1-year monitoring and emission inventory |
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Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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Abstract To effectively investigate the characteristics, source analysis, and chemical conversions of volatile organic compounds (VOCs) pollution in a typical petrochemical area, 81 VOC species from nine sampling sites were collected from 1st January to 31th December 2019 in Jinshan District. Results showed the concentration of VOCs was 51.63 ± 36.05 ppbv, and VOCs were dominated by alkane (40.10%) and alkenes (39.91%). The temporal variations of VOCs showed that the highest average VOC concentration appeared in July, and the lowest concentration of VOCs was in February. The concentration of VOCs was mainly connected with industrial processes and was transported to other areas through the downwind direction. Six PMF-derived sources including petrochemical industry, solvent utilization, vehicle exhaust, fuel evaporation, combustion, and other industry processes, contributing 37.08%, 16.74%, 16.69%, 14.99%, 9.53%, and 4.97%, respectively. Meanwhile, an anthropogenic VOC emission inventory was established by emission factors and the activity statistics for 2019, results indicated that the total emission of VOCs was estimated as 6.22 kt, petrochemical industry was the most important contributor of human-produced VOCs. The LOH concentration was 396.12 ppbv via OH radical loss rate method, and the OFP was 210.44 ppbv based on the MIR factor. Alkenes and aromatics were the important components of $ O_{3} $ formation. This study provides effective information for corresponding governments to establish VOCs contamination control directives. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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