Identification, Apportionment, and Photochemical Reactivity of Non-methane Hydrocarbon Sources in Busan, Korea
Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gij...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Choi, Eunhwa [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2010 |
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| Schlagwörter: |
Conditional probability function (CPF) Positive matrix factorization (PMF) |
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| Systematik: |
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| Anmerkung: |
© Springer Science+Business Media B.V. 2010 |
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| Übergeordnetes Werk: |
Enthalten in: Water, air & soil pollution - Springer Netherlands, 1971, 215(2010), 1-4 vom: 29. Juni, Seite 67-82 |
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| Übergeordnetes Werk: |
volume:215 ; year:2010 ; number:1-4 ; day:29 ; month:06 ; pages:67-82 |
| Links: |
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| DOI / URN: |
10.1007/s11270-010-0459-0 |
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OLC2084522145 |
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| 520 | |a Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. | ||
| 650 | 4 | |a Conditional probability function (CPF) | |
| 650 | 4 | |a Ozone formation | |
| 650 | 4 | |a Positive matrix factorization (PMF) | |
| 650 | 4 | |a Potential source contribution function (PSCF) | |
| 650 | 4 | |a Non-methane hydrocarbon (NMHC) | |
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| 700 | 1 | |a Jin, Byong-Bok |4 aut | |
| 700 | 1 | |a Yi, Seung-Muk |4 aut | |
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10.1007/s11270-010-0459-0 doi (DE-627)OLC2084522145 (DE-He213)s11270-010-0459-0-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk Choi, Eunhwa verfasserin aut Identification, Apportionment, and Photochemical Reactivity of Non-methane Hydrocarbon Sources in Busan, Korea 2010 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media B.V. 2010 Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. Conditional probability function (CPF) Ozone formation Positive matrix factorization (PMF) Potential source contribution function (PSCF) Non-methane hydrocarbon (NMHC) Heo, Jong-Bae aut Hopke, Philip K. aut Jin, Byong-Bok aut Yi, Seung-Muk aut Enthalten in Water, air & soil pollution Springer Netherlands, 1971 215(2010), 1-4 vom: 29. Juni, Seite 67-82 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:215 year:2010 number:1-4 day:29 month:06 pages:67-82 https://doi.org/10.1007/s11270-010-0459-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 215 2010 1-4 29 06 67-82 |
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10.1007/s11270-010-0459-0 doi (DE-627)OLC2084522145 (DE-He213)s11270-010-0459-0-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk Choi, Eunhwa verfasserin aut Identification, Apportionment, and Photochemical Reactivity of Non-methane Hydrocarbon Sources in Busan, Korea 2010 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media B.V. 2010 Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. Conditional probability function (CPF) Ozone formation Positive matrix factorization (PMF) Potential source contribution function (PSCF) Non-methane hydrocarbon (NMHC) Heo, Jong-Bae aut Hopke, Philip K. aut Jin, Byong-Bok aut Yi, Seung-Muk aut Enthalten in Water, air & soil pollution Springer Netherlands, 1971 215(2010), 1-4 vom: 29. Juni, Seite 67-82 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:215 year:2010 number:1-4 day:29 month:06 pages:67-82 https://doi.org/10.1007/s11270-010-0459-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 215 2010 1-4 29 06 67-82 |
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10.1007/s11270-010-0459-0 doi (DE-627)OLC2084522145 (DE-He213)s11270-010-0459-0-p DE-627 ger DE-627 rakwb eng 570 333.7 VZ 12 13 ssgn BIODIV DE-30 fid ZC 7520 VZ rvk ZC 7520 VZ rvk Choi, Eunhwa verfasserin aut Identification, Apportionment, and Photochemical Reactivity of Non-methane Hydrocarbon Sources in Busan, Korea 2010 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media B.V. 2010 Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. Conditional probability function (CPF) Ozone formation Positive matrix factorization (PMF) Potential source contribution function (PSCF) Non-methane hydrocarbon (NMHC) Heo, Jong-Bae aut Hopke, Philip K. aut Jin, Byong-Bok aut Yi, Seung-Muk aut Enthalten in Water, air & soil pollution Springer Netherlands, 1971 215(2010), 1-4 vom: 29. Juni, Seite 67-82 (DE-627)12929134X (DE-600)120499-3 (DE-576)014472643 0049-6979 nnns volume:215 year:2010 number:1-4 day:29 month:06 pages:67-82 https://doi.org/10.1007/s11270-010-0459-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-FOR SSG-OLC-IBL SSG-OPC-GGO GBV_ILN_22 GBV_ILN_70 GBV_ILN_2006 GBV_ILN_2027 GBV_ILN_4012 GBV_ILN_4082 GBV_ILN_4219 GBV_ILN_4309 GBV_ILN_4313 ZC 7520 ZC 7520 AR 215 2010 1-4 29 06 67-82 |
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identification, apportionment, and photochemical reactivity of non-methane hydrocarbon sources in busan, korea |
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Identification, Apportionment, and Photochemical Reactivity of Non-methane Hydrocarbon Sources in Busan, Korea |
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Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. © Springer Science+Business Media B.V. 2010 |
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Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. © Springer Science+Business Media B.V. 2010 |
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Abstract Hourly concentrations of non-methane hydrocarbons (NMHCs) recorded between June and August 2006, at two monitoring sites (Gijang and Jin) in Busan were analyzed to examine the characteristics and photochemical reactivity of NMHC sources. The two sites represent urban (Jin) and suburban (Gijang) Busan, which is a typical Korean city. Positive matrix factorization (PMF), applied to identify and apportion the sources of NMHCs, revealed nine sources for Gijang and ten sources for Jin. To explore the contribution of each NMHC source to ozone formation at the two sampling sites, the ozone formation potential was estimated for each source. The largest contributors to ozone formation were sources characterized by 1,2,3-trimethylbenzene (26.4%) at Gijang and by toluene, ethylbenzene, and xylenes (22.5%) at Jin, which were composed mostly of heavy hydrocarbons and aromatics. Secondary sources included two coating sources (20.9%, 12.2%) and vehicle exhaust (10.3%) at Gijang and a source represented by toluene (17.4%), vehicle exhaust (15.9%), and a coating-2 source (9.6%) at Jin. Conditional probability function (CPF) and potential source contribution function (PSCF) analysis methods were used to identify the directions of local sources and to locate potential source regions, respectively. The CPF and PSCF results agreed well for the majority of sources resolved by PMF and thus were very useful in identifying the major sources contributing to ozone formation at the two study sites. © Springer Science+Business Media B.V. 2010 |
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