Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction
Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray d...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Mengying [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Anmerkung: |
© Springer-Verlag GmbH Germany, part of Springer Nature 2019 |
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| Übergeordnetes Werk: |
Enthalten in: Ionics - Berlin : Springer, 1995, 25(2019), 9 vom: 26. Apr., Seite 4295-4303 |
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| Übergeordnetes Werk: |
volume:25 ; year:2019 ; number:9 ; day:26 ; month:04 ; pages:4295-4303 |
| Links: |
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| DOI / URN: |
10.1007/s11581-019-02976-9 |
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| Katalog-ID: |
SPR020876920 |
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| 520 | |a Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. | ||
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| 650 | 4 | |a Co-doped |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a High specific surface area |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Mesoporous |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Oxygen reduction reaction |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Wang, Chengyin |4 aut | |
| 700 | 1 | |a Hu, Shengnan |4 aut | |
| 700 | 1 | |a Wu, Huimin |4 aut | |
| 700 | 1 | |a Feng, Chuanqi |4 aut | |
| 700 | 1 | |a Zhang, Yanqing |4 aut | |
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10.1007/s11581-019-02976-9 doi (DE-627)SPR020876920 (SPR)s11581-019-02976-9-e DE-627 ger DE-627 rakwb eng Li, Mengying verfasserin aut Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. Carbon material (dpeaa)DE-He213 Co-doped (dpeaa)DE-He213 High specific surface area (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Wang, Chengyin aut Hu, Shengnan aut Wu, Huimin aut Feng, Chuanqi aut Zhang, Yanqing aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 9 vom: 26. Apr., Seite 4295-4303 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:9 day:26 month:04 pages:4295-4303 https://dx.doi.org/10.1007/s11581-019-02976-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 9 26 04 4295-4303 |
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10.1007/s11581-019-02976-9 doi (DE-627)SPR020876920 (SPR)s11581-019-02976-9-e DE-627 ger DE-627 rakwb eng Li, Mengying verfasserin aut Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. Carbon material (dpeaa)DE-He213 Co-doped (dpeaa)DE-He213 High specific surface area (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Wang, Chengyin aut Hu, Shengnan aut Wu, Huimin aut Feng, Chuanqi aut Zhang, Yanqing aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 9 vom: 26. Apr., Seite 4295-4303 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:9 day:26 month:04 pages:4295-4303 https://dx.doi.org/10.1007/s11581-019-02976-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 9 26 04 4295-4303 |
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10.1007/s11581-019-02976-9 doi (DE-627)SPR020876920 (SPR)s11581-019-02976-9-e DE-627 ger DE-627 rakwb eng Li, Mengying verfasserin aut Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. Carbon material (dpeaa)DE-He213 Co-doped (dpeaa)DE-He213 High specific surface area (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Wang, Chengyin aut Hu, Shengnan aut Wu, Huimin aut Feng, Chuanqi aut Zhang, Yanqing aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 9 vom: 26. Apr., Seite 4295-4303 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:9 day:26 month:04 pages:4295-4303 https://dx.doi.org/10.1007/s11581-019-02976-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 9 26 04 4295-4303 |
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10.1007/s11581-019-02976-9 doi (DE-627)SPR020876920 (SPR)s11581-019-02976-9-e DE-627 ger DE-627 rakwb eng Li, Mengying verfasserin aut Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. Carbon material (dpeaa)DE-He213 Co-doped (dpeaa)DE-He213 High specific surface area (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Wang, Chengyin aut Hu, Shengnan aut Wu, Huimin aut Feng, Chuanqi aut Zhang, Yanqing aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 9 vom: 26. Apr., Seite 4295-4303 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:9 day:26 month:04 pages:4295-4303 https://dx.doi.org/10.1007/s11581-019-02976-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 9 26 04 4295-4303 |
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10.1007/s11581-019-02976-9 doi (DE-627)SPR020876920 (SPR)s11581-019-02976-9-e DE-627 ger DE-627 rakwb eng Li, Mengying verfasserin aut Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. Carbon material (dpeaa)DE-He213 Co-doped (dpeaa)DE-He213 High specific surface area (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Wang, Chengyin aut Hu, Shengnan aut Wu, Huimin aut Feng, Chuanqi aut Zhang, Yanqing aut Enthalten in Ionics Berlin : Springer, 1995 25(2019), 9 vom: 26. Apr., Seite 4295-4303 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:25 year:2019 number:9 day:26 month:04 pages:4295-4303 https://dx.doi.org/10.1007/s11581-019-02976-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2019 9 26 04 4295-4303 |
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Li, Mengying @@aut@@ Wang, Chengyin @@aut@@ Hu, Shengnan @@aut@@ Wu, Huimin @@aut@@ Feng, Chuanqi @@aut@@ Zhang, Yanqing @@aut@@ |
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The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. 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Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction Carbon material (dpeaa)DE-He213 Co-doped (dpeaa)DE-He213 High specific surface area (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 |
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nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction |
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Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction |
| abstract |
Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. © Springer-Verlag GmbH Germany, part of Springer Nature 2019 |
| abstractGer |
Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. © Springer-Verlag GmbH Germany, part of Springer Nature 2019 |
| abstract_unstemmed |
Abstract Carbon, phosphorus or nitrogen-doped carbon and nitrogen, and phosphorus co-doped carbon materials were successfully synthesized. The scanning electron microscopy and transmission electron microscope indicated that the samples exhibited three-dimensional layered structure. While the X-ray diffraction and Raman results suggested that the samples were typical carbon materials with high purity, besides, the nitrogen adsorption-desorption isotherm results showed that the nitrogen, phosphorus co-doped carbon material had the highest specific surface area of 2346.2 $ m^{2} $ $ g^{−1} $ with uniform mesoporous (3.8 nm) and considerable pore volume (0.69 $ cm^{3} $ $ g^{−1} $). The cyclic voltammetry, electrochemical impedance spectra, liner sweep voltammetry, and chronoamperometry were tested in oxygen-saturated 0.1 M KOH solution. The electrochemical tests suggested that the nitrogen, phosphorus co-doped carbon material had a positive onset potential (0.92 V), half-wave potential (0.81 V), low resistance (73 Ω), and low Tafel slope (70 mV/decade) at low current region. More importantly, the oxygen reduction reaction was a 4-electron pathway with excellent methanol tolerance. © Springer-Verlag GmbH Germany, part of Springer Nature 2019 |
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| title_short |
Nitrogen, phosphorus co-doped mesoporous carbon materials as efficient catalysts for oxygen reduction reaction |
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https://dx.doi.org/10.1007/s11581-019-02976-9 |
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Wang, Chengyin Hu, Shengnan Wu, Huimin Feng, Chuanqi Zhang, Yanqing |
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2024-07-03T18:50:36.545Z |
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| score |
7.399971 |