Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water
Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The re...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhao, Shiyin [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020 |
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| Schlagwörter: |
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| Anmerkung: |
© Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
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| Übergeordnetes Werk: |
Enthalten in: Environmental science and pollution research - Springer Berlin Heidelberg, 1994, 27(2020), 31 vom: 08. Juli, Seite 39186-39197 |
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| Übergeordnetes Werk: |
volume:27 ; year:2020 ; number:31 ; day:08 ; month:07 ; pages:39186-39197 |
| Links: |
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| DOI / URN: |
10.1007/s11356-020-09865-z |
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OLC2119719861 |
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| 520 | |a Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. | ||
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10.1007/s11356-020-09865-z doi (DE-627)OLC2119719861 (DE-He213)s11356-020-09865-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Zhao, Shiyin verfasserin aut Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water 2020 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. Two-dimensional MOFs Microwave synthesis Antibiotics Adsorption Photocatalysis Li, Shun (orcid)0000-0003-1102-5572 aut Zhao, Zhicheng aut Su, Yiping aut Long, Yangke aut Zheng, Zuquan aut Cui, Daling aut Liu, Yong aut Wang, Chunfei aut Zhang, Xuanjun aut Zhang, Zuotai aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 27(2020), 31 vom: 08. Juli, Seite 39186-39197 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:27 year:2020 number:31 day:08 month:07 pages:39186-39197 https://doi.org/10.1007/s11356-020-09865-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 27 2020 31 08 07 39186-39197 |
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10.1007/s11356-020-09865-z doi (DE-627)OLC2119719861 (DE-He213)s11356-020-09865-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Zhao, Shiyin verfasserin aut Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water 2020 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. Two-dimensional MOFs Microwave synthesis Antibiotics Adsorption Photocatalysis Li, Shun (orcid)0000-0003-1102-5572 aut Zhao, Zhicheng aut Su, Yiping aut Long, Yangke aut Zheng, Zuquan aut Cui, Daling aut Liu, Yong aut Wang, Chunfei aut Zhang, Xuanjun aut Zhang, Zuotai aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 27(2020), 31 vom: 08. Juli, Seite 39186-39197 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:27 year:2020 number:31 day:08 month:07 pages:39186-39197 https://doi.org/10.1007/s11356-020-09865-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 27 2020 31 08 07 39186-39197 |
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10.1007/s11356-020-09865-z doi (DE-627)OLC2119719861 (DE-He213)s11356-020-09865-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Zhao, Shiyin verfasserin aut Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water 2020 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. Two-dimensional MOFs Microwave synthesis Antibiotics Adsorption Photocatalysis Li, Shun (orcid)0000-0003-1102-5572 aut Zhao, Zhicheng aut Su, Yiping aut Long, Yangke aut Zheng, Zuquan aut Cui, Daling aut Liu, Yong aut Wang, Chunfei aut Zhang, Xuanjun aut Zhang, Zuotai aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 27(2020), 31 vom: 08. Juli, Seite 39186-39197 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:27 year:2020 number:31 day:08 month:07 pages:39186-39197 https://doi.org/10.1007/s11356-020-09865-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 27 2020 31 08 07 39186-39197 |
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10.1007/s11356-020-09865-z doi (DE-627)OLC2119719861 (DE-He213)s11356-020-09865-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Zhao, Shiyin verfasserin aut Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water 2020 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. Two-dimensional MOFs Microwave synthesis Antibiotics Adsorption Photocatalysis Li, Shun (orcid)0000-0003-1102-5572 aut Zhao, Zhicheng aut Su, Yiping aut Long, Yangke aut Zheng, Zuquan aut Cui, Daling aut Liu, Yong aut Wang, Chunfei aut Zhang, Xuanjun aut Zhang, Zuotai aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 27(2020), 31 vom: 08. Juli, Seite 39186-39197 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:27 year:2020 number:31 day:08 month:07 pages:39186-39197 https://doi.org/10.1007/s11356-020-09865-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 27 2020 31 08 07 39186-39197 |
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10.1007/s11356-020-09865-z doi (DE-627)OLC2119719861 (DE-He213)s11356-020-09865-z-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Zhao, Shiyin verfasserin aut Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water 2020 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. Two-dimensional MOFs Microwave synthesis Antibiotics Adsorption Photocatalysis Li, Shun (orcid)0000-0003-1102-5572 aut Zhao, Zhicheng aut Su, Yiping aut Long, Yangke aut Zheng, Zuquan aut Cui, Daling aut Liu, Yong aut Wang, Chunfei aut Zhang, Xuanjun aut Zhang, Zuotai aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 27(2020), 31 vom: 08. Juli, Seite 39186-39197 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:27 year:2020 number:31 day:08 month:07 pages:39186-39197 https://doi.org/10.1007/s11356-020-09865-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR GBV_ILN_252 GBV_ILN_267 GBV_ILN_2018 GBV_ILN_4277 AR 27 2020 31 08 07 39186-39197 |
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Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water |
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Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. © Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
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Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. © Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
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Abstract Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 $ m^{2} $/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater. © Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
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