Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles
Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP n...
Ausführliche Beschreibung
Autor*in: |
Zhang, Qixian [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2008 |
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Schlagwörter: |
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Anmerkung: |
© Springer-Verlag 2008 |
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Übergeordnetes Werk: |
Enthalten in: Applied physics - Berlin : Springer, 1973, 91(2008), 4 vom: 10. Apr., Seite 631-635 |
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Übergeordnetes Werk: |
volume:91 ; year:2008 ; number:4 ; day:10 ; month:04 ; pages:631-635 |
Links: |
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DOI / URN: |
10.1007/s00339-008-4491-5 |
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Katalog-ID: |
SPR004099664 |
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520 | |a Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. | ||
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10.1007/s00339-008-4491-5 doi (DE-627)SPR004099664 (SPR)s00339-008-4491-5-e DE-627 ger DE-627 rakwb eng Zhang, Qixian verfasserin aut Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2008 Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. Line Shape (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Aggregation Effect (dpeaa)DE-He213 Typical Transmission Electron Microscopy Image (dpeaa)DE-He213 Longitudinal Optical (dpeaa)DE-He213 Zhang, Zhaochun aut Enthalten in Applied physics Berlin : Springer, 1973 91(2008), 4 vom: 10. Apr., Seite 631-635 (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:91 year:2008 number:4 day:10 month:04 pages:631-635 https://dx.doi.org/10.1007/s00339-008-4491-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 91 2008 4 10 04 631-635 |
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10.1007/s00339-008-4491-5 doi (DE-627)SPR004099664 (SPR)s00339-008-4491-5-e DE-627 ger DE-627 rakwb eng Zhang, Qixian verfasserin aut Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2008 Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. Line Shape (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Aggregation Effect (dpeaa)DE-He213 Typical Transmission Electron Microscopy Image (dpeaa)DE-He213 Longitudinal Optical (dpeaa)DE-He213 Zhang, Zhaochun aut Enthalten in Applied physics Berlin : Springer, 1973 91(2008), 4 vom: 10. Apr., Seite 631-635 (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:91 year:2008 number:4 day:10 month:04 pages:631-635 https://dx.doi.org/10.1007/s00339-008-4491-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 91 2008 4 10 04 631-635 |
allfields_unstemmed |
10.1007/s00339-008-4491-5 doi (DE-627)SPR004099664 (SPR)s00339-008-4491-5-e DE-627 ger DE-627 rakwb eng Zhang, Qixian verfasserin aut Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2008 Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. Line Shape (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Aggregation Effect (dpeaa)DE-He213 Typical Transmission Electron Microscopy Image (dpeaa)DE-He213 Longitudinal Optical (dpeaa)DE-He213 Zhang, Zhaochun aut Enthalten in Applied physics Berlin : Springer, 1973 91(2008), 4 vom: 10. Apr., Seite 631-635 (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:91 year:2008 number:4 day:10 month:04 pages:631-635 https://dx.doi.org/10.1007/s00339-008-4491-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 91 2008 4 10 04 631-635 |
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10.1007/s00339-008-4491-5 doi (DE-627)SPR004099664 (SPR)s00339-008-4491-5-e DE-627 ger DE-627 rakwb eng Zhang, Qixian verfasserin aut Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles 2008 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag 2008 Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. Line Shape (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Aggregation Effect (dpeaa)DE-He213 Typical Transmission Electron Microscopy Image (dpeaa)DE-He213 Longitudinal Optical (dpeaa)DE-He213 Zhang, Zhaochun aut Enthalten in Applied physics Berlin : Springer, 1973 91(2008), 4 vom: 10. Apr., Seite 631-635 (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:91 year:2008 number:4 day:10 month:04 pages:631-635 https://dx.doi.org/10.1007/s00339-008-4491-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 91 2008 4 10 04 631-635 |
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Enthalten in Applied physics 91(2008), 4 vom: 10. Apr., Seite 631-635 volume:91 year:2008 number:4 day:10 month:04 pages:631-635 |
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Enthalten in Applied physics 91(2008), 4 vom: 10. Apr., Seite 631-635 volume:91 year:2008 number:4 day:10 month:04 pages:631-635 |
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Applied physics |
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Zhang, Qixian @@aut@@ Zhang, Zhaochun @@aut@@ |
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2008-04-10T00:00:00Z |
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surface mode absorption and infrared optical properties of gallium phosphide nanoparticles |
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Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles |
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Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. © Springer-Verlag 2008 |
abstractGer |
Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. © Springer-Verlag 2008 |
abstract_unstemmed |
Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function. © Springer-Verlag 2008 |
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Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR004099664</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230328150636.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">201001s2008 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s00339-008-4491-5</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR004099664</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s00339-008-4491-5-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Zhang, Qixian</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Surface mode absorption and infrared optical properties of gallium phosphide nanoparticles</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2008</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© Springer-Verlag 2008</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract The surface optical (SO) mode of ellipsoidal gallium phosphide (GaP) nanoparticles is investigated by infrared transmission spectroscopy. The surface mode theory of diatomic cubic particles is generalized and applied to GaP nanoparticles in a systematic treatment. The Fröhlich mode of GaP nanoparticles has been observed in our experiment. As far as surface mode frequency is concerned, the result of the experiment agrees with that of the theoretical calculation. The characteristics of the SO mode peak, including frequency shift, broadening and line shape, are analyzed. The frequency shift is attributed to the surrounding medium effect, surface oxidation and the aggregation effect as well as intrinsic point defects; the broadening is mainly due to the non-spherical particle shape, aggregation and quantum confinement effect; and the line shape is related to the particle shape and the damping function.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Line Shape</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Optical Phonon</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Aggregation Effect</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Typical Transmission Electron Microscopy Image</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Longitudinal Optical</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Zhang, Zhaochun</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Applied physics</subfield><subfield code="d">Berlin : Springer, 1973</subfield><subfield code="g">91(2008), 4 vom: 10. Apr., Seite 631-635</subfield><subfield code="w">(DE-627)235503231</subfield><subfield code="w">(DE-600)1398311-8</subfield><subfield code="x">1432-0630</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:91</subfield><subfield code="g">year:2008</subfield><subfield code="g">number:4</subfield><subfield code="g">day:10</subfield><subfield code="g">month:04</subfield><subfield code="g">pages:631-635</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">https://dx.doi.org/10.1007/s00339-008-4491-5</subfield><subfield code="z">lizenzpflichtig</subfield><subfield code="3">Volltext</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_SPRINGER</subfield></datafield><datafield tag="912" 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