Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles
Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Nilsson, Hans J. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2005 |
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| Schlagwörter: |
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| Anmerkung: |
© Springer-Verlag 2005 |
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| Übergeordnetes Werk: |
Enthalten in: Analytical and bioanalytical chemistry - Berlin : Springer, 2002, 383(2005), 1 vom: 14. Juli, Seite 41-47 |
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| Übergeordnetes Werk: |
volume:383 ; year:2005 ; number:1 ; day:14 ; month:07 ; pages:41-47 |
| Links: |
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| DOI / URN: |
10.1007/s00216-005-3355-5 |
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| Katalog-ID: |
SPR002152983 |
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| 245 | 1 | 0 | |a Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles |
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| 520 | |a Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. | ||
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| 650 | 4 | |a STXM |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a NEXAFS |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Spectromicroscopy |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Plutonium |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Neptunium |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Tyliszczak, Tolek |4 aut | |
| 700 | 1 | |a Wilson, Richard E. |4 aut | |
| 700 | 1 | |a Werme, Lars |4 aut | |
| 700 | 1 | |a Shuh, David K. |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Analytical and bioanalytical chemistry |d Berlin : Springer, 2002 |g 383(2005), 1 vom: 14. Juli, Seite 41-47 |w (DE-627)25372337X |w (DE-600)1459122-4 |x 1618-2650 |7 nnns |
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10.1007/s00216-005-3355-5 doi (DE-627)SPR002152983 (SPR)s00216-005-3355-5-e DE-627 ger DE-627 rakwb eng Nilsson, Hans J. verfasserin aut Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles 2005 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2005 Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. Actinide (dpeaa)DE-He213 STXM (dpeaa)DE-He213 NEXAFS (dpeaa)DE-He213 Spectromicroscopy (dpeaa)DE-He213 Plutonium (dpeaa)DE-He213 Neptunium (dpeaa)DE-He213 Tyliszczak, Tolek aut Wilson, Richard E. aut Werme, Lars aut Shuh, David K. aut Enthalten in Analytical and bioanalytical chemistry Berlin : Springer, 2002 383(2005), 1 vom: 14. Juli, Seite 41-47 (DE-627)25372337X (DE-600)1459122-4 1618-2650 nnns volume:383 year:2005 number:1 day:14 month:07 pages:41-47 https://dx.doi.org/10.1007/s00216-005-3355-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 383 2005 1 14 07 41-47 |
| spelling |
10.1007/s00216-005-3355-5 doi (DE-627)SPR002152983 (SPR)s00216-005-3355-5-e DE-627 ger DE-627 rakwb eng Nilsson, Hans J. verfasserin aut Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles 2005 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2005 Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. Actinide (dpeaa)DE-He213 STXM (dpeaa)DE-He213 NEXAFS (dpeaa)DE-He213 Spectromicroscopy (dpeaa)DE-He213 Plutonium (dpeaa)DE-He213 Neptunium (dpeaa)DE-He213 Tyliszczak, Tolek aut Wilson, Richard E. aut Werme, Lars aut Shuh, David K. aut Enthalten in Analytical and bioanalytical chemistry Berlin : Springer, 2002 383(2005), 1 vom: 14. Juli, Seite 41-47 (DE-627)25372337X (DE-600)1459122-4 1618-2650 nnns volume:383 year:2005 number:1 day:14 month:07 pages:41-47 https://dx.doi.org/10.1007/s00216-005-3355-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 383 2005 1 14 07 41-47 |
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10.1007/s00216-005-3355-5 doi (DE-627)SPR002152983 (SPR)s00216-005-3355-5-e DE-627 ger DE-627 rakwb eng Nilsson, Hans J. verfasserin aut Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles 2005 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2005 Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. Actinide (dpeaa)DE-He213 STXM (dpeaa)DE-He213 NEXAFS (dpeaa)DE-He213 Spectromicroscopy (dpeaa)DE-He213 Plutonium (dpeaa)DE-He213 Neptunium (dpeaa)DE-He213 Tyliszczak, Tolek aut Wilson, Richard E. aut Werme, Lars aut Shuh, David K. aut Enthalten in Analytical and bioanalytical chemistry Berlin : Springer, 2002 383(2005), 1 vom: 14. Juli, Seite 41-47 (DE-627)25372337X (DE-600)1459122-4 1618-2650 nnns volume:383 year:2005 number:1 day:14 month:07 pages:41-47 https://dx.doi.org/10.1007/s00216-005-3355-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 383 2005 1 14 07 41-47 |
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10.1007/s00216-005-3355-5 doi (DE-627)SPR002152983 (SPR)s00216-005-3355-5-e DE-627 ger DE-627 rakwb eng Nilsson, Hans J. verfasserin aut Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles 2005 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2005 Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. Actinide (dpeaa)DE-He213 STXM (dpeaa)DE-He213 NEXAFS (dpeaa)DE-He213 Spectromicroscopy (dpeaa)DE-He213 Plutonium (dpeaa)DE-He213 Neptunium (dpeaa)DE-He213 Tyliszczak, Tolek aut Wilson, Richard E. aut Werme, Lars aut Shuh, David K. aut Enthalten in Analytical and bioanalytical chemistry Berlin : Springer, 2002 383(2005), 1 vom: 14. Juli, Seite 41-47 (DE-627)25372337X (DE-600)1459122-4 1618-2650 nnns volume:383 year:2005 number:1 day:14 month:07 pages:41-47 https://dx.doi.org/10.1007/s00216-005-3355-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 383 2005 1 14 07 41-47 |
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10.1007/s00216-005-3355-5 doi (DE-627)SPR002152983 (SPR)s00216-005-3355-5-e DE-627 ger DE-627 rakwb eng Nilsson, Hans J. verfasserin aut Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles 2005 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2005 Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. Actinide (dpeaa)DE-He213 STXM (dpeaa)DE-He213 NEXAFS (dpeaa)DE-He213 Spectromicroscopy (dpeaa)DE-He213 Plutonium (dpeaa)DE-He213 Neptunium (dpeaa)DE-He213 Tyliszczak, Tolek aut Wilson, Richard E. aut Werme, Lars aut Shuh, David K. aut Enthalten in Analytical and bioanalytical chemistry Berlin : Springer, 2002 383(2005), 1 vom: 14. Juli, Seite 41-47 (DE-627)25372337X (DE-600)1459122-4 1618-2650 nnns volume:383 year:2005 number:1 day:14 month:07 pages:41-47 https://dx.doi.org/10.1007/s00216-005-3355-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 383 2005 1 14 07 41-47 |
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English |
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Enthalten in Analytical and bioanalytical chemistry 383(2005), 1 vom: 14. Juli, Seite 41-47 volume:383 year:2005 number:1 day:14 month:07 pages:41-47 |
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Enthalten in Analytical and bioanalytical chemistry 383(2005), 1 vom: 14. Juli, Seite 41-47 volume:383 year:2005 number:1 day:14 month:07 pages:41-47 |
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Actinide STXM NEXAFS Spectromicroscopy Plutonium Neptunium |
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Analytical and bioanalytical chemistry |
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Nilsson, Hans J. @@aut@@ Tyliszczak, Tolek @@aut@@ Wilson, Richard E. @@aut@@ Werme, Lars @@aut@@ Shuh, David K. @@aut@@ |
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2005-07-14T00:00:00Z |
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The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. 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Nilsson, Hans J. |
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Nilsson, Hans J. misc Actinide misc STXM misc NEXAFS misc Spectromicroscopy misc Plutonium misc Neptunium Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles |
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Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles Actinide (dpeaa)DE-He213 STXM (dpeaa)DE-He213 NEXAFS (dpeaa)DE-He213 Spectromicroscopy (dpeaa)DE-He213 Plutonium (dpeaa)DE-He213 Neptunium (dpeaa)DE-He213 |
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misc Actinide misc STXM misc NEXAFS misc Spectromicroscopy misc Plutonium misc Neptunium |
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Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles |
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Nilsson, Hans J. |
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Analytical and bioanalytical chemistry |
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Nilsson, Hans J. Tyliszczak, Tolek Wilson, Richard E. Werme, Lars Shuh, David K. |
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Nilsson, Hans J. |
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10.1007/s00216-005-3355-5 |
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soft x-ray scanning transmission x-ray microscopy (stxm) of actinide particles |
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Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles |
| abstract |
Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. © Springer-Verlag 2005 |
| abstractGer |
Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. © Springer-Verlag 2005 |
| abstract_unstemmed |
Abstract A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide $ 4d_{5/2} $ edges of the imaged transuranic particles, $ NpO_{2} $ and $ PuO_{2} $, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the $ 4d_{5/2} $ edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular $ PuO_{2} $ particle with the dimensions of 650 × 650 nm. The Pu $ 4d_{5/2} $ NEXAFS spectra were collected at several different locations from the $ PuO_{2} $ particle and were identical. A representative oxygen K-edge spectrum from $ UO_{2} $ was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. © Springer-Verlag 2005 |
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| title_short |
Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles |
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https://dx.doi.org/10.1007/s00216-005-3355-5 |
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Tyliszczak, Tolek Wilson, Richard E. Werme, Lars Shuh, David K. |
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Tyliszczak, Tolek Wilson, Richard E. Werme, Lars Shuh, David K. |
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| doi_str |
10.1007/s00216-005-3355-5 |
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2024-07-04T01:55:44.418Z |
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|
| score |
7.40007 |