Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode

Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onse...
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Autor*in:	Araminaitė, Rūta [verfasserIn] Garjonytė, Rasa Malinauskas, Albertas

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2009

Schlagwörter:	Electrocatalysis Prussian blue Ascorbate Rotating disk electrode

Anmerkung:	© © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009

Übergeordnetes Werk:	Enthalten in: Central European journal of chemistry - Warsaw : Central European Science Journals, 2003, 7(2009), 4 vom: 22. Okt.
Übergeordnetes Werk:	volume:7 ; year:2009 ; number:4 ; day:22 ; month:10

Links:	Volltext

DOI / URN:	10.2478/s11532-009-0061-8

Katalog-ID:	SPR020603681

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520			\|a Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential.
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allfields	10.2478/s11532-009-0061-8 doi (DE-627)SPR020603681 (SPR)s11532-009-0061-8-e DE-627 ger DE-627 rakwb eng Araminaitė, Rūta verfasserin aut Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009 Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. Electrocatalysis (dpeaa)DE-He213 Prussian blue (dpeaa)DE-He213 Ascorbate (dpeaa)DE-He213 Rotating disk electrode (dpeaa)DE-He213 Garjonytė, Rasa aut Malinauskas, Albertas aut Enthalten in Central European journal of chemistry Warsaw : Central European Science Journals, 2003 7(2009), 4 vom: 22. Okt. (DE-627)358627516 (DE-600)2097193-X 1644-3624 nnns volume:7 year:2009 number:4 day:22 month:10 https://dx.doi.org/10.2478/s11532-009-0061-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2005 GBV_ILN_2014 GBV_ILN_2190 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2009 4 22 10
spelling	10.2478/s11532-009-0061-8 doi (DE-627)SPR020603681 (SPR)s11532-009-0061-8-e DE-627 ger DE-627 rakwb eng Araminaitė, Rūta verfasserin aut Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009 Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. Electrocatalysis (dpeaa)DE-He213 Prussian blue (dpeaa)DE-He213 Ascorbate (dpeaa)DE-He213 Rotating disk electrode (dpeaa)DE-He213 Garjonytė, Rasa aut Malinauskas, Albertas aut Enthalten in Central European journal of chemistry Warsaw : Central European Science Journals, 2003 7(2009), 4 vom: 22. Okt. (DE-627)358627516 (DE-600)2097193-X 1644-3624 nnns volume:7 year:2009 number:4 day:22 month:10 https://dx.doi.org/10.2478/s11532-009-0061-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2005 GBV_ILN_2014 GBV_ILN_2190 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2009 4 22 10
allfields_unstemmed	10.2478/s11532-009-0061-8 doi (DE-627)SPR020603681 (SPR)s11532-009-0061-8-e DE-627 ger DE-627 rakwb eng Araminaitė, Rūta verfasserin aut Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009 Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. Electrocatalysis (dpeaa)DE-He213 Prussian blue (dpeaa)DE-He213 Ascorbate (dpeaa)DE-He213 Rotating disk electrode (dpeaa)DE-He213 Garjonytė, Rasa aut Malinauskas, Albertas aut Enthalten in Central European journal of chemistry Warsaw : Central European Science Journals, 2003 7(2009), 4 vom: 22. Okt. (DE-627)358627516 (DE-600)2097193-X 1644-3624 nnns volume:7 year:2009 number:4 day:22 month:10 https://dx.doi.org/10.2478/s11532-009-0061-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2005 GBV_ILN_2014 GBV_ILN_2190 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2009 4 22 10
allfieldsGer	10.2478/s11532-009-0061-8 doi (DE-627)SPR020603681 (SPR)s11532-009-0061-8-e DE-627 ger DE-627 rakwb eng Araminaitė, Rūta verfasserin aut Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009 Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. Electrocatalysis (dpeaa)DE-He213 Prussian blue (dpeaa)DE-He213 Ascorbate (dpeaa)DE-He213 Rotating disk electrode (dpeaa)DE-He213 Garjonytė, Rasa aut Malinauskas, Albertas aut Enthalten in Central European journal of chemistry Warsaw : Central European Science Journals, 2003 7(2009), 4 vom: 22. Okt. (DE-627)358627516 (DE-600)2097193-X 1644-3624 nnns volume:7 year:2009 number:4 day:22 month:10 https://dx.doi.org/10.2478/s11532-009-0061-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2005 GBV_ILN_2014 GBV_ILN_2190 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2009 4 22 10
allfieldsSound	10.2478/s11532-009-0061-8 doi (DE-627)SPR020603681 (SPR)s11532-009-0061-8-e DE-627 ger DE-627 rakwb eng Araminaitė, Rūta verfasserin aut Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009 Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. Electrocatalysis (dpeaa)DE-He213 Prussian blue (dpeaa)DE-He213 Ascorbate (dpeaa)DE-He213 Rotating disk electrode (dpeaa)DE-He213 Garjonytė, Rasa aut Malinauskas, Albertas aut Enthalten in Central European journal of chemistry Warsaw : Central European Science Journals, 2003 7(2009), 4 vom: 22. Okt. (DE-627)358627516 (DE-600)2097193-X 1644-3624 nnns volume:7 year:2009 number:4 day:22 month:10 https://dx.doi.org/10.2478/s11532-009-0061-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2005 GBV_ILN_2014 GBV_ILN_2190 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2009 4 22 10
language	English
source	Enthalten in Central European journal of chemistry 7(2009), 4 vom: 22. Okt. volume:7 year:2009 number:4 day:22 month:10
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institution	findex.gbv.de
topic_facet	Electrocatalysis Prussian blue Ascorbate Rotating disk electrode
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container_title	Central European journal of chemistry
authorswithroles_txt_mv	Araminaitė, Rūta @@aut@@ Garjonytė, Rasa @@aut@@ Malinauskas, Albertas @@aut@@
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author	Araminaitė, Rūta
spellingShingle	Araminaitė, Rūta misc Electrocatalysis misc Prussian blue misc Ascorbate misc Rotating disk electrode Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode
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topic_title	Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode Electrocatalysis (dpeaa)DE-He213 Prussian blue (dpeaa)DE-He213 Ascorbate (dpeaa)DE-He213 Rotating disk electrode (dpeaa)DE-He213
topic	misc Electrocatalysis misc Prussian blue misc Ascorbate misc Rotating disk electrode
topic_unstemmed	misc Electrocatalysis misc Prussian blue misc Ascorbate misc Rotating disk electrode
topic_browse	misc Electrocatalysis misc Prussian blue misc Ascorbate misc Rotating disk electrode
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title	Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode
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title_full	Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode
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title_sort	rotating disk electrode study of electrocatalytic oxidation of ascorbate at prussian blue modified electrode
title_auth	Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode
abstract	Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009
abstractGer	Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009
abstract_unstemmed	Abstract Electrooxidation of ascorbate has been studied with the use of a rotating disk electrode. The results obtained show an efficient electrocatalytic oxidation of ascorbate at the Prussian blue (PB) modified electrode to proceed in solutions of pH 5.5 and 7.3. Depending on solution pH, the onset potential for ascorbate electrooxidation at PB modified electrode appears shifted by 0.1–0.2 V to lower values, as compared to an unmodified glassy carbon electrode. Within the electrode potential window of 0.3 to 0.5 V vs. Ag/AgCl, and electrode rotation velocity of 50–2000 rpm, the catalytic current obeys Koutecky-Levich equation at a submillimolar ascorbate concentration. Kinetic current densities, obtained from the data treatment, are higher for a pH 5.5 solution, and also at higher electrode potential. © © Versita Warsaw and Springer-Verlag Berlin Heidelberg 2009
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title_short	Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode
url	https://dx.doi.org/10.2478/s11532-009-0061-8
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Rotating disk electrode study of electrocatalytic oxidation of ascorbate at Prussian blue modified electrode

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