Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles
Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Yanwei [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s) 2018 |
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| Übergeordnetes Werk: |
Enthalten in: Pure and applied geophysics - Basel : Birkhäuser, 1939, 176(2018), 1 vom: 26. Juni, Seite 345-356 |
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| Übergeordnetes Werk: |
volume:176 ; year:2018 ; number:1 ; day:26 ; month:06 ; pages:345-356 |
| Links: |
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| DOI / URN: |
10.1007/s00024-018-1903-0 |
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| Katalog-ID: |
SPR000247677 |
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| 520 | |a Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. | ||
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| 650 | 4 | |a chemical aging |7 (dpeaa)DE-He213 | |
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10.1007/s00024-018-1903-0 doi (DE-627)SPR000247677 (SPR)s00024-018-1903-0-e DE-627 ger DE-627 rakwb eng Li, Yanwei verfasserin (orcid)0000-0002-5375-1751 aut Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2018 Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. Biomass burning particles (dpeaa)DE-He213 hygroscopic properties (dpeaa)DE-He213 CCN (dpeaa)DE-He213 chemical aging (dpeaa)DE-He213 Enthalten in Pure and applied geophysics Basel : Birkhäuser, 1939 176(2018), 1 vom: 26. Juni, Seite 345-356 (DE-627)265506743 (DE-600)1464028-4 1420-9136 nnns volume:176 year:2018 number:1 day:26 month:06 pages:345-356 https://dx.doi.org/10.1007/s00024-018-1903-0 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 176 2018 1 26 06 345-356 |
| spelling |
10.1007/s00024-018-1903-0 doi (DE-627)SPR000247677 (SPR)s00024-018-1903-0-e DE-627 ger DE-627 rakwb eng Li, Yanwei verfasserin (orcid)0000-0002-5375-1751 aut Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2018 Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. Biomass burning particles (dpeaa)DE-He213 hygroscopic properties (dpeaa)DE-He213 CCN (dpeaa)DE-He213 chemical aging (dpeaa)DE-He213 Enthalten in Pure and applied geophysics Basel : Birkhäuser, 1939 176(2018), 1 vom: 26. Juni, Seite 345-356 (DE-627)265506743 (DE-600)1464028-4 1420-9136 nnns volume:176 year:2018 number:1 day:26 month:06 pages:345-356 https://dx.doi.org/10.1007/s00024-018-1903-0 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 176 2018 1 26 06 345-356 |
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10.1007/s00024-018-1903-0 doi (DE-627)SPR000247677 (SPR)s00024-018-1903-0-e DE-627 ger DE-627 rakwb eng Li, Yanwei verfasserin (orcid)0000-0002-5375-1751 aut Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2018 Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. Biomass burning particles (dpeaa)DE-He213 hygroscopic properties (dpeaa)DE-He213 CCN (dpeaa)DE-He213 chemical aging (dpeaa)DE-He213 Enthalten in Pure and applied geophysics Basel : Birkhäuser, 1939 176(2018), 1 vom: 26. Juni, Seite 345-356 (DE-627)265506743 (DE-600)1464028-4 1420-9136 nnns volume:176 year:2018 number:1 day:26 month:06 pages:345-356 https://dx.doi.org/10.1007/s00024-018-1903-0 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 176 2018 1 26 06 345-356 |
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10.1007/s00024-018-1903-0 doi (DE-627)SPR000247677 (SPR)s00024-018-1903-0-e DE-627 ger DE-627 rakwb eng Li, Yanwei verfasserin (orcid)0000-0002-5375-1751 aut Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2018 Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. Biomass burning particles (dpeaa)DE-He213 hygroscopic properties (dpeaa)DE-He213 CCN (dpeaa)DE-He213 chemical aging (dpeaa)DE-He213 Enthalten in Pure and applied geophysics Basel : Birkhäuser, 1939 176(2018), 1 vom: 26. Juni, Seite 345-356 (DE-627)265506743 (DE-600)1464028-4 1420-9136 nnns volume:176 year:2018 number:1 day:26 month:06 pages:345-356 https://dx.doi.org/10.1007/s00024-018-1903-0 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 176 2018 1 26 06 345-356 |
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10.1007/s00024-018-1903-0 doi (DE-627)SPR000247677 (SPR)s00024-018-1903-0-e DE-627 ger DE-627 rakwb eng Li, Yanwei verfasserin (orcid)0000-0002-5375-1751 aut Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2018 Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. Biomass burning particles (dpeaa)DE-He213 hygroscopic properties (dpeaa)DE-He213 CCN (dpeaa)DE-He213 chemical aging (dpeaa)DE-He213 Enthalten in Pure and applied geophysics Basel : Birkhäuser, 1939 176(2018), 1 vom: 26. Juni, Seite 345-356 (DE-627)265506743 (DE-600)1464028-4 1420-9136 nnns volume:176 year:2018 number:1 day:26 month:06 pages:345-356 https://dx.doi.org/10.1007/s00024-018-1903-0 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 176 2018 1 26 06 345-356 |
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Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. 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Li, Yanwei |
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Li, Yanwei misc Biomass burning particles misc hygroscopic properties misc CCN misc chemical aging Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles |
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Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles Biomass burning particles (dpeaa)DE-He213 hygroscopic properties (dpeaa)DE-He213 CCN (dpeaa)DE-He213 chemical aging (dpeaa)DE-He213 |
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Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles |
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cloud condensation nuclei activity and hygroscopicity of fresh and aged biomass burning particles |
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Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles |
| abstract |
Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. © The Author(s) 2018 |
| abstractGer |
Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. © The Author(s) 2018 |
| abstract_unstemmed |
Abstract Biomass burning particles are one of the largest aerosol sources worldwide and contribute a significant fraction of the global cloud condensation nuclei (CCN) burden. Chemical aging experiments of sawgrass burning particles took place in a smog chamber by turning on the UV light after HONO or $ H_{2} %$ O_{2} $ injection. The CCN activity and corresponding hygroscopicity of fresh and aged particles were measured. Most of the fresh particles can serve as reasonable CCN, and the average activation diameters at 0.2% supersaturation were 114–125 nm in the experiments. The aging process caused that the mass fraction of organic aerosols decrease and condensed phase nitrate $ NO_{3} $− increase, and also the average atomic oxygen to carbon (O:C) ratios increase, which were the main reasons that the aged particles were more CCN active and hygroscopic. The average activation diameters decreased by 8–15% at 0.2% supersaturation after aging, and hygroscopic parameter κ increased by 30–42%. The chemical aging productions were a little different in experiments, but the CCN property and hygroscopicity change trends were quite similar. © The Author(s) 2018 |
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| title_short |
Cloud Condensation Nuclei Activity and Hygroscopicity of Fresh and Aged Biomass Burning Particles |
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https://dx.doi.org/10.1007/s00024-018-1903-0 |
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| doi_str |
10.1007/s00024-018-1903-0 |
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2024-07-03T14:55:01.398Z |
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| score |
7.4017506 |