Multiple sulfur and oxygen isotope compositions in Beijing aerosol
Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur sourc...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Guo, ZhaoBing [verfasserIn] Wu, MengLong [verfasserIn] Liu, FengLing [verfasserIn] Wei, Ying [verfasserIn] Li, DongFang [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2014 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Science in China - Heidelberg : Springer, 1997, 57(2014), 11 vom: 08. Aug., Seite 2671-2675 |
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| Übergeordnetes Werk: |
volume:57 ; year:2014 ; number:11 ; day:08 ; month:08 ; pages:2671-2675 |
| Links: |
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| DOI / URN: |
10.1007/s11430-014-4899-z |
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SPR019240783 |
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| 520 | |a Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. | ||
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10.1007/s11430-014-4899-z doi (DE-627)SPR019240783 (SPR)s11430-014-4899-z-e DE-627 ger DE-627 rakwb eng 550 ASE 38.00 bkl Guo, ZhaoBing verfasserin aut Multiple sulfur and oxygen isotope compositions in Beijing aerosol 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. Beijing aerosol (dpeaa)DE-He213 multiple sulfur isotope (dpeaa)DE-He213 oxygen isotope (dpeaa)DE-He213 mass-independent fractionation (dpeaa)DE-He213 Wu, MengLong verfasserin aut Liu, FengLing verfasserin aut Wei, Ying verfasserin aut Li, DongFang verfasserin aut Enthalten in Science in China Heidelberg : Springer, 1997 57(2014), 11 vom: 08. Aug., Seite 2671-2675 (DE-627)385614748 (DE-600)2142896-7 1862-2801 nnns volume:57 year:2014 number:11 day:08 month:08 pages:2671-2675 https://dx.doi.org/10.1007/s11430-014-4899-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 38.00 ASE AR 57 2014 11 08 08 2671-2675 |
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10.1007/s11430-014-4899-z doi (DE-627)SPR019240783 (SPR)s11430-014-4899-z-e DE-627 ger DE-627 rakwb eng 550 ASE 38.00 bkl Guo, ZhaoBing verfasserin aut Multiple sulfur and oxygen isotope compositions in Beijing aerosol 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. Beijing aerosol (dpeaa)DE-He213 multiple sulfur isotope (dpeaa)DE-He213 oxygen isotope (dpeaa)DE-He213 mass-independent fractionation (dpeaa)DE-He213 Wu, MengLong verfasserin aut Liu, FengLing verfasserin aut Wei, Ying verfasserin aut Li, DongFang verfasserin aut Enthalten in Science in China Heidelberg : Springer, 1997 57(2014), 11 vom: 08. Aug., Seite 2671-2675 (DE-627)385614748 (DE-600)2142896-7 1862-2801 nnns volume:57 year:2014 number:11 day:08 month:08 pages:2671-2675 https://dx.doi.org/10.1007/s11430-014-4899-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 38.00 ASE AR 57 2014 11 08 08 2671-2675 |
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10.1007/s11430-014-4899-z doi (DE-627)SPR019240783 (SPR)s11430-014-4899-z-e DE-627 ger DE-627 rakwb eng 550 ASE 38.00 bkl Guo, ZhaoBing verfasserin aut Multiple sulfur and oxygen isotope compositions in Beijing aerosol 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. Beijing aerosol (dpeaa)DE-He213 multiple sulfur isotope (dpeaa)DE-He213 oxygen isotope (dpeaa)DE-He213 mass-independent fractionation (dpeaa)DE-He213 Wu, MengLong verfasserin aut Liu, FengLing verfasserin aut Wei, Ying verfasserin aut Li, DongFang verfasserin aut Enthalten in Science in China Heidelberg : Springer, 1997 57(2014), 11 vom: 08. Aug., Seite 2671-2675 (DE-627)385614748 (DE-600)2142896-7 1862-2801 nnns volume:57 year:2014 number:11 day:08 month:08 pages:2671-2675 https://dx.doi.org/10.1007/s11430-014-4899-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 38.00 ASE AR 57 2014 11 08 08 2671-2675 |
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10.1007/s11430-014-4899-z doi (DE-627)SPR019240783 (SPR)s11430-014-4899-z-e DE-627 ger DE-627 rakwb eng 550 ASE 38.00 bkl Guo, ZhaoBing verfasserin aut Multiple sulfur and oxygen isotope compositions in Beijing aerosol 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. Beijing aerosol (dpeaa)DE-He213 multiple sulfur isotope (dpeaa)DE-He213 oxygen isotope (dpeaa)DE-He213 mass-independent fractionation (dpeaa)DE-He213 Wu, MengLong verfasserin aut Liu, FengLing verfasserin aut Wei, Ying verfasserin aut Li, DongFang verfasserin aut Enthalten in Science in China Heidelberg : Springer, 1997 57(2014), 11 vom: 08. Aug., Seite 2671-2675 (DE-627)385614748 (DE-600)2142896-7 1862-2801 nnns volume:57 year:2014 number:11 day:08 month:08 pages:2671-2675 https://dx.doi.org/10.1007/s11430-014-4899-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 38.00 ASE AR 57 2014 11 08 08 2671-2675 |
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10.1007/s11430-014-4899-z doi (DE-627)SPR019240783 (SPR)s11430-014-4899-z-e DE-627 ger DE-627 rakwb eng 550 ASE 38.00 bkl Guo, ZhaoBing verfasserin aut Multiple sulfur and oxygen isotope compositions in Beijing aerosol 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. Beijing aerosol (dpeaa)DE-He213 multiple sulfur isotope (dpeaa)DE-He213 oxygen isotope (dpeaa)DE-He213 mass-independent fractionation (dpeaa)DE-He213 Wu, MengLong verfasserin aut Liu, FengLing verfasserin aut Wei, Ying verfasserin aut Li, DongFang verfasserin aut Enthalten in Science in China Heidelberg : Springer, 1997 57(2014), 11 vom: 08. Aug., Seite 2671-2675 (DE-627)385614748 (DE-600)2142896-7 1862-2801 nnns volume:57 year:2014 number:11 day:08 month:08 pages:2671-2675 https://dx.doi.org/10.1007/s11430-014-4899-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 38.00 ASE AR 57 2014 11 08 08 2671-2675 |
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The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. 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multiple sulfur and oxygen isotope compositions in beijing aerosol |
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Multiple sulfur and oxygen isotope compositions in Beijing aerosol |
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Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. |
| abstractGer |
Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. |
| abstract_unstemmed |
Abstract Multiple sulfur isotopes (32S, 33S, 34S, 36S) and oxygen isotopes (16O, 18O) in Beijing aerosols were measured with MAT-253 isotope mass spectrometer. The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. In addition, thermochemical reactions of sulfur-bearing compounds might be also a source of sulfur isotope anomalies based on the correlation between $ Δ^{33} $S and CAPE. |
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The δ34S values of Beijing aerosol samples range from 1.68‰ to 12.57‰ with an average value of 5.86‰, indicating that the major sulfur source is from direct emission during coal combustion. The δ18O values vary from −5.29‰ to 9.02‰ with an average value of 5.17‰, revealing that the sulfate in Beijing aerosols is mainly composed of the secondary sulfate. The main heterogeneous oxidation of $ SO_{2} $ in atmosphere is related to $ H_{2} %$ O_{2} $ in July and August, whereas $ H_{2} %$ O_{2} $ oxidation and $ Fe^{3+} $ catalytic oxidation with $ SO_{2} $ exist simultaneously in September and October. Remarkable sulfur isotope mass-independent fractionation effect is found in Beijing aerosols, which is commonly attributed to the photochemical oxidation of $ SO_{2} $ in the stratosphere. 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