Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge

Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithi...
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Autor*in:	Natarajan, Angulakshmi [verfasserIn] Murugavel, Kathiresan Madasamy, Kanagaraj Suriyakumar, Shruti Illayaraja, N. Anupriya, N. Christy, Maria Nahm, K. S. Zhou, Yingke Stephan, A. Manuel

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	Lithium-air batteries Viologen Redox catalyst ORR

Anmerkung:	© Springer-Verlag GmbH Germany, part of Springer Nature 2019

Übergeordnetes Werk:	Enthalten in: Ionics - Berlin : Springer, 1995, 25(2019), 8 vom: 25. März, Seite 3837-3845
Übergeordnetes Werk:	volume:25 ; year:2019 ; number:8 ; day:25 ; month:03 ; pages:3837-3845

Links:	Volltext

DOI / URN:	10.1007/s11581-019-02955-0

Katalog-ID:	SPR02087667X

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520			\|a Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses.
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700	1		\|a Stephan, A. Manuel \|4 aut
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allfields	10.1007/s11581-019-02955-0 doi (DE-627)SPR02087667X (SPR)s11581-019-02955-0-e DE-627 ger DE-627 rakwb eng Natarajan, Angulakshmi verfasserin aut Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. Lithium-air batteries (dpeaa)DE-He213 Viologen (dpeaa)DE-He213 Redox catalyst (dpeaa)DE-He213 ORR (dpeaa)DE-He213 Murugavel, Kathiresan aut Madasamy, Kanagaraj aut Suriyakumar, Shruti aut Illayaraja, N. aut Anupriya, N. aut Christy, Maria aut Nahm, K. S. aut Zhou, Yingke aut Stephan, A. Manuel aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 8 vom: 25. März, Seite 3837-3845 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845 https://dx.doi.org/10.1007/s11581-019-02955-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 8 25 03 3837-3845
spelling	10.1007/s11581-019-02955-0 doi (DE-627)SPR02087667X (SPR)s11581-019-02955-0-e DE-627 ger DE-627 rakwb eng Natarajan, Angulakshmi verfasserin aut Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. Lithium-air batteries (dpeaa)DE-He213 Viologen (dpeaa)DE-He213 Redox catalyst (dpeaa)DE-He213 ORR (dpeaa)DE-He213 Murugavel, Kathiresan aut Madasamy, Kanagaraj aut Suriyakumar, Shruti aut Illayaraja, N. aut Anupriya, N. aut Christy, Maria aut Nahm, K. S. aut Zhou, Yingke aut Stephan, A. Manuel aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 8 vom: 25. März, Seite 3837-3845 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845 https://dx.doi.org/10.1007/s11581-019-02955-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 8 25 03 3837-3845
allfields_unstemmed	10.1007/s11581-019-02955-0 doi (DE-627)SPR02087667X (SPR)s11581-019-02955-0-e DE-627 ger DE-627 rakwb eng Natarajan, Angulakshmi verfasserin aut Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. Lithium-air batteries (dpeaa)DE-He213 Viologen (dpeaa)DE-He213 Redox catalyst (dpeaa)DE-He213 ORR (dpeaa)DE-He213 Murugavel, Kathiresan aut Madasamy, Kanagaraj aut Suriyakumar, Shruti aut Illayaraja, N. aut Anupriya, N. aut Christy, Maria aut Nahm, K. S. aut Zhou, Yingke aut Stephan, A. Manuel aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 8 vom: 25. März, Seite 3837-3845 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845 https://dx.doi.org/10.1007/s11581-019-02955-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 8 25 03 3837-3845
allfieldsGer	10.1007/s11581-019-02955-0 doi (DE-627)SPR02087667X (SPR)s11581-019-02955-0-e DE-627 ger DE-627 rakwb eng Natarajan, Angulakshmi verfasserin aut Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. Lithium-air batteries (dpeaa)DE-He213 Viologen (dpeaa)DE-He213 Redox catalyst (dpeaa)DE-He213 ORR (dpeaa)DE-He213 Murugavel, Kathiresan aut Madasamy, Kanagaraj aut Suriyakumar, Shruti aut Illayaraja, N. aut Anupriya, N. aut Christy, Maria aut Nahm, K. S. aut Zhou, Yingke aut Stephan, A. Manuel aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 8 vom: 25. März, Seite 3837-3845 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845 https://dx.doi.org/10.1007/s11581-019-02955-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 8 25 03 3837-3845
allfieldsSound	10.1007/s11581-019-02955-0 doi (DE-627)SPR02087667X (SPR)s11581-019-02955-0-e DE-627 ger DE-627 rakwb eng Natarajan, Angulakshmi verfasserin aut Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. Lithium-air batteries (dpeaa)DE-He213 Viologen (dpeaa)DE-He213 Redox catalyst (dpeaa)DE-He213 ORR (dpeaa)DE-He213 Murugavel, Kathiresan aut Madasamy, Kanagaraj aut Suriyakumar, Shruti aut Illayaraja, N. aut Anupriya, N. aut Christy, Maria aut Nahm, K. S. aut Zhou, Yingke aut Stephan, A. Manuel aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 8 vom: 25. März, Seite 3837-3845 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845 https://dx.doi.org/10.1007/s11581-019-02955-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 8 25 03 3837-3845
language	English
source	Enthalten in Ionics 25(2019), 8 vom: 25. März, Seite 3837-3845 volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845
sourceStr	Enthalten in Ionics 25(2019), 8 vom: 25. März, Seite 3837-3845 volume:25 year:2019 number:8 day:25 month:03 pages:3837-3845
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Lithium-air batteries Viologen Redox catalyst ORR
isfreeaccess_bool	false
container_title	Ionics
authorswithroles_txt_mv	Natarajan, Angulakshmi @@aut@@ Murugavel, Kathiresan @@aut@@ Madasamy, Kanagaraj @@aut@@ Suriyakumar, Shruti @@aut@@ Illayaraja, N. @@aut@@ Anupriya, N. @@aut@@ Christy, Maria @@aut@@ Nahm, K. S. @@aut@@ Zhou, Yingke @@aut@@ Stephan, A. Manuel @@aut@@
publishDateDaySort_date	2019-03-25T00:00:00Z
hierarchy_top_id	509398944
id	SPR02087667X
language_de	englisch
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author	Natarajan, Angulakshmi
spellingShingle	Natarajan, Angulakshmi misc Lithium-air batteries misc Viologen misc Redox catalyst misc ORR Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge
authorStr	Natarajan, Angulakshmi
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topic_title	Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge Lithium-air batteries (dpeaa)DE-He213 Viologen (dpeaa)DE-He213 Redox catalyst (dpeaa)DE-He213 ORR (dpeaa)DE-He213
topic	misc Lithium-air batteries misc Viologen misc Redox catalyst misc ORR
topic_unstemmed	misc Lithium-air batteries misc Viologen misc Redox catalyst misc ORR
topic_browse	misc Lithium-air batteries misc Viologen misc Redox catalyst misc ORR
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title	Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge
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title_full	Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge
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author_browse	Natarajan, Angulakshmi Murugavel, Kathiresan Madasamy, Kanagaraj Suriyakumar, Shruti Illayaraja, N. Anupriya, N. Christy, Maria Nahm, K. S. Zhou, Yingke Stephan, A. Manuel
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author-letter	Natarajan, Angulakshmi
doi_str_mv	10.1007/s11581-019-02955-0
title_sort	charge-discharge behavior of li-$ o_{2} $ cell with viologen as redox catalyst: influence of cationic charge
title_auth	Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge
abstract	Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. © Springer-Verlag GmbH Germany, part of Springer Nature 2019
abstractGer	Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. © Springer-Verlag GmbH Germany, part of Springer Nature 2019
abstract_unstemmed	Abstract The high theoretical energy density of lithium-air batteries has attracted the attention of many researchers as this system is expected to fulfill the demands radically from all sectors. Unfortunately, the issues such as deposition of undesirable discharge in the cathode, formation of lithium dendrites, and decomposition of electrolytes hamper it from commercialization. In the present work, viologens carrying different positive charges were synthesized and used as a catalyst in the carbon-assisted air cathode for the first time, and its cycling performance was analyzed. The lithium air cell with monomeric viologen offered highest discharge capacity and the deposition of $ Li_{2} %$ O_{2} $ in the cycled cathode was confirmed by XRD and FT-IR analyses. © Springer-Verlag GmbH Germany, part of Springer Nature 2019
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title_short	Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge
url	https://dx.doi.org/10.1007/s11581-019-02955-0
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author2	Murugavel, Kathiresan Madasamy, Kanagaraj Suriyakumar, Shruti Illayaraja, N. Anupriya, N. Christy, Maria Nahm, K. S. Zhou, Yingke Stephan, A. Manuel
author2Str	Murugavel, Kathiresan Madasamy, Kanagaraj Suriyakumar, Shruti Illayaraja, N. Anupriya, N. Christy, Maria Nahm, K. S. Zhou, Yingke Stephan, A. Manuel
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doi_str	10.1007/s11581-019-02955-0
up_date	2024-07-03T18:50:30.356Z
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Charge-discharge behavior of Li-$ O_{2} $ cell with viologen as redox catalyst: influence of cationic charge

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