Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control
Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and on...
Ausführliche Beschreibung
Autor*in: |
Uemura, Shinobu [verfasserIn] Sakata, Kenki [verfasserIn] Aono, Masashi [verfasserIn] Nakamura, Yusuke [verfasserIn] Kunitake, Masashi [verfasserIn] |
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Sprache: |
Englisch |
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2016 |
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Übergeordnetes Werk: |
Enthalten in: Frontiers of chemical engineering in China - Beijing : Higher Education Press, 2007, 10(2016), 2 vom: 23. März, Seite 294-300 |
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Übergeordnetes Werk: |
volume:10 ; year:2016 ; number:2 ; day:23 ; month:03 ; pages:294-300 |
Links: |
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DOI / URN: |
10.1007/s11705-016-1564-4 |
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Katalog-ID: |
SPR021950083 |
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520 | |a Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. | ||
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700 | 1 | |a Sakata, Kenki |e verfasserin |4 aut | |
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700 | 1 | |a Kunitake, Masashi |e verfasserin |4 aut | |
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10.1007/s11705-016-1564-4 doi (DE-627)SPR021950083 (SPR)s11705-016-1564-4-e DE-627 ger DE-627 rakwb eng 540 ASE Uemura, Shinobu verfasserin aut Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. self-assembly (dpeaa)DE-He213 scanning tunneling microscopy (dpeaa)DE-He213 electrochemistry (dpeaa)DE-He213 structural phase transition (dpeaa)DE-He213 melem (dpeaa)DE-He213 Sakata, Kenki verfasserin aut Aono, Masashi verfasserin aut Nakamura, Yusuke verfasserin aut Kunitake, Masashi verfasserin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 10(2016), 2 vom: 23. März, Seite 294-300 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:10 year:2016 number:2 day:23 month:03 pages:294-300 https://dx.doi.org/10.1007/s11705-016-1564-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 10 2016 2 23 03 294-300 |
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10.1007/s11705-016-1564-4 doi (DE-627)SPR021950083 (SPR)s11705-016-1564-4-e DE-627 ger DE-627 rakwb eng 540 ASE Uemura, Shinobu verfasserin aut Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. self-assembly (dpeaa)DE-He213 scanning tunneling microscopy (dpeaa)DE-He213 electrochemistry (dpeaa)DE-He213 structural phase transition (dpeaa)DE-He213 melem (dpeaa)DE-He213 Sakata, Kenki verfasserin aut Aono, Masashi verfasserin aut Nakamura, Yusuke verfasserin aut Kunitake, Masashi verfasserin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 10(2016), 2 vom: 23. März, Seite 294-300 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:10 year:2016 number:2 day:23 month:03 pages:294-300 https://dx.doi.org/10.1007/s11705-016-1564-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 10 2016 2 23 03 294-300 |
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10.1007/s11705-016-1564-4 doi (DE-627)SPR021950083 (SPR)s11705-016-1564-4-e DE-627 ger DE-627 rakwb eng 540 ASE Uemura, Shinobu verfasserin aut Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. self-assembly (dpeaa)DE-He213 scanning tunneling microscopy (dpeaa)DE-He213 electrochemistry (dpeaa)DE-He213 structural phase transition (dpeaa)DE-He213 melem (dpeaa)DE-He213 Sakata, Kenki verfasserin aut Aono, Masashi verfasserin aut Nakamura, Yusuke verfasserin aut Kunitake, Masashi verfasserin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 10(2016), 2 vom: 23. März, Seite 294-300 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:10 year:2016 number:2 day:23 month:03 pages:294-300 https://dx.doi.org/10.1007/s11705-016-1564-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 10 2016 2 23 03 294-300 |
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10.1007/s11705-016-1564-4 doi (DE-627)SPR021950083 (SPR)s11705-016-1564-4-e DE-627 ger DE-627 rakwb eng 540 ASE Uemura, Shinobu verfasserin aut Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. self-assembly (dpeaa)DE-He213 scanning tunneling microscopy (dpeaa)DE-He213 electrochemistry (dpeaa)DE-He213 structural phase transition (dpeaa)DE-He213 melem (dpeaa)DE-He213 Sakata, Kenki verfasserin aut Aono, Masashi verfasserin aut Nakamura, Yusuke verfasserin aut Kunitake, Masashi verfasserin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 10(2016), 2 vom: 23. März, Seite 294-300 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:10 year:2016 number:2 day:23 month:03 pages:294-300 https://dx.doi.org/10.1007/s11705-016-1564-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 10 2016 2 23 03 294-300 |
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10.1007/s11705-016-1564-4 doi (DE-627)SPR021950083 (SPR)s11705-016-1564-4-e DE-627 ger DE-627 rakwb eng 540 ASE Uemura, Shinobu verfasserin aut Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. self-assembly (dpeaa)DE-He213 scanning tunneling microscopy (dpeaa)DE-He213 electrochemistry (dpeaa)DE-He213 structural phase transition (dpeaa)DE-He213 melem (dpeaa)DE-He213 Sakata, Kenki verfasserin aut Aono, Masashi verfasserin aut Nakamura, Yusuke verfasserin aut Kunitake, Masashi verfasserin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 10(2016), 2 vom: 23. März, Seite 294-300 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:10 year:2016 number:2 day:23 month:03 pages:294-300 https://dx.doi.org/10.1007/s11705-016-1564-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 10 2016 2 23 03 294-300 |
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540 ASE Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control self-assembly (dpeaa)DE-He213 scanning tunneling microscopy (dpeaa)DE-He213 electrochemistry (dpeaa)DE-He213 structural phase transition (dpeaa)DE-He213 melem (dpeaa)DE-He213 |
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Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control |
abstract |
Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. |
abstractGer |
Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. |
abstract_unstemmed |
Abstract Two-dimensional self-assembly of melem at pH-controlled aqueous solution-Au(111) interfaces has been investigated by electrochemical scanning tunneling microscopy. In the solutions with pH>pKb1 of melem, two ordered self-assembled structures (honeycomb and close-packed structures) and one disordered fibrillar structure were observed as a function of the surface coverage of melem controlled by the electrode potential. In contrast, in the acidic solution with pH<pKb1 of melem, only the self-assembled honeycomb network was observed in a relatively wide potential range probably due to the presence of monoprotonated melem cations. Dots attributed to counteranions were frequently observed in the pores of the honeycomb network. The lack of close-packed and fibrillar structures at low pH (<pKb1) is attributed to ionic repulsion of melemium cations. |
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Two-dimensional self-assembly of melem and melemium cations at pH-controlled aqueous solution–Au(111) interfaces under electrochemical control |
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