Investigation on two triphenylene based electron transport materials

Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of int...
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Autor*in:	Cai, Minghan [verfasserIn] Zhao, Chongguang [verfasserIn] Zhang, Dongdong [verfasserIn] Song, Xiaozeng [verfasserIn] Duan, Lian [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Übergeordnetes Werk:	Enthalten in: Science in China - Asheville, NC : Science in China Press, 1995, 62(2019), 6 vom: 28. März, Seite 775-783
Übergeordnetes Werk:	volume:62 ; year:2019 ; number:6 ; day:28 ; month:03 ; pages:775-783

Links:	Volltext

DOI / URN:	10.1007/s11426-018-9434-6

Katalog-ID:	SPR019181728

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520			\|a Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated.
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allfields	10.1007/s11426-018-9434-6 doi (DE-627)SPR019181728 (SPR)s11426-018-9434-6-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Cai, Minghan verfasserin aut Investigation on two triphenylene based electron transport materials 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated. Zhao, Chongguang verfasserin aut Zhang, Dongdong verfasserin aut Song, Xiaozeng verfasserin aut Duan, Lian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 62(2019), 6 vom: 28. März, Seite 775-783 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:62 year:2019 number:6 day:28 month:03 pages:775-783 https://dx.doi.org/10.1007/s11426-018-9434-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 62 2019 6 28 03 775-783
spelling	10.1007/s11426-018-9434-6 doi (DE-627)SPR019181728 (SPR)s11426-018-9434-6-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Cai, Minghan verfasserin aut Investigation on two triphenylene based electron transport materials 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated. Zhao, Chongguang verfasserin aut Zhang, Dongdong verfasserin aut Song, Xiaozeng verfasserin aut Duan, Lian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 62(2019), 6 vom: 28. März, Seite 775-783 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:62 year:2019 number:6 day:28 month:03 pages:775-783 https://dx.doi.org/10.1007/s11426-018-9434-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 62 2019 6 28 03 775-783
allfields_unstemmed	10.1007/s11426-018-9434-6 doi (DE-627)SPR019181728 (SPR)s11426-018-9434-6-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Cai, Minghan verfasserin aut Investigation on two triphenylene based electron transport materials 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated. Zhao, Chongguang verfasserin aut Zhang, Dongdong verfasserin aut Song, Xiaozeng verfasserin aut Duan, Lian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 62(2019), 6 vom: 28. März, Seite 775-783 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:62 year:2019 number:6 day:28 month:03 pages:775-783 https://dx.doi.org/10.1007/s11426-018-9434-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 62 2019 6 28 03 775-783
allfieldsGer	10.1007/s11426-018-9434-6 doi (DE-627)SPR019181728 (SPR)s11426-018-9434-6-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Cai, Minghan verfasserin aut Investigation on two triphenylene based electron transport materials 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated. Zhao, Chongguang verfasserin aut Zhang, Dongdong verfasserin aut Song, Xiaozeng verfasserin aut Duan, Lian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 62(2019), 6 vom: 28. März, Seite 775-783 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:62 year:2019 number:6 day:28 month:03 pages:775-783 https://dx.doi.org/10.1007/s11426-018-9434-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 62 2019 6 28 03 775-783
allfieldsSound	10.1007/s11426-018-9434-6 doi (DE-627)SPR019181728 (SPR)s11426-018-9434-6-e DE-627 ger DE-627 rakwb eng 540 550 570 ASE 35.00 bkl Cai, Minghan verfasserin aut Investigation on two triphenylene based electron transport materials 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated. Zhao, Chongguang verfasserin aut Zhang, Dongdong verfasserin aut Song, Xiaozeng verfasserin aut Duan, Lian verfasserin aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 62(2019), 6 vom: 28. März, Seite 775-783 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:62 year:2019 number:6 day:28 month:03 pages:775-783 https://dx.doi.org/10.1007/s11426-018-9434-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 35.00 ASE AR 62 2019 6 28 03 775-783
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author	Cai, Minghan
spellingShingle	Cai, Minghan ddc 540 bkl 35.00 Investigation on two triphenylene based electron transport materials
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title	Investigation on two triphenylene based electron transport materials
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title_full	Investigation on two triphenylene based electron transport materials
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title_sort	investigation on two triphenylene based electron transport materials
title_auth	Investigation on two triphenylene based electron transport materials
abstract	Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated.
abstractGer	Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated.
abstract_unstemmed	Abstract Promoting electron mobility is the key to designing high performance electron transport materials (ETMs). Formation of intermolecular interaction can be helpful to enhance their electron mobilities as a result of more ordered molecular stacking. Here, to reveal the inherent influence of intermolecular π-π stacking on the electron mobilities, we designed two ETMs, namely, 2,4-diphenyl-6-[3-(2-triphenylenyl)phenyl]-1,3,5-triazine (TPTRZ) and 2,4-diphenyl-6-[4′-(2-triphenylenyl)[1,1′-biphenyl]-3-yl]-1,3,5-triazine (TPPTRZ). Thermal, photophysical and electrochemical measurement results indicate they are good ETM candidates. Additionally, TPTRZ and TPPTRZ exhibit high electron mobilities of 3.60×$ 10^{−5} $ and 3.58×$ 10^{−5} $ $ cm^{2} $ $ V^{−1} $ $ s^{−1} $, respectively, at an electric field of 7×$ 10^{5} $ V $ cm^{−1} $. By taking X-ray single crystal structure, theoretical calculation and time of flight (TOF) results into consideration, it is revealed that strong intermolecular π-π stacking induced by planar triphenylene and triphenyltriazine units renders TPTRZ and TPPTRZ small energetic and positional disorder parameters, and results in their high electron mobilities thereby. By further enhancing intermolecular π-π stacking, ETMs with even higher electron mobilities can thus be anticipated.
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title_short	Investigation on two triphenylene based electron transport materials
url	https://dx.doi.org/10.1007/s11426-018-9434-6
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author2	Zhao, Chongguang Zhang, Dongdong Song, Xiaozeng Duan, Lian
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