Biosensing strategy based on photocurrent quenching of quantum dots via energy resonance absorption
Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absor...
Ausführliche Beschreibung
Autor*in: |
Wen, Guangming [verfasserIn] Wang, Peng [verfasserIn] Tu, Wenwen [verfasserIn] Lei, Jianping [verfasserIn] Ju, Huangxian [verfasserIn] |
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Englisch |
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2015 |
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Enthalten in: Science in China - Asheville, NC : Science in China Press, 1995, 58(2015), 5 vom: 15. März, Seite 879-884 |
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Übergeordnetes Werk: |
volume:58 ; year:2015 ; number:5 ; day:15 ; month:03 ; pages:879-884 |
Links: |
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DOI / URN: |
10.1007/s11426-014-5315-4 |
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520 | |a Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. | ||
650 | 4 | |a energy resonance absorption |7 (dpeaa)DE-He213 | |
650 | 4 | |a photocurrent quenching |7 (dpeaa)DE-He213 | |
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650 | 4 | |a biosensing |7 (dpeaa)DE-He213 | |
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700 | 1 | |a Ju, Huangxian |e verfasserin |4 aut | |
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10.1007/s11426-014-5315-4 doi (DE-627)SPR019171641 (SPR)s11426-014-5315-4-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Wen, Guangming verfasserin aut Biosensing strategy based on photocurrent quenching of quantum dots via energy resonance absorption 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. energy resonance absorption (dpeaa)DE-He213 photocurrent quenching (dpeaa)DE-He213 photoelelctrochemistry (dpeaa)DE-He213 biosensing (dpeaa)DE-He213 DNA (dpeaa)DE-He213 Wang, Peng verfasserin aut Tu, Wenwen verfasserin aut Lei, Jianping verfasserin aut Ju, Huangxian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 58(2015), 5 vom: 15. März, Seite 879-884 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:58 year:2015 number:5 day:15 month:03 pages:879-884 https://dx.doi.org/10.1007/s11426-014-5315-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 58 2015 5 15 03 879-884 |
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10.1007/s11426-014-5315-4 doi (DE-627)SPR019171641 (SPR)s11426-014-5315-4-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Wen, Guangming verfasserin aut Biosensing strategy based on photocurrent quenching of quantum dots via energy resonance absorption 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. energy resonance absorption (dpeaa)DE-He213 photocurrent quenching (dpeaa)DE-He213 photoelelctrochemistry (dpeaa)DE-He213 biosensing (dpeaa)DE-He213 DNA (dpeaa)DE-He213 Wang, Peng verfasserin aut Tu, Wenwen verfasserin aut Lei, Jianping verfasserin aut Ju, Huangxian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 58(2015), 5 vom: 15. März, Seite 879-884 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:58 year:2015 number:5 day:15 month:03 pages:879-884 https://dx.doi.org/10.1007/s11426-014-5315-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 58 2015 5 15 03 879-884 |
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10.1007/s11426-014-5315-4 doi (DE-627)SPR019171641 (SPR)s11426-014-5315-4-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Wen, Guangming verfasserin aut Biosensing strategy based on photocurrent quenching of quantum dots via energy resonance absorption 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. energy resonance absorption (dpeaa)DE-He213 photocurrent quenching (dpeaa)DE-He213 photoelelctrochemistry (dpeaa)DE-He213 biosensing (dpeaa)DE-He213 DNA (dpeaa)DE-He213 Wang, Peng verfasserin aut Tu, Wenwen verfasserin aut Lei, Jianping verfasserin aut Ju, Huangxian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 58(2015), 5 vom: 15. März, Seite 879-884 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:58 year:2015 number:5 day:15 month:03 pages:879-884 https://dx.doi.org/10.1007/s11426-014-5315-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 58 2015 5 15 03 879-884 |
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10.1007/s11426-014-5315-4 doi (DE-627)SPR019171641 (SPR)s11426-014-5315-4-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Wen, Guangming verfasserin aut Biosensing strategy based on photocurrent quenching of quantum dots via energy resonance absorption 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. energy resonance absorption (dpeaa)DE-He213 photocurrent quenching (dpeaa)DE-He213 photoelelctrochemistry (dpeaa)DE-He213 biosensing (dpeaa)DE-He213 DNA (dpeaa)DE-He213 Wang, Peng verfasserin aut Tu, Wenwen verfasserin aut Lei, Jianping verfasserin aut Ju, Huangxian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 58(2015), 5 vom: 15. März, Seite 879-884 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:58 year:2015 number:5 day:15 month:03 pages:879-884 https://dx.doi.org/10.1007/s11426-014-5315-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 58 2015 5 15 03 879-884 |
allfieldsSound |
10.1007/s11426-014-5315-4 doi (DE-627)SPR019171641 (SPR)s11426-014-5315-4-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Wen, Guangming verfasserin aut Biosensing strategy based on photocurrent quenching of quantum dots via energy resonance absorption 2015 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. energy resonance absorption (dpeaa)DE-He213 photocurrent quenching (dpeaa)DE-He213 photoelelctrochemistry (dpeaa)DE-He213 biosensing (dpeaa)DE-He213 DNA (dpeaa)DE-He213 Wang, Peng verfasserin aut Tu, Wenwen verfasserin aut Lei, Jianping verfasserin aut Ju, Huangxian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 58(2015), 5 vom: 15. März, Seite 879-884 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:58 year:2015 number:5 day:15 month:03 pages:879-884 https://dx.doi.org/10.1007/s11426-014-5315-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 58 2015 5 15 03 879-884 |
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The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. 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Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. |
abstractGer |
Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. |
abstract_unstemmed |
Abstract A new concept of energy resonance absorption for photocurrent quenching was proposed using a system of quantum dots (QDs) and the matched dye. The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. The result demonstrated that the photocurrent quenching via energy resonance absorption not only contributed to the theoretical study of photoelectrochemistry, but also provided a universal tool for photoelectrochemical biosensing. |
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The QDs were used as the photocurrent producer, and the dye had an absorption band overlapped with that of the QDs, which led to the resonance absorption of the excitation energy and thus decreased the photocurrent of QDs. By using porphyrin and fluorscein isothiocyanate isomer I as the resonance absorption dyes, the proposed mechanism was proved by UV-Vis spectra, photoluminescence spectra and photocurrent-to-wavelength response, respectively. The interaction of the absorption-matched dye with biomolecule could be conveniently used to introduce it into the photocurrent quenching system, leading to a simple switch-off biosensing method for detection of the biomolecule. As example, a label-free method was proposed for photoelectrochemical detection of target DNA. This method showed a detection range from 6.0 to 600 nmol/L with a detection limit of 2.5 nmol/L. 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