Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries

Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on the...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Wang, Dan [verfasserIn] Wang, Yan [verfasserIn] Zou, Youlan [verfasserIn] Lu, Chunsheng [verfasserIn] Ma, Zengsheng [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2018

Übergeordnetes Werk:	Enthalten in: Acta mechanica - Wien : Springer, 1965, 229(2018), 8 vom: 09. Mai, Seite 3293-3303
Übergeordnetes Werk:	volume:229 ; year:2018 ; number:8 ; day:09 ; month:05 ; pages:3293-3303

Links:	Volltext

DOI / URN:	10.1007/s00707-018-2169-4

Katalog-ID:	SPR007512074

Internformat


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520			\|a Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes.
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author_variant	d w dw y w yw y z yz c l cl z m zm
matchkey_str	article:16196937:2018----::nstoimcaiapoeteosaoeiaihainrcs
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publishDate	2018
allfields	10.1007/s00707-018-2169-4 doi (DE-627)SPR007512074 (SPR)s00707-018-2169-4-e DE-627 ger DE-627 rakwb eng 530 ASE 50.31 bkl 50.33 bkl 33.11 bkl Wang, Dan verfasserin aut Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes. Wang, Yan verfasserin aut Zou, Youlan verfasserin aut Lu, Chunsheng verfasserin aut Ma, Zengsheng verfasserin aut Enthalten in Acta mechanica Wien : Springer, 1965 229(2018), 8 vom: 09. Mai, Seite 3293-3303 (DE-627)270126139 (DE-600)1476343-6 1619-6937 nnns volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303 https://dx.doi.org/10.1007/s00707-018-2169-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.31 ASE 50.33 ASE 33.11 ASE AR 229 2018 8 09 05 3293-3303
spelling	10.1007/s00707-018-2169-4 doi (DE-627)SPR007512074 (SPR)s00707-018-2169-4-e DE-627 ger DE-627 rakwb eng 530 ASE 50.31 bkl 50.33 bkl 33.11 bkl Wang, Dan verfasserin aut Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes. Wang, Yan verfasserin aut Zou, Youlan verfasserin aut Lu, Chunsheng verfasserin aut Ma, Zengsheng verfasserin aut Enthalten in Acta mechanica Wien : Springer, 1965 229(2018), 8 vom: 09. Mai, Seite 3293-3303 (DE-627)270126139 (DE-600)1476343-6 1619-6937 nnns volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303 https://dx.doi.org/10.1007/s00707-018-2169-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.31 ASE 50.33 ASE 33.11 ASE AR 229 2018 8 09 05 3293-3303
allfields_unstemmed	10.1007/s00707-018-2169-4 doi (DE-627)SPR007512074 (SPR)s00707-018-2169-4-e DE-627 ger DE-627 rakwb eng 530 ASE 50.31 bkl 50.33 bkl 33.11 bkl Wang, Dan verfasserin aut Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes. Wang, Yan verfasserin aut Zou, Youlan verfasserin aut Lu, Chunsheng verfasserin aut Ma, Zengsheng verfasserin aut Enthalten in Acta mechanica Wien : Springer, 1965 229(2018), 8 vom: 09. Mai, Seite 3293-3303 (DE-627)270126139 (DE-600)1476343-6 1619-6937 nnns volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303 https://dx.doi.org/10.1007/s00707-018-2169-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.31 ASE 50.33 ASE 33.11 ASE AR 229 2018 8 09 05 3293-3303
allfieldsGer	10.1007/s00707-018-2169-4 doi (DE-627)SPR007512074 (SPR)s00707-018-2169-4-e DE-627 ger DE-627 rakwb eng 530 ASE 50.31 bkl 50.33 bkl 33.11 bkl Wang, Dan verfasserin aut Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes. Wang, Yan verfasserin aut Zou, Youlan verfasserin aut Lu, Chunsheng verfasserin aut Ma, Zengsheng verfasserin aut Enthalten in Acta mechanica Wien : Springer, 1965 229(2018), 8 vom: 09. Mai, Seite 3293-3303 (DE-627)270126139 (DE-600)1476343-6 1619-6937 nnns volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303 https://dx.doi.org/10.1007/s00707-018-2169-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.31 ASE 50.33 ASE 33.11 ASE AR 229 2018 8 09 05 3293-3303
allfieldsSound	10.1007/s00707-018-2169-4 doi (DE-627)SPR007512074 (SPR)s00707-018-2169-4-e DE-627 ger DE-627 rakwb eng 530 ASE 50.31 bkl 50.33 bkl 33.11 bkl Wang, Dan verfasserin aut Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes. Wang, Yan verfasserin aut Zou, Youlan verfasserin aut Lu, Chunsheng verfasserin aut Ma, Zengsheng verfasserin aut Enthalten in Acta mechanica Wien : Springer, 1965 229(2018), 8 vom: 09. Mai, Seite 3293-3303 (DE-627)270126139 (DE-600)1476343-6 1619-6937 nnns volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303 https://dx.doi.org/10.1007/s00707-018-2169-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_267 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.31 ASE 50.33 ASE 33.11 ASE AR 229 2018 8 09 05 3293-3303
language	English
source	Enthalten in Acta mechanica 229(2018), 8 vom: 09. Mai, Seite 3293-3303 volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303
sourceStr	Enthalten in Acta mechanica 229(2018), 8 vom: 09. Mai, Seite 3293-3303 volume:229 year:2018 number:8 day:09 month:05 pages:3293-3303
format_phy_str_mv	Article
institution	findex.gbv.de
dewey-raw	530
isfreeaccess_bool	false
container_title	Acta mechanica
authorswithroles_txt_mv	Wang, Dan @@aut@@ Wang, Yan @@aut@@ Zou, Youlan @@aut@@ Lu, Chunsheng @@aut@@ Ma, Zengsheng @@aut@@
publishDateDaySort_date	2018-05-09T00:00:00Z
hierarchy_top_id	270126139
dewey-sort	3530
id	SPR007512074
language_de	englisch
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author	Wang, Dan
spellingShingle	Wang, Dan ddc 530 bkl 50.31 bkl 50.33 bkl 33.11 Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries
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topic_title	530 ASE 50.31 bkl 50.33 bkl 33.11 bkl Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries
topic	ddc 530 bkl 50.31 bkl 50.33 bkl 33.11
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title	Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries
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title_full	Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries
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author_browse	Wang, Dan Wang, Yan Zou, Youlan Lu, Chunsheng Ma, Zengsheng
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title_sort	anisotropic mechanical properties of si anodes in a lithiation process of lithium-ion batteries
title_auth	Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries
abstract	Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes.
abstractGer	Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes.
abstract_unstemmed	Abstract High-capacity active electrodes, such as Si anodes in Li-ion batteries, undergo a significant volume deformation of up to %$\sim %$ 400% during lithiation. Such a huge volume change could cause mechanical fracture and pulverization of electrode materials and result in harmful effects on their electrochemical performance. To have better understanding on this problem, the two-phase lithiation process of hollow core–shell and film structural electrodes is simulated by using a diffusion lithiation model. It is shown that the anisotropic hoop stress is larger than the isotropic one, which may easily induce damage of hollow core–shell negative electrodes. In addition, the anisotropic nature of mechanical properties can also remarkably magnify the edge stress intensity factor of hollow core–shell and film electrodes. These results on the morphological evolution and stress generation shed light on the design of novel and failure-resistant electrodes.
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container_issue	8
title_short	Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries
url	https://dx.doi.org/10.1007/s00707-018-2169-4
remote_bool	true
author2	Wang, Yan Zou, Youlan Lu, Chunsheng Ma, Zengsheng
author2Str	Wang, Yan Zou, Youlan Lu, Chunsheng Ma, Zengsheng
ppnlink	270126139
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doi_str	10.1007/s00707-018-2169-4
up_date	2024-07-03T13:26:03.387Z
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Anisotropic mechanical properties of Si anodes in a lithiation process of lithium-ion batteries

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