Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method
Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, p...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Shi, Limin [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2007 |
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| Schlagwörter: |
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| Anmerkung: |
© Springer Science+Business Media, LLC 2007 |
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| Übergeordnetes Werk: |
Enthalten in: Catalysis letters - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988, 113(2007), 1-2 vom: Jan., Seite 59-64 |
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| Übergeordnetes Werk: |
volume:113 ; year:2007 ; number:1-2 ; month:01 ; pages:59-64 |
| Links: |
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| DOI / URN: |
10.1007/s10562-006-9012-6 |
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| Katalog-ID: |
SPR011318619 |
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| 245 | 1 | 0 | |a Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method |
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| 520 | |a Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. | ||
| 650 | 4 | |a MnO |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a –CeO |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a mixed oxide |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a solid solution |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a methane combustion |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a low-temperature activity |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Chu, Wei |4 aut | |
| 700 | 1 | |a Qu, Fenfen |4 aut | |
| 700 | 1 | |a Luo, Shizhong |4 aut | |
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10.1007/s10562-006-9012-6 doi (DE-627)SPR011318619 (SPR)s10562-006-9012-6-e DE-627 ger DE-627 rakwb eng Shi, Limin verfasserin aut Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method 2007 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Science+Business Media, LLC 2007 Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. MnO (dpeaa)DE-He213 –CeO (dpeaa)DE-He213 mixed oxide (dpeaa)DE-He213 solid solution (dpeaa)DE-He213 methane combustion (dpeaa)DE-He213 low-temperature activity (dpeaa)DE-He213 Chu, Wei aut Qu, Fenfen aut Luo, Shizhong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 113(2007), 1-2 vom: Jan., Seite 59-64 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:113 year:2007 number:1-2 month:01 pages:59-64 https://dx.doi.org/10.1007/s10562-006-9012-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 113 2007 1-2 01 59-64 |
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10.1007/s10562-006-9012-6 doi (DE-627)SPR011318619 (SPR)s10562-006-9012-6-e DE-627 ger DE-627 rakwb eng Shi, Limin verfasserin aut Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method 2007 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Science+Business Media, LLC 2007 Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. MnO (dpeaa)DE-He213 –CeO (dpeaa)DE-He213 mixed oxide (dpeaa)DE-He213 solid solution (dpeaa)DE-He213 methane combustion (dpeaa)DE-He213 low-temperature activity (dpeaa)DE-He213 Chu, Wei aut Qu, Fenfen aut Luo, Shizhong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 113(2007), 1-2 vom: Jan., Seite 59-64 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:113 year:2007 number:1-2 month:01 pages:59-64 https://dx.doi.org/10.1007/s10562-006-9012-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 113 2007 1-2 01 59-64 |
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10.1007/s10562-006-9012-6 doi (DE-627)SPR011318619 (SPR)s10562-006-9012-6-e DE-627 ger DE-627 rakwb eng Shi, Limin verfasserin aut Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method 2007 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Science+Business Media, LLC 2007 Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. MnO (dpeaa)DE-He213 –CeO (dpeaa)DE-He213 mixed oxide (dpeaa)DE-He213 solid solution (dpeaa)DE-He213 methane combustion (dpeaa)DE-He213 low-temperature activity (dpeaa)DE-He213 Chu, Wei aut Qu, Fenfen aut Luo, Shizhong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 113(2007), 1-2 vom: Jan., Seite 59-64 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:113 year:2007 number:1-2 month:01 pages:59-64 https://dx.doi.org/10.1007/s10562-006-9012-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 113 2007 1-2 01 59-64 |
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10.1007/s10562-006-9012-6 doi (DE-627)SPR011318619 (SPR)s10562-006-9012-6-e DE-627 ger DE-627 rakwb eng Shi, Limin verfasserin aut Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method 2007 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Science+Business Media, LLC 2007 Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. MnO (dpeaa)DE-He213 –CeO (dpeaa)DE-He213 mixed oxide (dpeaa)DE-He213 solid solution (dpeaa)DE-He213 methane combustion (dpeaa)DE-He213 low-temperature activity (dpeaa)DE-He213 Chu, Wei aut Qu, Fenfen aut Luo, Shizhong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 113(2007), 1-2 vom: Jan., Seite 59-64 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:113 year:2007 number:1-2 month:01 pages:59-64 https://dx.doi.org/10.1007/s10562-006-9012-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 113 2007 1-2 01 59-64 |
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10.1007/s10562-006-9012-6 doi (DE-627)SPR011318619 (SPR)s10562-006-9012-6-e DE-627 ger DE-627 rakwb eng Shi, Limin verfasserin aut Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method 2007 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Science+Business Media, LLC 2007 Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. MnO (dpeaa)DE-He213 –CeO (dpeaa)DE-He213 mixed oxide (dpeaa)DE-He213 solid solution (dpeaa)DE-He213 methane combustion (dpeaa)DE-He213 low-temperature activity (dpeaa)DE-He213 Chu, Wei aut Qu, Fenfen aut Luo, Shizhong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 113(2007), 1-2 vom: Jan., Seite 59-64 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:113 year:2007 number:1-2 month:01 pages:59-64 https://dx.doi.org/10.1007/s10562-006-9012-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 113 2007 1-2 01 59-64 |
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Shi, Limin @@aut@@ Chu, Wei @@aut@@ Qu, Fenfen @@aut@@ Luo, Shizhong @@aut@@ |
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| author |
Shi, Limin |
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Shi, Limin misc MnO misc –CeO misc mixed oxide misc solid solution misc methane combustion misc low-temperature activity Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method |
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Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method MnO (dpeaa)DE-He213 –CeO (dpeaa)DE-He213 mixed oxide (dpeaa)DE-He213 solid solution (dpeaa)DE-He213 methane combustion (dpeaa)DE-He213 low-temperature activity (dpeaa)DE-He213 |
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Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method |
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Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method |
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Shi, Limin Chu, Wei Qu, Fenfen Luo, Shizhong |
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low-temperature catalytic combustion of methane over $ mno_{x} $–$ ceo_{2} $ mixed oxide catalysts: effect of preparation method |
| title_auth |
Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method |
| abstract |
Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. © Springer Science+Business Media, LLC 2007 |
| abstractGer |
Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. © Springer Science+Business Media, LLC 2007 |
| abstract_unstemmed |
Abstract The effect of preparation method on $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts for methane combustion at low temperature was investigated by means of BET, XRD, XPS, $ H_{2} $-TPR techniques and methane oxidation reaction. The catalysts were prepared by the conventional coprecipitation, plasma and modified coprecipitation methods, respectively. It was found that the catalyst prepared by modified coprecipitation was the most active, over which methane conversion reached 90% at a temperature as low as 390 °C. The XRD results showed the preparation methods had no effect on the solid solution structure of $ MnO_{x} $–$ CeO_{2} $ catalysts. More $ Mn^{4+} $ and richer lattice oxygen were found on the surface of the modified coprecipitation prepared catalyst with the help of XPS analysis, and its reduction and BET surface area were remarkably promoted. These factors could be responsible for its higher activity for methane combustion at low temperature. © Springer Science+Business Media, LLC 2007 |
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Low-temperature catalytic combustion of methane over $ MnO_{x} $–$ CeO_{2} $ mixed oxide catalysts: Effect of preparation method |
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https://dx.doi.org/10.1007/s10562-006-9012-6 |
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Chu, Wei Qu, Fenfen Luo, Shizhong |
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10.1007/s10562-006-9012-6 |
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| score |
7.3993587 |