Possibility of Reductive Deactivation of S-Triazines and Parent Compounds on Waters and Sediments
Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the env...
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| Autor*in: |
GalvÍn, R. Marín [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2005 |
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| Systematik: |
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| Anmerkung: |
© Springer Science + Business Media, Inc. 2005 |
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| Übergeordnetes Werk: |
Enthalten in: Water, air & soil pollution - Kluwer Academic Publishers, 1971, 165(2005), 1-4 vom: Juli, Seite 347-364 |
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| Übergeordnetes Werk: |
volume:165 ; year:2005 ; number:1-4 ; month:07 ; pages:347-364 |
| Links: |
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| DOI / URN: |
10.1007/s11270-005-6913-8 |
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OLC2084492459 |
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| 520 | |a Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. | ||
| 650 | 4 | |a deactivation | |
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| 650 | 4 | |a triazine herbicides | |
| 700 | 1 | |a Montoya, M. Ruiz |4 aut | |
| 700 | 1 | |a Higuera, M. J. |4 aut | |
| 700 | 1 | |a Pérez, R. |4 aut | |
| 700 | 1 | |a Mellado, J. M. Rodríguez |4 aut | |
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10.1007/s11270-005-6913-8 doi (DE-627)OLC2084492459 (DE-He213)s11270-005-6913-8-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk GalvÍn, R. Marín verfasserin aut Possibility of Reductive Deactivation of S-Triazines and Parent Compounds on Waters and Sediments 2005 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science + Business Media, Inc. 2005 Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. deactivation degradation electrochemical reduction triazine herbicides Montoya, M. Ruiz aut Higuera, M. J. aut Pérez, R. aut Mellado, J. M. Rodríguez aut Enthalten in Water, air & soil pollution Kluwer Academic Publishers, 1971 165(2005), 1-4 vom: Juli, Seite 347-364 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:165 year:2005 number:1-4 month:07 pages:347-364 https://doi.org/10.1007/s11270-005-6913-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_31 GBV_ILN_40 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4116 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 165 2005 1-4 07 347-364 |
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10.1007/s11270-005-6913-8 doi (DE-627)OLC2084492459 (DE-He213)s11270-005-6913-8-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk GalvÍn, R. Marín verfasserin aut Possibility of Reductive Deactivation of S-Triazines and Parent Compounds on Waters and Sediments 2005 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science + Business Media, Inc. 2005 Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. deactivation degradation electrochemical reduction triazine herbicides Montoya, M. Ruiz aut Higuera, M. J. aut Pérez, R. aut Mellado, J. M. Rodríguez aut Enthalten in Water, air & soil pollution Kluwer Academic Publishers, 1971 165(2005), 1-4 vom: Juli, Seite 347-364 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:165 year:2005 number:1-4 month:07 pages:347-364 https://doi.org/10.1007/s11270-005-6913-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_31 GBV_ILN_40 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4116 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 165 2005 1-4 07 347-364 |
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10.1007/s11270-005-6913-8 doi (DE-627)OLC2084492459 (DE-He213)s11270-005-6913-8-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk GalvÍn, R. Marín verfasserin aut Possibility of Reductive Deactivation of S-Triazines and Parent Compounds on Waters and Sediments 2005 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science + Business Media, Inc. 2005 Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. deactivation degradation electrochemical reduction triazine herbicides Montoya, M. Ruiz aut Higuera, M. J. aut Pérez, R. aut Mellado, J. M. Rodríguez aut Enthalten in Water, air & soil pollution Kluwer Academic Publishers, 1971 165(2005), 1-4 vom: Juli, Seite 347-364 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:165 year:2005 number:1-4 month:07 pages:347-364 https://doi.org/10.1007/s11270-005-6913-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_31 GBV_ILN_40 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4116 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 165 2005 1-4 07 347-364 |
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10.1007/s11270-005-6913-8 doi (DE-627)OLC2084492459 (DE-He213)s11270-005-6913-8-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk GalvÍn, R. Marín verfasserin aut Possibility of Reductive Deactivation of S-Triazines and Parent Compounds on Waters and Sediments 2005 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science + Business Media, Inc. 2005 Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. deactivation degradation electrochemical reduction triazine herbicides Montoya, M. Ruiz aut Higuera, M. J. aut Pérez, R. aut Mellado, J. M. Rodríguez aut Enthalten in Water, air & soil pollution Kluwer Academic Publishers, 1971 165(2005), 1-4 vom: Juli, Seite 347-364 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:165 year:2005 number:1-4 month:07 pages:347-364 https://doi.org/10.1007/s11270-005-6913-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_31 GBV_ILN_40 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4116 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 165 2005 1-4 07 347-364 |
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possibility of reductive deactivation of s-triazines and parent compounds on waters and sediments |
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Possibility of Reductive Deactivation of S-Triazines and Parent Compounds on Waters and Sediments |
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Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. © Springer Science + Business Media, Inc. 2005 |
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Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. © Springer Science + Business Media, Inc. 2005 |
| abstract_unstemmed |
Abstract Electrochemistry can be a valuable instrument to preserve the aquatic environment, first, by elucidating the oxidation-reduction mechanisms of substances having toxicological potential at laboratory scale; second, by aiding through extrapolation to comprise the evolution and fate in the environment of these pollutants and, finally, by establishing the basis of some electrochemical deactivation processes at industrial scale. In this way, this paper deals on studies of a type of highly pollutant substances for the aquatic media such as the S-triazines. The first part of the paper is focused to show the electrochemical reduction behavior of some S-triazines (eleven compounds have been studied). Later, the probable consequences at natural scale of these electroreductive processes are evaluated. Thus, the electrochemical reduction of diluted solutions of s-triazine herbicides and parent compounds takes place at potentials of −0.90 to −1.20 V, at very acidic pH values. The electroreduction products generated in all cases have loss the aromaticity and, depending on the compound, the chlorine atom or the –$ SCH_{3} $ group. So, the resulting molecules present lower toxicity than the original compounds. For this reason, the electroreductive way can be an efficient option for the detoxification of S-triazine polluted waters. On the other hand, the natural deactivation of the s-triazines present in natural waters, in addition to the conventional photooxidative route taking place in well illuminated and oxygenated waters, could take place through the reductive process when the waters are essentially anoxic, acidic, and rich in suspended materials. This natural reduction, moreover, could favour the later oxidation or metabolization of the byproducts emanating of the original plaguicides. Finally, the reduction of S-triazines, both forced (industrial water depuration via electrochemical reduction) and no forced (natural aquatic media) requires more negative redox potentials, that is, more reductive environments as the molecules become more complex. © Springer Science + Business Media, Inc. 2005 |
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