Time-resolved photo-phonon spectroscopy of exchange coupled $ Cr^{3+} $ pairs in ruby
Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiativ...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Shegeda, A. M. [verfasserIn] |
|---|
| Format: |
Artikel |
|---|---|
| Sprache: |
Englisch |
| Erschienen: |
2003 |
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| Anmerkung: |
© MAIK "Nauka/Interperiodica" 2003 |
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| Übergeordnetes Werk: |
Enthalten in: Journal of experimental and theoretical physics / JETP letters - Nauka/Interperiodica, 1993, 78(2003), 11 vom: Dez., Seite 730-733 |
|---|---|
| Übergeordnetes Werk: |
volume:78 ; year:2003 ; number:11 ; month:12 ; pages:730-733 |
| Links: |
|---|
| DOI / URN: |
10.1134/1.1648297 |
|---|
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OLC2085751601 |
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| 520 | |a Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. | ||
| 700 | 1 | |a Lisin, V. N. |4 aut | |
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10.1134/1.1648297 doi (DE-627)OLC2085751601 (DE-He213)1.1648297-p DE-627 ger DE-627 rakwb eng 530 VZ 33.00 bkl Shegeda, A. M. verfasserin aut Time-resolved photo-phonon spectroscopy of exchange coupled $ Cr^{3+} $ pairs in ruby 2003 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © MAIK "Nauka/Interperiodica" 2003 Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. Lisin, V. N. aut Enthalten in Journal of experimental and theoretical physics / JETP letters Nauka/Interperiodica, 1993 78(2003), 11 vom: Dez., Seite 730-733 (DE-627)182384713 (DE-600)917787-5 (DE-576)053745841 0021-3640 nnns volume:78 year:2003 number:11 month:12 pages:730-733 https://doi.org/10.1134/1.1648297 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY 33.00 VZ AR 78 2003 11 12 730-733 |
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10.1134/1.1648297 doi (DE-627)OLC2085751601 (DE-He213)1.1648297-p DE-627 ger DE-627 rakwb eng 530 VZ 33.00 bkl Shegeda, A. M. verfasserin aut Time-resolved photo-phonon spectroscopy of exchange coupled $ Cr^{3+} $ pairs in ruby 2003 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © MAIK "Nauka/Interperiodica" 2003 Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. Lisin, V. N. aut Enthalten in Journal of experimental and theoretical physics / JETP letters Nauka/Interperiodica, 1993 78(2003), 11 vom: Dez., Seite 730-733 (DE-627)182384713 (DE-600)917787-5 (DE-576)053745841 0021-3640 nnns volume:78 year:2003 number:11 month:12 pages:730-733 https://doi.org/10.1134/1.1648297 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY 33.00 VZ AR 78 2003 11 12 730-733 |
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10.1134/1.1648297 doi (DE-627)OLC2085751601 (DE-He213)1.1648297-p DE-627 ger DE-627 rakwb eng 530 VZ 33.00 bkl Shegeda, A. M. verfasserin aut Time-resolved photo-phonon spectroscopy of exchange coupled $ Cr^{3+} $ pairs in ruby 2003 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © MAIK "Nauka/Interperiodica" 2003 Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. Lisin, V. N. aut Enthalten in Journal of experimental and theoretical physics / JETP letters Nauka/Interperiodica, 1993 78(2003), 11 vom: Dez., Seite 730-733 (DE-627)182384713 (DE-600)917787-5 (DE-576)053745841 0021-3640 nnns volume:78 year:2003 number:11 month:12 pages:730-733 https://doi.org/10.1134/1.1648297 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY 33.00 VZ AR 78 2003 11 12 730-733 |
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10.1134/1.1648297 doi (DE-627)OLC2085751601 (DE-He213)1.1648297-p DE-627 ger DE-627 rakwb eng 530 VZ 33.00 bkl Shegeda, A. M. verfasserin aut Time-resolved photo-phonon spectroscopy of exchange coupled $ Cr^{3+} $ pairs in ruby 2003 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © MAIK "Nauka/Interperiodica" 2003 Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. Lisin, V. N. aut Enthalten in Journal of experimental and theoretical physics / JETP letters Nauka/Interperiodica, 1993 78(2003), 11 vom: Dez., Seite 730-733 (DE-627)182384713 (DE-600)917787-5 (DE-576)053745841 0021-3640 nnns volume:78 year:2003 number:11 month:12 pages:730-733 https://doi.org/10.1134/1.1648297 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY 33.00 VZ AR 78 2003 11 12 730-733 |
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10.1134/1.1648297 doi (DE-627)OLC2085751601 (DE-He213)1.1648297-p DE-627 ger DE-627 rakwb eng 530 VZ 33.00 bkl Shegeda, A. M. verfasserin aut Time-resolved photo-phonon spectroscopy of exchange coupled $ Cr^{3+} $ pairs in ruby 2003 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © MAIK "Nauka/Interperiodica" 2003 Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. Lisin, V. N. aut Enthalten in Journal of experimental and theoretical physics / JETP letters Nauka/Interperiodica, 1993 78(2003), 11 vom: Dez., Seite 730-733 (DE-627)182384713 (DE-600)917787-5 (DE-576)053745841 0021-3640 nnns volume:78 year:2003 number:11 month:12 pages:730-733 https://doi.org/10.1134/1.1648297 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY 33.00 VZ AR 78 2003 11 12 730-733 |
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Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. © MAIK "Nauka/Interperiodica" 2003 |
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Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. © MAIK "Nauka/Interperiodica" 2003 |
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Abstract A rather simple method is used to simultaneously detect both optical absorption spectra and excited-state nonradiative transitions in 0.03 and 0.16 at. % ruby at temperature 2 K. The technique utilizes a time-resolved bolometer detection of phonons generated by the excited-state nonradiative relaxation following optical excitation with a pulsed tunable dye laser. The observed excitation spectra of phonons coincide well with currently known absorption spectra of both chromium single ions and pairs of the nearest neighbors. For the first time, the fast (≤ µs) resonant energy transfer from single chromium ions to the fourth nearest neighbors is observed directly. New strongly perturbed Cr-single-ion sites are observed. © MAIK "Nauka/Interperiodica" 2003 |
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