Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar

Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typic...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Musielak, Marion [verfasserIn] Brusseau, Mark L. [verfasserIn] Marcoux, Manuel [verfasserIn] Morrison, Candice [verfasserIn] Quintard, Michel [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2014

Schlagwörter:	Vapor intrusion NAPL Sorption Concrete Effective diffusion

Übergeordnetes Werk:	Enthalten in: Transport in porous media - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1986, 104(2014), 1 vom: 18. Mai, Seite 77-90
Übergeordnetes Werk:	volume:104 ; year:2014 ; number:1 ; day:18 ; month:05 ; pages:77-90

Links:	Volltext

DOI / URN:	10.1007/s11242-014-0321-8

Katalog-ID:	SPR018075444

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520			\|a Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion.
650		4	\|a Vapor intrusion \|7 (dpeaa)DE-He213
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650		4	\|a Effective diffusion \|7 (dpeaa)DE-He213
700	1		\|a Brusseau, Mark L. \|e verfasserin \|4 aut
700	1		\|a Marcoux, Manuel \|e verfasserin \|4 aut
700	1		\|a Morrison, Candice \|e verfasserin \|4 aut
700	1		\|a Quintard, Michel \|e verfasserin \|4 aut
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publishDate	2014
allfields	10.1007/s11242-014-0321-8 doi (DE-627)SPR018075444 (SPR)s11242-014-0321-8-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Musielak, Marion verfasserin aut Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion. Vapor intrusion (dpeaa)DE-He213 NAPL (dpeaa)DE-He213 Sorption (dpeaa)DE-He213 Concrete (dpeaa)DE-He213 Effective diffusion (dpeaa)DE-He213 Brusseau, Mark L. verfasserin aut Marcoux, Manuel verfasserin aut Morrison, Candice verfasserin aut Quintard, Michel verfasserin aut Enthalten in Transport in porous media Dordrecht [u.a.] : Springer Science + Business Media B.V, 1986 104(2014), 1 vom: 18. Mai, Seite 77-90 (DE-627)269017720 (DE-600)1473676-7 1573-1634 nnns volume:104 year:2014 number:1 day:18 month:05 pages:77-90 https://dx.doi.org/10.1007/s11242-014-0321-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 104 2014 1 18 05 77-90
spelling	10.1007/s11242-014-0321-8 doi (DE-627)SPR018075444 (SPR)s11242-014-0321-8-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Musielak, Marion verfasserin aut Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion. Vapor intrusion (dpeaa)DE-He213 NAPL (dpeaa)DE-He213 Sorption (dpeaa)DE-He213 Concrete (dpeaa)DE-He213 Effective diffusion (dpeaa)DE-He213 Brusseau, Mark L. verfasserin aut Marcoux, Manuel verfasserin aut Morrison, Candice verfasserin aut Quintard, Michel verfasserin aut Enthalten in Transport in porous media Dordrecht [u.a.] : Springer Science + Business Media B.V, 1986 104(2014), 1 vom: 18. Mai, Seite 77-90 (DE-627)269017720 (DE-600)1473676-7 1573-1634 nnns volume:104 year:2014 number:1 day:18 month:05 pages:77-90 https://dx.doi.org/10.1007/s11242-014-0321-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 104 2014 1 18 05 77-90
allfields_unstemmed	10.1007/s11242-014-0321-8 doi (DE-627)SPR018075444 (SPR)s11242-014-0321-8-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Musielak, Marion verfasserin aut Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion. Vapor intrusion (dpeaa)DE-He213 NAPL (dpeaa)DE-He213 Sorption (dpeaa)DE-He213 Concrete (dpeaa)DE-He213 Effective diffusion (dpeaa)DE-He213 Brusseau, Mark L. verfasserin aut Marcoux, Manuel verfasserin aut Morrison, Candice verfasserin aut Quintard, Michel verfasserin aut Enthalten in Transport in porous media Dordrecht [u.a.] : Springer Science + Business Media B.V, 1986 104(2014), 1 vom: 18. Mai, Seite 77-90 (DE-627)269017720 (DE-600)1473676-7 1573-1634 nnns volume:104 year:2014 number:1 day:18 month:05 pages:77-90 https://dx.doi.org/10.1007/s11242-014-0321-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 104 2014 1 18 05 77-90
allfieldsGer	10.1007/s11242-014-0321-8 doi (DE-627)SPR018075444 (SPR)s11242-014-0321-8-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Musielak, Marion verfasserin aut Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion. Vapor intrusion (dpeaa)DE-He213 NAPL (dpeaa)DE-He213 Sorption (dpeaa)DE-He213 Concrete (dpeaa)DE-He213 Effective diffusion (dpeaa)DE-He213 Brusseau, Mark L. verfasserin aut Marcoux, Manuel verfasserin aut Morrison, Candice verfasserin aut Quintard, Michel verfasserin aut Enthalten in Transport in porous media Dordrecht [u.a.] : Springer Science + Business Media B.V, 1986 104(2014), 1 vom: 18. Mai, Seite 77-90 (DE-627)269017720 (DE-600)1473676-7 1573-1634 nnns volume:104 year:2014 number:1 day:18 month:05 pages:77-90 https://dx.doi.org/10.1007/s11242-014-0321-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 104 2014 1 18 05 77-90
allfieldsSound	10.1007/s11242-014-0321-8 doi (DE-627)SPR018075444 (SPR)s11242-014-0321-8-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Musielak, Marion verfasserin aut Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion. Vapor intrusion (dpeaa)DE-He213 NAPL (dpeaa)DE-He213 Sorption (dpeaa)DE-He213 Concrete (dpeaa)DE-He213 Effective diffusion (dpeaa)DE-He213 Brusseau, Mark L. verfasserin aut Marcoux, Manuel verfasserin aut Morrison, Candice verfasserin aut Quintard, Michel verfasserin aut Enthalten in Transport in porous media Dordrecht [u.a.] : Springer Science + Business Media B.V, 1986 104(2014), 1 vom: 18. Mai, Seite 77-90 (DE-627)269017720 (DE-600)1473676-7 1573-1634 nnns volume:104 year:2014 number:1 day:18 month:05 pages:77-90 https://dx.doi.org/10.1007/s11242-014-0321-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 104 2014 1 18 05 77-90
language	English
source	Enthalten in Transport in porous media 104(2014), 1 vom: 18. Mai, Seite 77-90 volume:104 year:2014 number:1 day:18 month:05 pages:77-90
sourceStr	Enthalten in Transport in porous media 104(2014), 1 vom: 18. Mai, Seite 77-90 volume:104 year:2014 number:1 day:18 month:05 pages:77-90
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Vapor intrusion NAPL Sorption Concrete Effective diffusion
dewey-raw	530
isfreeaccess_bool	false
container_title	Transport in porous media
authorswithroles_txt_mv	Musielak, Marion @@aut@@ Brusseau, Mark L. @@aut@@ Marcoux, Manuel @@aut@@ Morrison, Candice @@aut@@ Quintard, Michel @@aut@@
publishDateDaySort_date	2014-05-18T00:00:00Z
hierarchy_top_id	269017720
dewey-sort	3530
id	SPR018075444
language_de	englisch
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author	Musielak, Marion
spellingShingle	Musielak, Marion ddc 530 bkl 33.00 misc Vapor intrusion misc NAPL misc Sorption misc Concrete misc Effective diffusion Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar
authorStr	Musielak, Marion
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topic_title	530 ASE 33.00 bkl Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar Vapor intrusion (dpeaa)DE-He213 NAPL (dpeaa)DE-He213 Sorption (dpeaa)DE-He213 Concrete (dpeaa)DE-He213 Effective diffusion (dpeaa)DE-He213
topic	ddc 530 bkl 33.00 misc Vapor intrusion misc NAPL misc Sorption misc Concrete misc Effective diffusion
topic_unstemmed	ddc 530 bkl 33.00 misc Vapor intrusion misc NAPL misc Sorption misc Concrete misc Effective diffusion
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title	Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar
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title_full	Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar
author_sort	Musielak, Marion
journal	Transport in porous media
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author_browse	Musielak, Marion Brusseau, Mark L. Marcoux, Manuel Morrison, Candice Quintard, Michel
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title_sort	determination of chlorinated solvent sorption by porous material—application to trichloroethene vapor on cement mortar
title_auth	Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar
abstract	Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion.
abstractGer	Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion.
abstract_unstemmed	Abstract Experiments have been performed to investigate the sorption of trichloroethene (TCE) vapor by concrete material or, more specifically, the cement mortar component. Gas-flow experiments were conducted using columns packed with small pieces of cement mortar obtained from the grinding of typical concrete material. Transport and retardation of TCE at high vapor concentrations (500 mg L%$^{-1})%$ was compared to that of a non-reactive gas tracer (Sulfur Hexafluoride, SF%$_{6})%$. The results show a large magnitude of retardation (retardation factor %$=%$ 23) and sorption (sorption coefficient %$=%$ 10.6 cm%$^{3}%$ g%$^{-1})%$ for TCE, compared to negligible sorption for SF%$_{6}%$. This magnitude of sorption obtained with pollutant vapor is much bigger than the one obtained for aqueous-flow experiments conducted for water-saturated systems. The considerable sorption exhibited for TCE under vapor-flow conditions is attributed to some combination of accumulation at the air-water interface and vapor-phase adsorption, both of which are anticipated to be significant for this system given the large surface area associated with the cement mortar. Transport of both SF%$_{6}%$ and TCE was simulated successfully with a two-region physical non-equilibrium model, consistent with the dual-medium structure of the crushed cement mortar. This work emphasizes the importance of taking into account sorption phenomena when modeling transport of volatile organic compounds through concrete material, especially in regard to assessing vapor intrusion.
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title_short	Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar
url	https://dx.doi.org/10.1007/s11242-014-0321-8
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author2	Brusseau, Mark L. Marcoux, Manuel Morrison, Candice Quintard, Michel
author2Str	Brusseau, Mark L. Marcoux, Manuel Morrison, Candice Quintard, Michel
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doi_str	10.1007/s11242-014-0321-8
up_date	2024-07-03T17:10:51.573Z
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Determination of Chlorinated Solvent Sorption by Porous Material—Application to Trichloroethene Vapor on Cement Mortar

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