Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups
The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dime...
Ausführliche Beschreibung
Autor*in: |
Li, Niang-Xiu [verfasserIn] |
---|
Format: |
Artikel |
---|---|
Sprache: |
Englisch |
Erschienen: |
2022 |
---|
Schlagwörter: |
---|
Systematik: |
|
---|
Anmerkung: |
© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
---|
Übergeordnetes Werk: |
Enthalten in: Catalysis letters - Springer US, 1988, 153(2022), 10 vom: 23. Nov., Seite 2910-2916 |
---|---|
Übergeordnetes Werk: |
volume:153 ; year:2022 ; number:10 ; day:23 ; month:11 ; pages:2910-2916 |
Links: |
---|
DOI / URN: |
10.1007/s10562-022-04226-6 |
---|
Katalog-ID: |
OLC2145549137 |
---|
LEADER | 01000naa a22002652 4500 | ||
---|---|---|---|
001 | OLC2145549137 | ||
003 | DE-627 | ||
005 | 20240118105304.0 | ||
007 | tu | ||
008 | 240118s2022 xx ||||| 00| ||eng c | ||
024 | 7 | |a 10.1007/s10562-022-04226-6 |2 doi | |
035 | |a (DE-627)OLC2145549137 | ||
035 | |a (DE-He213)s10562-022-04226-6-p | ||
040 | |a DE-627 |b ger |c DE-627 |e rakwb | ||
041 | |a eng | ||
082 | 0 | 4 | |a 540 |a 660 |q VZ |
084 | |a VA 2890 |q VZ |2 rvk | ||
100 | 1 | |a Li, Niang-Xiu |e verfasserin |4 aut | |
245 | 1 | 0 | |a Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups |
264 | 1 | |c 2022 | |
336 | |a Text |b txt |2 rdacontent | ||
337 | |a ohne Hilfsmittel zu benutzen |b n |2 rdamedia | ||
338 | |a Band |b nc |2 rdacarrier | ||
500 | |a © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. | ||
520 | |a The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. | ||
650 | 4 | |a Photocatalytic Reduction CO | |
650 | 4 | |a CO | |
650 | 4 | |a Mn-based Complexes | |
700 | 1 | |a Chen, Yu-Mei |4 aut | |
700 | 1 | |a Xu, Quan-Qing |0 (orcid)0000-0001-5377-901X |4 aut | |
700 | 1 | |a Yang, Zhi |4 aut | |
773 | 0 | 8 | |i Enthalten in |t Catalysis letters |d Springer US, 1988 |g 153(2022), 10 vom: 23. Nov., Seite 2910-2916 |w (DE-627)130436550 |w (DE-600)644234-1 |w (DE-576)025720724 |x 1011-372X |7 nnns |
773 | 1 | 8 | |g volume:153 |g year:2022 |g number:10 |g day:23 |g month:11 |g pages:2910-2916 |
856 | 4 | 1 | |u https://doi.org/10.1007/s10562-022-04226-6 |z lizenzpflichtig |3 Volltext |
912 | |a GBV_USEFLAG_A | ||
912 | |a SYSFLAG_A | ||
912 | |a GBV_OLC | ||
912 | |a SSG-OLC-TEC | ||
912 | |a SSG-OLC-CHE | ||
936 | r | v | |a VA 2890 |
951 | |a AR | ||
952 | |d 153 |j 2022 |e 10 |b 23 |c 11 |h 2910-2916 |
author_variant |
n x l nxl y m c ymc q q x qqx z y zy |
---|---|
matchkey_str |
article:1011372X:2022----::htctltceutooc_tcuigagnscmlxsihiyiieoi |
hierarchy_sort_str |
2022 |
publishDate |
2022 |
allfields |
10.1007/s10562-022-04226-6 doi (DE-627)OLC2145549137 (DE-He213)s10562-022-04226-6-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Niang-Xiu verfasserin aut Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. Photocatalytic Reduction CO CO Mn-based Complexes Chen, Yu-Mei aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Yang, Zhi aut Enthalten in Catalysis letters Springer US, 1988 153(2022), 10 vom: 23. Nov., Seite 2910-2916 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 https://doi.org/10.1007/s10562-022-04226-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE VA 2890 AR 153 2022 10 23 11 2910-2916 |
spelling |
10.1007/s10562-022-04226-6 doi (DE-627)OLC2145549137 (DE-He213)s10562-022-04226-6-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Niang-Xiu verfasserin aut Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. Photocatalytic Reduction CO CO Mn-based Complexes Chen, Yu-Mei aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Yang, Zhi aut Enthalten in Catalysis letters Springer US, 1988 153(2022), 10 vom: 23. Nov., Seite 2910-2916 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 https://doi.org/10.1007/s10562-022-04226-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE VA 2890 AR 153 2022 10 23 11 2910-2916 |
allfields_unstemmed |
10.1007/s10562-022-04226-6 doi (DE-627)OLC2145549137 (DE-He213)s10562-022-04226-6-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Niang-Xiu verfasserin aut Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. Photocatalytic Reduction CO CO Mn-based Complexes Chen, Yu-Mei aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Yang, Zhi aut Enthalten in Catalysis letters Springer US, 1988 153(2022), 10 vom: 23. Nov., Seite 2910-2916 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 https://doi.org/10.1007/s10562-022-04226-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE VA 2890 AR 153 2022 10 23 11 2910-2916 |
allfieldsGer |
10.1007/s10562-022-04226-6 doi (DE-627)OLC2145549137 (DE-He213)s10562-022-04226-6-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Niang-Xiu verfasserin aut Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. Photocatalytic Reduction CO CO Mn-based Complexes Chen, Yu-Mei aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Yang, Zhi aut Enthalten in Catalysis letters Springer US, 1988 153(2022), 10 vom: 23. Nov., Seite 2910-2916 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 https://doi.org/10.1007/s10562-022-04226-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE VA 2890 AR 153 2022 10 23 11 2910-2916 |
allfieldsSound |
10.1007/s10562-022-04226-6 doi (DE-627)OLC2145549137 (DE-He213)s10562-022-04226-6-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Niang-Xiu verfasserin aut Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups 2022 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. Photocatalytic Reduction CO CO Mn-based Complexes Chen, Yu-Mei aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Yang, Zhi aut Enthalten in Catalysis letters Springer US, 1988 153(2022), 10 vom: 23. Nov., Seite 2910-2916 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 https://doi.org/10.1007/s10562-022-04226-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE VA 2890 AR 153 2022 10 23 11 2910-2916 |
language |
English |
source |
Enthalten in Catalysis letters 153(2022), 10 vom: 23. Nov., Seite 2910-2916 volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 |
sourceStr |
Enthalten in Catalysis letters 153(2022), 10 vom: 23. Nov., Seite 2910-2916 volume:153 year:2022 number:10 day:23 month:11 pages:2910-2916 |
format_phy_str_mv |
Article |
institution |
findex.gbv.de |
topic_facet |
Photocatalytic Reduction CO CO Mn-based Complexes |
dewey-raw |
540 |
isfreeaccess_bool |
false |
container_title |
Catalysis letters |
authorswithroles_txt_mv |
Li, Niang-Xiu @@aut@@ Chen, Yu-Mei @@aut@@ Xu, Quan-Qing @@aut@@ Yang, Zhi @@aut@@ |
publishDateDaySort_date |
2022-11-23T00:00:00Z |
hierarchy_top_id |
130436550 |
dewey-sort |
3540 |
id |
OLC2145549137 |
language_de |
englisch |
fullrecord |
<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">OLC2145549137</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20240118105304.0</controlfield><controlfield tag="007">tu</controlfield><controlfield tag="008">240118s2022 xx ||||| 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s10562-022-04226-6</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)OLC2145549137</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-He213)s10562-022-04226-6-p</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">540</subfield><subfield code="a">660</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">VA 2890</subfield><subfield code="q">VZ</subfield><subfield code="2">rvk</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Li, Niang-Xiu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2022</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">ohne Hilfsmittel zu benutzen</subfield><subfield code="b">n</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Band</subfield><subfield code="b">nc</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Photocatalytic Reduction CO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">CO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Mn-based Complexes</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Chen, Yu-Mei</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Xu, Quan-Qing</subfield><subfield code="0">(orcid)0000-0001-5377-901X</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Yang, Zhi</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Catalysis letters</subfield><subfield code="d">Springer US, 1988</subfield><subfield code="g">153(2022), 10 vom: 23. Nov., Seite 2910-2916</subfield><subfield code="w">(DE-627)130436550</subfield><subfield code="w">(DE-600)644234-1</subfield><subfield code="w">(DE-576)025720724</subfield><subfield code="x">1011-372X</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:153</subfield><subfield code="g">year:2022</subfield><subfield code="g">number:10</subfield><subfield code="g">day:23</subfield><subfield code="g">month:11</subfield><subfield code="g">pages:2910-2916</subfield></datafield><datafield tag="856" ind1="4" ind2="1"><subfield code="u">https://doi.org/10.1007/s10562-022-04226-6</subfield><subfield code="z">lizenzpflichtig</subfield><subfield code="3">Volltext</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_OLC</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-TEC</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-CHE</subfield></datafield><datafield tag="936" ind1="r" ind2="v"><subfield code="a">VA 2890</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">153</subfield><subfield code="j">2022</subfield><subfield code="e">10</subfield><subfield code="b">23</subfield><subfield code="c">11</subfield><subfield code="h">2910-2916</subfield></datafield></record></collection>
|
author |
Li, Niang-Xiu |
spellingShingle |
Li, Niang-Xiu ddc 540 rvk VA 2890 misc Photocatalytic Reduction CO misc CO misc Mn-based Complexes Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups |
authorStr |
Li, Niang-Xiu |
ppnlink_with_tag_str_mv |
@@773@@(DE-627)130436550 |
format |
Article |
dewey-ones |
540 - Chemistry & allied sciences 660 - Chemical engineering |
delete_txt_mv |
keep |
author_role |
aut aut aut aut |
collection |
OLC |
remote_str |
false |
illustrated |
Not Illustrated |
issn |
1011-372X |
topic_title |
540 660 VZ VA 2890 VZ rvk Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups Photocatalytic Reduction CO CO Mn-based Complexes |
topic |
ddc 540 rvk VA 2890 misc Photocatalytic Reduction CO misc CO misc Mn-based Complexes |
topic_unstemmed |
ddc 540 rvk VA 2890 misc Photocatalytic Reduction CO misc CO misc Mn-based Complexes |
topic_browse |
ddc 540 rvk VA 2890 misc Photocatalytic Reduction CO misc CO misc Mn-based Complexes |
format_facet |
Aufsätze Gedruckte Aufsätze |
format_main_str_mv |
Text Zeitschrift/Artikel |
carriertype_str_mv |
nc |
hierarchy_parent_title |
Catalysis letters |
hierarchy_parent_id |
130436550 |
dewey-tens |
540 - Chemistry 660 - Chemical engineering |
hierarchy_top_title |
Catalysis letters |
isfreeaccess_txt |
false |
familylinks_str_mv |
(DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 |
title |
Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups |
ctrlnum |
(DE-627)OLC2145549137 (DE-He213)s10562-022-04226-6-p |
title_full |
Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups |
author_sort |
Li, Niang-Xiu |
journal |
Catalysis letters |
journalStr |
Catalysis letters |
lang_code |
eng |
isOA_bool |
false |
dewey-hundreds |
500 - Science 600 - Technology |
recordtype |
marc |
publishDateSort |
2022 |
contenttype_str_mv |
txt |
container_start_page |
2910 |
author_browse |
Li, Niang-Xiu Chen, Yu-Mei Xu, Quan-Qing Yang, Zhi |
container_volume |
153 |
class |
540 660 VZ VA 2890 VZ rvk |
format_se |
Aufsätze |
author-letter |
Li, Niang-Xiu |
doi_str_mv |
10.1007/s10562-022-04226-6 |
normlink |
(ORCID)0000-0001-5377-901X |
normlink_prefix_str_mv |
(orcid)0000-0001-5377-901X |
dewey-full |
540 660 |
title_sort |
photocatalytic reduction of $ co_{2} $ to co using manganese complexes with bipyridine modified electron-donating groups |
title_auth |
Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups |
abstract |
The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
abstractGer |
The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
abstract_unstemmed |
The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
collection_details |
GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE |
container_issue |
10 |
title_short |
Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups |
url |
https://doi.org/10.1007/s10562-022-04226-6 |
remote_bool |
false |
author2 |
Chen, Yu-Mei Xu, Quan-Qing Yang, Zhi |
author2Str |
Chen, Yu-Mei Xu, Quan-Qing Yang, Zhi |
ppnlink |
130436550 |
mediatype_str_mv |
n |
isOA_txt |
false |
hochschulschrift_bool |
false |
doi_str |
10.1007/s10562-022-04226-6 |
up_date |
2024-07-04T03:33:16.013Z |
_version_ |
1803617824691716096 |
fullrecord_marcxml |
<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">OLC2145549137</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20240118105304.0</controlfield><controlfield tag="007">tu</controlfield><controlfield tag="008">240118s2022 xx ||||| 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s10562-022-04226-6</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)OLC2145549137</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-He213)s10562-022-04226-6-p</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">540</subfield><subfield code="a">660</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">VA 2890</subfield><subfield code="q">VZ</subfield><subfield code="2">rvk</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Li, Niang-Xiu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Photocatalytic Reduction of $ CO_{2} $ to CO Using Manganese Complexes with Bipyridine Modified Electron-Donating Groups</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2022</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">ohne Hilfsmittel zu benutzen</subfield><subfield code="b">n</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Band</subfield><subfield code="b">nc</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">The present work deals with the Mn-based complex formed after substitution with groups (–$ NH_{2} $ and –Br) on 2, 2′-bipyridine ligand and their photocatalytic activity for $ CO_{2} $ reduction. The photocatalytic system involves [Ru(bpy)3]2+ [Ru] as a photosensitizer (PS) in a mixture of N, N-dimethylformamide (DMF) and triethanolamine (TEOA) and the 1-benzyl-1,4-dihydronicotinamide (BIH), BIH and TEOA as the sacrificial agent and the auxiliary sacrificial agent in photocatalytic system, respectively. The results revealed that electron-donating groups of the complexes play an essential role in the photocatalytic reaction. Both density functional and high-resolution mass spectrometry supported the process of photocatalytic reduction of $ CO_{2} $ to CO in the presence of manganese complexes. Graphical Abstract Mn-based complex with 4,4′-diamine—2,2′-bipyridine as a ligand was synthesized. The photocatalytic $ CO_{2} $ reduction behaviours of the catalysts were investigated. The plausible mechanisms were proposed based on the main intermediates detected by HRMS and DFT.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Photocatalytic Reduction CO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">CO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Mn-based Complexes</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Chen, Yu-Mei</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Xu, Quan-Qing</subfield><subfield code="0">(orcid)0000-0001-5377-901X</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Yang, Zhi</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Catalysis letters</subfield><subfield code="d">Springer US, 1988</subfield><subfield code="g">153(2022), 10 vom: 23. Nov., Seite 2910-2916</subfield><subfield code="w">(DE-627)130436550</subfield><subfield code="w">(DE-600)644234-1</subfield><subfield code="w">(DE-576)025720724</subfield><subfield code="x">1011-372X</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:153</subfield><subfield code="g">year:2022</subfield><subfield code="g">number:10</subfield><subfield code="g">day:23</subfield><subfield code="g">month:11</subfield><subfield code="g">pages:2910-2916</subfield></datafield><datafield tag="856" ind1="4" ind2="1"><subfield code="u">https://doi.org/10.1007/s10562-022-04226-6</subfield><subfield code="z">lizenzpflichtig</subfield><subfield code="3">Volltext</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_OLC</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-TEC</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-CHE</subfield></datafield><datafield tag="936" ind1="r" ind2="v"><subfield code="a">VA 2890</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">153</subfield><subfield code="j">2022</subfield><subfield code="e">10</subfield><subfield code="b">23</subfield><subfield code="c">11</subfield><subfield code="h">2910-2916</subfield></datafield></record></collection>
|
score |
7.3998175 |