Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Wan [verfasserIn] Xiao, Chengwei [verfasserIn] Zhao, Yuan [verfasserIn] Zhao, Qingqing [verfasserIn] Fan, Rong [verfasserIn] Xue, Jianjun [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2016 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Catalysis letters - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988, 146(2016), 12 vom: 28. Okt., Seite 2585-2595 |
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| Übergeordnetes Werk: |
volume:146 ; year:2016 ; number:12 ; day:28 ; month:10 ; pages:2585-2595 |
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| DOI / URN: |
10.1007/s10562-016-1894-3 |
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| Katalog-ID: |
SPR011345284 |
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| 520 | |a Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract | ||
| 650 | 4 | |a Nitrate |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Electrochemical reduction |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Dual-chamber cell |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Ti/TiO |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a nanotube array anode |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Fe |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Xiao, Chengwei |e verfasserin |4 aut | |
| 700 | 1 | |a Zhao, Yuan |e verfasserin |4 aut | |
| 700 | 1 | |a Zhao, Qingqing |e verfasserin |4 aut | |
| 700 | 1 | |a Fan, Rong |e verfasserin |4 aut | |
| 700 | 1 | |a Xue, Jianjun |e verfasserin |4 aut | |
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10.1007/s10562-016-1894-3 doi (DE-627)SPR011345284 (SPR)s10562-016-1894-3-e DE-627 ger DE-627 rakwb eng 540 660 ASE 35.17 bkl Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate (dpeaa)DE-He213 Electrochemical reduction (dpeaa)DE-He213 Dual-chamber cell (dpeaa)DE-He213 Ti/TiO (dpeaa)DE-He213 nanotube array anode (dpeaa)DE-He213 Fe (dpeaa)DE-He213 Xiao, Chengwei verfasserin aut Zhao, Yuan verfasserin aut Zhao, Qingqing verfasserin aut Fan, Rong verfasserin aut Xue, Jianjun verfasserin aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://dx.doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 ASE AR 146 2016 12 28 10 2585-2595 |
| spelling |
10.1007/s10562-016-1894-3 doi (DE-627)SPR011345284 (SPR)s10562-016-1894-3-e DE-627 ger DE-627 rakwb eng 540 660 ASE 35.17 bkl Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate (dpeaa)DE-He213 Electrochemical reduction (dpeaa)DE-He213 Dual-chamber cell (dpeaa)DE-He213 Ti/TiO (dpeaa)DE-He213 nanotube array anode (dpeaa)DE-He213 Fe (dpeaa)DE-He213 Xiao, Chengwei verfasserin aut Zhao, Yuan verfasserin aut Zhao, Qingqing verfasserin aut Fan, Rong verfasserin aut Xue, Jianjun verfasserin aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://dx.doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 ASE AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)SPR011345284 (SPR)s10562-016-1894-3-e DE-627 ger DE-627 rakwb eng 540 660 ASE 35.17 bkl Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate (dpeaa)DE-He213 Electrochemical reduction (dpeaa)DE-He213 Dual-chamber cell (dpeaa)DE-He213 Ti/TiO (dpeaa)DE-He213 nanotube array anode (dpeaa)DE-He213 Fe (dpeaa)DE-He213 Xiao, Chengwei verfasserin aut Zhao, Yuan verfasserin aut Zhao, Qingqing verfasserin aut Fan, Rong verfasserin aut Xue, Jianjun verfasserin aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://dx.doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 ASE AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)SPR011345284 (SPR)s10562-016-1894-3-e DE-627 ger DE-627 rakwb eng 540 660 ASE 35.17 bkl Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate (dpeaa)DE-He213 Electrochemical reduction (dpeaa)DE-He213 Dual-chamber cell (dpeaa)DE-He213 Ti/TiO (dpeaa)DE-He213 nanotube array anode (dpeaa)DE-He213 Fe (dpeaa)DE-He213 Xiao, Chengwei verfasserin aut Zhao, Yuan verfasserin aut Zhao, Qingqing verfasserin aut Fan, Rong verfasserin aut Xue, Jianjun verfasserin aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://dx.doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 ASE AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)SPR011345284 (SPR)s10562-016-1894-3-e DE-627 ger DE-627 rakwb eng 540 660 ASE 35.17 bkl Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate (dpeaa)DE-He213 Electrochemical reduction (dpeaa)DE-He213 Dual-chamber cell (dpeaa)DE-He213 Ti/TiO (dpeaa)DE-He213 nanotube array anode (dpeaa)DE-He213 Fe (dpeaa)DE-He213 Xiao, Chengwei verfasserin aut Zhao, Yuan verfasserin aut Zhao, Qingqing verfasserin aut Fan, Rong verfasserin aut Xue, Jianjun verfasserin aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://dx.doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 ASE AR 146 2016 12 28 10 2585-2595 |
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Enthalten in Catalysis letters 146(2016), 12 vom: 28. Okt., Seite 2585-2595 volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 |
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Nitrate Electrochemical reduction Dual-chamber cell Ti/TiO nanotube array anode Fe |
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Li, Wan @@aut@@ Xiao, Chengwei @@aut@@ Zhao, Yuan @@aut@@ Zhao, Qingqing @@aut@@ Fan, Rong @@aut@@ Xue, Jianjun @@aut@@ |
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The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. 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Li, Wan |
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Li, Wan ddc 540 bkl 35.17 misc Nitrate misc Electrochemical reduction misc Dual-chamber cell misc Ti/TiO misc nanotube array anode misc Fe Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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540 660 ASE 35.17 bkl Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell Nitrate (dpeaa)DE-He213 Electrochemical reduction (dpeaa)DE-He213 Dual-chamber cell (dpeaa)DE-He213 Ti/TiO (dpeaa)DE-He213 nanotube array anode (dpeaa)DE-He213 Fe (dpeaa)DE-He213 |
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ddc 540 bkl 35.17 misc Nitrate misc Electrochemical reduction misc Dual-chamber cell misc Ti/TiO misc nanotube array anode misc Fe |
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Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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Li, Wan Xiao, Chengwei Zhao, Yuan Zhao, Qingqing Fan, Rong Xue, Jianjun |
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Elektronische Aufsätze |
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Li, Wan |
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electrochemical reduction of high-concentrated nitrate using ti/$ tio_{2} $ nanotube array anode and fe cathode in dual-chamber cell |
| title_auth |
Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
| abstract |
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract |
| abstractGer |
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract |
| abstract_unstemmed |
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract |
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12 |
| title_short |
Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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https://dx.doi.org/10.1007/s10562-016-1894-3 |
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Xiao, Chengwei Zhao, Yuan Zhao, Qingqing Fan, Rong Xue, Jianjun |
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2024-07-03T22:04:16.607Z |
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| score |
7.401787 |