$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $
Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO t...
Ausführliche Beschreibung
Autor*in: |
Majidian, Nasrollah [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2014 |
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Schlagwörter: |
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Anmerkung: |
© Korean Institute of Chemical Engineers, Seoul, Korea 2014 |
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Übergeordnetes Werk: |
Enthalten in: The Korean journal of chemical engineering - Seoul : Inst., 1984, 31(2014), 7 vom: 07. März, Seite 1162-1167 |
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Übergeordnetes Werk: |
volume:31 ; year:2014 ; number:7 ; day:07 ; month:03 ; pages:1162-1167 |
Links: |
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DOI / URN: |
10.1007/s11814-014-0010-x |
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Katalog-ID: |
SPR022508465 |
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245 | 1 | 0 | |a $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ |
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520 | |a Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. | ||
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700 | 1 | |a Habibi, Narges |4 aut | |
700 | 1 | |a Rezaei, Mehran |4 aut | |
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10.1007/s11814-014-0010-x doi (DE-627)SPR022508465 (SPR)s11814-014-0010-x-e DE-627 ger DE-627 rakwb eng Majidian, Nasrollah verfasserin aut $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. Nanostructured (dpeaa)DE-He213 -Al (dpeaa)DE-He213 O (dpeaa)DE-He213 Nickel Catalyst (dpeaa)DE-He213 Dry Reforming (dpeaa)DE-He213 Syngas (dpeaa)DE-He213 Habibi, Narges aut Rezaei, Mehran aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 31(2014), 7 vom: 07. März, Seite 1162-1167 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 https://dx.doi.org/10.1007/s11814-014-0010-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 31 2014 7 07 03 1162-1167 |
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10.1007/s11814-014-0010-x doi (DE-627)SPR022508465 (SPR)s11814-014-0010-x-e DE-627 ger DE-627 rakwb eng Majidian, Nasrollah verfasserin aut $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. Nanostructured (dpeaa)DE-He213 -Al (dpeaa)DE-He213 O (dpeaa)DE-He213 Nickel Catalyst (dpeaa)DE-He213 Dry Reforming (dpeaa)DE-He213 Syngas (dpeaa)DE-He213 Habibi, Narges aut Rezaei, Mehran aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 31(2014), 7 vom: 07. März, Seite 1162-1167 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 https://dx.doi.org/10.1007/s11814-014-0010-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 31 2014 7 07 03 1162-1167 |
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10.1007/s11814-014-0010-x doi (DE-627)SPR022508465 (SPR)s11814-014-0010-x-e DE-627 ger DE-627 rakwb eng Majidian, Nasrollah verfasserin aut $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. Nanostructured (dpeaa)DE-He213 -Al (dpeaa)DE-He213 O (dpeaa)DE-He213 Nickel Catalyst (dpeaa)DE-He213 Dry Reforming (dpeaa)DE-He213 Syngas (dpeaa)DE-He213 Habibi, Narges aut Rezaei, Mehran aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 31(2014), 7 vom: 07. März, Seite 1162-1167 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 https://dx.doi.org/10.1007/s11814-014-0010-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 31 2014 7 07 03 1162-1167 |
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10.1007/s11814-014-0010-x doi (DE-627)SPR022508465 (SPR)s11814-014-0010-x-e DE-627 ger DE-627 rakwb eng Majidian, Nasrollah verfasserin aut $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. Nanostructured (dpeaa)DE-He213 -Al (dpeaa)DE-He213 O (dpeaa)DE-He213 Nickel Catalyst (dpeaa)DE-He213 Dry Reforming (dpeaa)DE-He213 Syngas (dpeaa)DE-He213 Habibi, Narges aut Rezaei, Mehran aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 31(2014), 7 vom: 07. März, Seite 1162-1167 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 https://dx.doi.org/10.1007/s11814-014-0010-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 31 2014 7 07 03 1162-1167 |
allfieldsSound |
10.1007/s11814-014-0010-x doi (DE-627)SPR022508465 (SPR)s11814-014-0010-x-e DE-627 ger DE-627 rakwb eng Majidian, Nasrollah verfasserin aut $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. Nanostructured (dpeaa)DE-He213 -Al (dpeaa)DE-He213 O (dpeaa)DE-He213 Nickel Catalyst (dpeaa)DE-He213 Dry Reforming (dpeaa)DE-He213 Syngas (dpeaa)DE-He213 Habibi, Narges aut Rezaei, Mehran aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 31(2014), 7 vom: 07. März, Seite 1162-1167 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 https://dx.doi.org/10.1007/s11814-014-0010-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 31 2014 7 07 03 1162-1167 |
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Enthalten in The Korean journal of chemical engineering 31(2014), 7 vom: 07. März, Seite 1162-1167 volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 |
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Enthalten in The Korean journal of chemical engineering 31(2014), 7 vom: 07. März, Seite 1162-1167 volume:31 year:2014 number:7 day:07 month:03 pages:1162-1167 |
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Majidian, Nasrollah @@aut@@ Habibi, Narges @@aut@@ Rezaei, Mehran @@aut@@ |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR022508465</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230520003136.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">201006s2014 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s11814-014-0010-x</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR022508465</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s11814-014-0010-x-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Majidian, Nasrollah</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2014</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© Korean Institute of Chemical Engineers, Seoul, Korea 2014</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. 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Majidian, Nasrollah |
spellingShingle |
Majidian, Nasrollah misc Nanostructured misc -Al misc O misc Nickel Catalyst misc Dry Reforming misc Syngas $ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ |
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$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ Nanostructured (dpeaa)DE-He213 -Al (dpeaa)DE-He213 O (dpeaa)DE-He213 Nickel Catalyst (dpeaa)DE-He213 Dry Reforming (dpeaa)DE-He213 Syngas (dpeaa)DE-He213 |
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misc Nanostructured misc -Al misc O misc Nickel Catalyst misc Dry Reforming misc Syngas |
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$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ |
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(DE-627)SPR022508465 (SPR)s11814-014-0010-x-e |
title_full |
$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ |
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Majidian, Nasrollah |
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Majidian, Nasrollah Habibi, Narges Rezaei, Mehran |
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10.1007/s11814-014-0010-x |
title_sort |
$ ch_{4} $ reforming with $ co_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ al_{2} %$ o_{3} $ |
title_auth |
$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ |
abstract |
Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. © Korean Institute of Chemical Engineers, Seoul, Korea 2014 |
abstractGer |
Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. © Korean Institute of Chemical Engineers, Seoul, Korea 2014 |
abstract_unstemmed |
Abstract Nanostructured γ-$ Al_{2} %$ O_{3} $ with high surface area and mesoporous structure was synthesized by sol-gel method and employed as catalyst support for nickel catalysts in methane reforming with carbon dioxide. The prepared samples were characterized by XRD, BET, TPR, TPH, SEM and TPO techniques. The BET analysis showed a high surface area of $ 204m^{2} %$ g^{−1} $ and a narrow pore-size distribution centered at a diameter of 5.5 nm for catalyst support. The results revealed that an increase in nickel loading from 5 to 15 wt% decreased the surface area of catalyst from 182 to 160 $ m^{2} %$ g^{−1} $. In addition, the catalytic results showed an increase in methane conversion with increase in nickel content. TPO analysis revealed that the coke deposition increased with increasing in nickel loading, and the catalyst with 15 wt% of nickel showed the highest degree of carbon formation. SEM and TPH analyses confirmed the formation of whisker type carbon over the spent catalysts. Increasing $ CO_{2} $/$ CH_{4} $ ratio increased the methane conversion. The BET analysis of spent catalysts indicated that the mesoporous structure of catalysts still remained after reaction. © Korean Institute of Chemical Engineers, Seoul, Korea 2014 |
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container_issue |
7 |
title_short |
$ CH_{4} $ reforming with $ CO_{2} $ for syngas production over nickel catalysts supported on mesoporous nanostructured γ-$ Al_{2} %$ O_{3} $ |
url |
https://dx.doi.org/10.1007/s11814-014-0010-x |
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author2 |
Habibi, Narges Rezaei, Mehran |
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doi_str |
10.1007/s11814-014-0010-x |
up_date |
2024-07-04T03:17:51.187Z |
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|
score |
7.397979 |