The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C
Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were con...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
El Mendili, Yassine [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2014 |
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| Schlagwörter: |
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| Anmerkung: |
© ASM International 2014 |
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| Übergeordnetes Werk: |
Enthalten in: Journal of materials engineering and performance - New York, NY : Springer, 1992, 23(2014), 4 vom: 31. Jan., Seite 1350-1357 |
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| Übergeordnetes Werk: |
volume:23 ; year:2014 ; number:4 ; day:31 ; month:01 ; pages:1350-1357 |
| Links: |
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| DOI / URN: |
10.1007/s11665-014-0879-x |
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| Katalog-ID: |
SPR021597251 |
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| 520 | |a Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. | ||
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| 700 | 1 | |a Bardeau, Jean-François |4 aut | |
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10.1007/s11665-014-0879-x doi (DE-627)SPR021597251 (SPR)s11665-014-0879-x-e DE-627 ger DE-627 rakwb eng El Mendili, Yassine verfasserin aut The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © ASM International 2014 Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. carbon/alloy steels (dpeaa)DE-He213 corrosion testing (dpeaa)DE-He213 advanced characterization (dpeaa)DE-He213 environment (dpeaa)DE-He213 Abdelouas, Abdesselam aut Bardeau, Jean-François aut Enthalten in Journal of materials engineering and performance New York, NY : Springer, 1992 23(2014), 4 vom: 31. Jan., Seite 1350-1357 (DE-627)329975447 (DE-600)2048384-3 1544-1024 nnns volume:23 year:2014 number:4 day:31 month:01 pages:1350-1357 https://dx.doi.org/10.1007/s11665-014-0879-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 23 2014 4 31 01 1350-1357 |
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10.1007/s11665-014-0879-x doi (DE-627)SPR021597251 (SPR)s11665-014-0879-x-e DE-627 ger DE-627 rakwb eng El Mendili, Yassine verfasserin aut The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © ASM International 2014 Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. carbon/alloy steels (dpeaa)DE-He213 corrosion testing (dpeaa)DE-He213 advanced characterization (dpeaa)DE-He213 environment (dpeaa)DE-He213 Abdelouas, Abdesselam aut Bardeau, Jean-François aut Enthalten in Journal of materials engineering and performance New York, NY : Springer, 1992 23(2014), 4 vom: 31. Jan., Seite 1350-1357 (DE-627)329975447 (DE-600)2048384-3 1544-1024 nnns volume:23 year:2014 number:4 day:31 month:01 pages:1350-1357 https://dx.doi.org/10.1007/s11665-014-0879-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 23 2014 4 31 01 1350-1357 |
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10.1007/s11665-014-0879-x doi (DE-627)SPR021597251 (SPR)s11665-014-0879-x-e DE-627 ger DE-627 rakwb eng El Mendili, Yassine verfasserin aut The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © ASM International 2014 Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. carbon/alloy steels (dpeaa)DE-He213 corrosion testing (dpeaa)DE-He213 advanced characterization (dpeaa)DE-He213 environment (dpeaa)DE-He213 Abdelouas, Abdesselam aut Bardeau, Jean-François aut Enthalten in Journal of materials engineering and performance New York, NY : Springer, 1992 23(2014), 4 vom: 31. Jan., Seite 1350-1357 (DE-627)329975447 (DE-600)2048384-3 1544-1024 nnns volume:23 year:2014 number:4 day:31 month:01 pages:1350-1357 https://dx.doi.org/10.1007/s11665-014-0879-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 23 2014 4 31 01 1350-1357 |
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10.1007/s11665-014-0879-x doi (DE-627)SPR021597251 (SPR)s11665-014-0879-x-e DE-627 ger DE-627 rakwb eng El Mendili, Yassine verfasserin aut The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © ASM International 2014 Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. carbon/alloy steels (dpeaa)DE-He213 corrosion testing (dpeaa)DE-He213 advanced characterization (dpeaa)DE-He213 environment (dpeaa)DE-He213 Abdelouas, Abdesselam aut Bardeau, Jean-François aut Enthalten in Journal of materials engineering and performance New York, NY : Springer, 1992 23(2014), 4 vom: 31. Jan., Seite 1350-1357 (DE-627)329975447 (DE-600)2048384-3 1544-1024 nnns volume:23 year:2014 number:4 day:31 month:01 pages:1350-1357 https://dx.doi.org/10.1007/s11665-014-0879-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 23 2014 4 31 01 1350-1357 |
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10.1007/s11665-014-0879-x doi (DE-627)SPR021597251 (SPR)s11665-014-0879-x-e DE-627 ger DE-627 rakwb eng El Mendili, Yassine verfasserin aut The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © ASM International 2014 Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. carbon/alloy steels (dpeaa)DE-He213 corrosion testing (dpeaa)DE-He213 advanced characterization (dpeaa)DE-He213 environment (dpeaa)DE-He213 Abdelouas, Abdesselam aut Bardeau, Jean-François aut Enthalten in Journal of materials engineering and performance New York, NY : Springer, 1992 23(2014), 4 vom: 31. Jan., Seite 1350-1357 (DE-627)329975447 (DE-600)2048384-3 1544-1024 nnns volume:23 year:2014 number:4 day:31 month:01 pages:1350-1357 https://dx.doi.org/10.1007/s11665-014-0879-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 23 2014 4 31 01 1350-1357 |
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El Mendili, Yassine @@aut@@ Abdelouas, Abdesselam @@aut@@ Bardeau, Jean-François @@aut@@ |
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The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C carbon/alloy steels (dpeaa)DE-He213 corrosion testing (dpeaa)DE-He213 advanced characterization (dpeaa)DE-He213 environment (dpeaa)DE-He213 |
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corrosion behavior of carbon steel in sulfide aqueous media at 30°c |
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The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C |
| abstract |
Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. © ASM International 2014 |
| abstractGer |
Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. © ASM International 2014 |
| abstract_unstemmed |
Abstract In this paper, we studied the effect of sulfide ions on the corrosion behavior of carbon steel to simulate the geological disposal of high-level radioactive waste. In geological storage conditions, sulfidogenic environment was sustained by sulfate-reducing bacteria. Corrosion tests were conducted in systems in a controlled atmosphere of 5% $ H_{2} $/$ N_{2} $. Batch experiments were conducted at 30°C for 1 month with steel coupons immersed in $ Na_{2} $S solutions. The structural characterization of the corrosion products was investigated by scanning electron microscope/energy dispersive x-ray spectroscopy, confocal micro-Raman spectrometry, and x-ray diffraction. In the absence of sulfide ion, a magnetite ($ Fe_{3} %$ O_{4} $) corrosion product layer was formed on steel surface while in the presence of sulfide ions we observed the formation of a poorly crystallized irons sulfide at low-sulfide concentration (1 mg/L) and a solid adherent pyrrhotite layer at higher sulfide concentration (5-15 mg/L). The strong drop in steel corrosion rate with sulfide concentration was revealed and related to the formation of well-crystallized pyrrhotite. © ASM International 2014 |
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The Corrosion Behavior of Carbon Steel in Sulfide Aqueous Media at 30°C |
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https://dx.doi.org/10.1007/s11665-014-0879-x |
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Abdelouas, Abdesselam Bardeau, Jean-François |
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|
| score |
7.400386 |