Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal

Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands,...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Ouni, Inès Bejaoui [verfasserIn] Chapron, David Aroui, Hassen Fontana, Marc D.

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2016

Schlagwörter:	BaTiO3 Tetragonal Phase Optical Phonon Phonon Frequency Phonon Dispersion Curve

Anmerkung:	© Springer-Verlag Berlin Heidelberg 2016

Übergeordnetes Werk:	Enthalten in: Applied physics - Berlin : Springer, 1973, 122(2016), 4 vom: 04. Apr.
Übergeordnetes Werk:	volume:122 ; year:2016 ; number:4 ; day:04 ; month:04

Links:	Volltext

DOI / URN:	10.1007/s00339-016-0013-z

Katalog-ID:	SPR004160444

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245	1	0	\|a Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal
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520			\|a Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion.
650		4	\|a BaTiO3 \|7 (dpeaa)DE-He213
650		4	\|a Tetragonal Phase \|7 (dpeaa)DE-He213
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650		4	\|a Phonon Frequency \|7 (dpeaa)DE-He213
650		4	\|a Phonon Dispersion Curve \|7 (dpeaa)DE-He213
700	1		\|a Chapron, David \|4 aut
700	1		\|a Aroui, Hassen \|4 aut
700	1		\|a Fontana, Marc D. \|4 aut
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matchkey_str	article:14320630:2016----::hrabhvoohgfeunypiapoosnergnl
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publishDate	2016
allfields	10.1007/s00339-016-0013-z doi (DE-627)SPR004160444 (SPR)s00339-016-0013-z-e DE-627 ger DE-627 rakwb eng Ouni, Inès Bejaoui verfasserin aut Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. BaTiO3 (dpeaa)DE-He213 Tetragonal Phase (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Phonon Frequency (dpeaa)DE-He213 Phonon Dispersion Curve (dpeaa)DE-He213 Chapron, David aut Aroui, Hassen aut Fontana, Marc D. aut Enthalten in Applied physics Berlin : Springer, 1973 122(2016), 4 vom: 04. Apr. (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:122 year:2016 number:4 day:04 month:04 https://dx.doi.org/10.1007/s00339-016-0013-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 122 2016 4 04 04
spelling	10.1007/s00339-016-0013-z doi (DE-627)SPR004160444 (SPR)s00339-016-0013-z-e DE-627 ger DE-627 rakwb eng Ouni, Inès Bejaoui verfasserin aut Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. BaTiO3 (dpeaa)DE-He213 Tetragonal Phase (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Phonon Frequency (dpeaa)DE-He213 Phonon Dispersion Curve (dpeaa)DE-He213 Chapron, David aut Aroui, Hassen aut Fontana, Marc D. aut Enthalten in Applied physics Berlin : Springer, 1973 122(2016), 4 vom: 04. Apr. (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:122 year:2016 number:4 day:04 month:04 https://dx.doi.org/10.1007/s00339-016-0013-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 122 2016 4 04 04
allfields_unstemmed	10.1007/s00339-016-0013-z doi (DE-627)SPR004160444 (SPR)s00339-016-0013-z-e DE-627 ger DE-627 rakwb eng Ouni, Inès Bejaoui verfasserin aut Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. BaTiO3 (dpeaa)DE-He213 Tetragonal Phase (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Phonon Frequency (dpeaa)DE-He213 Phonon Dispersion Curve (dpeaa)DE-He213 Chapron, David aut Aroui, Hassen aut Fontana, Marc D. aut Enthalten in Applied physics Berlin : Springer, 1973 122(2016), 4 vom: 04. Apr. (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:122 year:2016 number:4 day:04 month:04 https://dx.doi.org/10.1007/s00339-016-0013-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 122 2016 4 04 04
allfieldsGer	10.1007/s00339-016-0013-z doi (DE-627)SPR004160444 (SPR)s00339-016-0013-z-e DE-627 ger DE-627 rakwb eng Ouni, Inès Bejaoui verfasserin aut Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. BaTiO3 (dpeaa)DE-He213 Tetragonal Phase (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Phonon Frequency (dpeaa)DE-He213 Phonon Dispersion Curve (dpeaa)DE-He213 Chapron, David aut Aroui, Hassen aut Fontana, Marc D. aut Enthalten in Applied physics Berlin : Springer, 1973 122(2016), 4 vom: 04. Apr. (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:122 year:2016 number:4 day:04 month:04 https://dx.doi.org/10.1007/s00339-016-0013-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 122 2016 4 04 04
allfieldsSound	10.1007/s00339-016-0013-z doi (DE-627)SPR004160444 (SPR)s00339-016-0013-z-e DE-627 ger DE-627 rakwb eng Ouni, Inès Bejaoui verfasserin aut Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. BaTiO3 (dpeaa)DE-He213 Tetragonal Phase (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Phonon Frequency (dpeaa)DE-He213 Phonon Dispersion Curve (dpeaa)DE-He213 Chapron, David aut Aroui, Hassen aut Fontana, Marc D. aut Enthalten in Applied physics Berlin : Springer, 1973 122(2016), 4 vom: 04. Apr. (DE-627)235503231 (DE-600)1398311-8 1432-0630 nnns volume:122 year:2016 number:4 day:04 month:04 https://dx.doi.org/10.1007/s00339-016-0013-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 122 2016 4 04 04
language	English
source	Enthalten in Applied physics 122(2016), 4 vom: 04. Apr. volume:122 year:2016 number:4 day:04 month:04
sourceStr	Enthalten in Applied physics 122(2016), 4 vom: 04. Apr. volume:122 year:2016 number:4 day:04 month:04
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	BaTiO3 Tetragonal Phase Optical Phonon Phonon Frequency Phonon Dispersion Curve
isfreeaccess_bool	false
container_title	Applied physics
authorswithroles_txt_mv	Ouni, Inès Bejaoui @@aut@@ Chapron, David @@aut@@ Aroui, Hassen @@aut@@ Fontana, Marc D. @@aut@@
publishDateDaySort_date	2016-04-04T00:00:00Z
hierarchy_top_id	235503231
id	SPR004160444
language_de	englisch
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author	Ouni, Inès Bejaoui
spellingShingle	Ouni, Inès Bejaoui misc BaTiO3 misc Tetragonal Phase misc Optical Phonon misc Phonon Frequency misc Phonon Dispersion Curve Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal
authorStr	Ouni, Inès Bejaoui
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topic_title	Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal BaTiO3 (dpeaa)DE-He213 Tetragonal Phase (dpeaa)DE-He213 Optical Phonon (dpeaa)DE-He213 Phonon Frequency (dpeaa)DE-He213 Phonon Dispersion Curve (dpeaa)DE-He213
topic	misc BaTiO3 misc Tetragonal Phase misc Optical Phonon misc Phonon Frequency misc Phonon Dispersion Curve
topic_unstemmed	misc BaTiO3 misc Tetragonal Phase misc Optical Phonon misc Phonon Frequency misc Phonon Dispersion Curve
topic_browse	misc BaTiO3 misc Tetragonal Phase misc Optical Phonon misc Phonon Frequency misc Phonon Dispersion Curve
format_facet	Elektronische Aufsätze Aufsätze Elektronische Ressource
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title	Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal
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title_full	Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal
author_sort	Ouni, Inès Bejaoui
journal	Applied physics
journalStr	Applied physics
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author_browse	Ouni, Inès Bejaoui Chapron, David Aroui, Hassen Fontana, Marc D.
container_volume	122
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author-letter	Ouni, Inès Bejaoui
doi_str_mv	10.1007/s00339-016-0013-z
title_sort	thermal behavior of high-frequency optical phonons in tetragonal $ batio_{3} $ single crystal
title_auth	Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal
abstract	Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. © Springer-Verlag Berlin Heidelberg 2016
abstractGer	Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. © Springer-Verlag Berlin Heidelberg 2016
abstract_unstemmed	Abstract The temperature dependence of the optical phonon modes in the tetragonal $ BaTiO_{3} $ single crystal was investigated by means of polarized Raman spectroscopy measurements. A special attention was devoted to the Raman spectra deconvolution to separate between first- and second-order bands, which can be discriminated from the difference in the temperature behavior of scattered intensity. Both A1 mode motions along the polar c axis and E vibrations (except the well-known soft mode) normal to c were studied and discussed. The temperature dependences of frequency and damping of each optical phonon were achieved and then interpreted in terms of third- and fourth-order anharmonic potential. It was derived from this analysis that the A1 transverse optical phonon arising from the hardening of the soft phonon of the cubic phase possesses large anharmonic motion of Ti versus O ions. A significant anharmonicity was as well found for phonons associated with O octahedral distortion. © Springer-Verlag Berlin Heidelberg 2016
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title_short	Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal
url	https://dx.doi.org/10.1007/s00339-016-0013-z
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author2	Chapron, David Aroui, Hassen Fontana, Marc D.
author2Str	Chapron, David Aroui, Hassen Fontana, Marc D.
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doi_str	10.1007/s00339-016-0013-z
up_date	2024-07-03T23:54:42.898Z
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Thermal behavior of high-frequency optical phonons in tetragonal $ BaTiO_{3} $ single crystal

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