MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes

Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e.,...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Park, Hongyeol [verfasserIn] Yeom, Dae Hoon Kim, Jaegyeong Lee, Jung Kyoo

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2014

Schlagwörter:	Lithium-ion Battery Anode Manganese Oxide Carbon Composite Transition Metal Oxide

Anmerkung:	© Korean Institute of Chemical Engineers, Seoul, Korea 2014

Übergeordnetes Werk:	Enthalten in: The Korean journal of chemical engineering - Seoul : Inst., 1984, 32(2014), 1 vom: 29. Dez., Seite 178-183
Übergeordnetes Werk:	volume:32 ; year:2014 ; number:1 ; day:29 ; month:12 ; pages:178-183

Links:	Volltext

DOI / URN:	10.1007/s11814-014-0265-2

Katalog-ID:	SPR022509534

Internformat


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245	1	0	\|a MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
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520			\|a Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications.
650		4	\|a Lithium-ion Battery \|7 (dpeaa)DE-He213
650		4	\|a Anode \|7 (dpeaa)DE-He213
650		4	\|a Manganese Oxide \|7 (dpeaa)DE-He213
650		4	\|a Carbon Composite \|7 (dpeaa)DE-He213
650		4	\|a Transition Metal Oxide \|7 (dpeaa)DE-He213
700	1		\|a Yeom, Dae Hoon \|4 aut
700	1		\|a Kim, Jaegyeong \|4 aut
700	1		\|a Lee, Jung Kyoo \|4 aut
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912			\|a GBV_ILN_138
912			\|a GBV_ILN_150
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912			\|a GBV_ILN_152
912			\|a GBV_ILN_161
912			\|a GBV_ILN_170
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912			\|a GBV_ILN_187
912			\|a GBV_ILN_213
912			\|a GBV_ILN_224
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912			\|a GBV_ILN_250
912			\|a GBV_ILN_281
912			\|a GBV_ILN_285
912			\|a GBV_ILN_293
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_636
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2006
912			\|a GBV_ILN_2007
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2009
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
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912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2031
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2037
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912			\|a GBV_ILN_2044
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912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2057
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912			\|a GBV_ILN_2065
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912			\|a GBV_ILN_2070
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912			\|a GBV_ILN_2088
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matchkey_str	article:19757220:2014----::ncaoopstpeaeboeohdohraratofrihefra
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allfields	10.1007/s11814-014-0265-2 doi (DE-627)SPR022509534 (SPR)s11814-014-0265-2-e DE-627 ger DE-627 rakwb eng Park, Hongyeol verfasserin aut MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. Lithium-ion Battery (dpeaa)DE-He213 Anode (dpeaa)DE-He213 Manganese Oxide (dpeaa)DE-He213 Carbon Composite (dpeaa)DE-He213 Transition Metal Oxide (dpeaa)DE-He213 Yeom, Dae Hoon aut Kim, Jaegyeong aut Lee, Jung Kyoo aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 32(2014), 1 vom: 29. Dez., Seite 178-183 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:32 year:2014 number:1 day:29 month:12 pages:178-183 https://dx.doi.org/10.1007/s11814-014-0265-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2014 1 29 12 178-183
spelling	10.1007/s11814-014-0265-2 doi (DE-627)SPR022509534 (SPR)s11814-014-0265-2-e DE-627 ger DE-627 rakwb eng Park, Hongyeol verfasserin aut MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. Lithium-ion Battery (dpeaa)DE-He213 Anode (dpeaa)DE-He213 Manganese Oxide (dpeaa)DE-He213 Carbon Composite (dpeaa)DE-He213 Transition Metal Oxide (dpeaa)DE-He213 Yeom, Dae Hoon aut Kim, Jaegyeong aut Lee, Jung Kyoo aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 32(2014), 1 vom: 29. Dez., Seite 178-183 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:32 year:2014 number:1 day:29 month:12 pages:178-183 https://dx.doi.org/10.1007/s11814-014-0265-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2014 1 29 12 178-183
allfields_unstemmed	10.1007/s11814-014-0265-2 doi (DE-627)SPR022509534 (SPR)s11814-014-0265-2-e DE-627 ger DE-627 rakwb eng Park, Hongyeol verfasserin aut MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. Lithium-ion Battery (dpeaa)DE-He213 Anode (dpeaa)DE-He213 Manganese Oxide (dpeaa)DE-He213 Carbon Composite (dpeaa)DE-He213 Transition Metal Oxide (dpeaa)DE-He213 Yeom, Dae Hoon aut Kim, Jaegyeong aut Lee, Jung Kyoo aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 32(2014), 1 vom: 29. Dez., Seite 178-183 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:32 year:2014 number:1 day:29 month:12 pages:178-183 https://dx.doi.org/10.1007/s11814-014-0265-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2014 1 29 12 178-183
allfieldsGer	10.1007/s11814-014-0265-2 doi (DE-627)SPR022509534 (SPR)s11814-014-0265-2-e DE-627 ger DE-627 rakwb eng Park, Hongyeol verfasserin aut MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. Lithium-ion Battery (dpeaa)DE-He213 Anode (dpeaa)DE-He213 Manganese Oxide (dpeaa)DE-He213 Carbon Composite (dpeaa)DE-He213 Transition Metal Oxide (dpeaa)DE-He213 Yeom, Dae Hoon aut Kim, Jaegyeong aut Lee, Jung Kyoo aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 32(2014), 1 vom: 29. Dez., Seite 178-183 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:32 year:2014 number:1 day:29 month:12 pages:178-183 https://dx.doi.org/10.1007/s11814-014-0265-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2014 1 29 12 178-183
allfieldsSound	10.1007/s11814-014-0265-2 doi (DE-627)SPR022509534 (SPR)s11814-014-0265-2-e DE-627 ger DE-627 rakwb eng Park, Hongyeol verfasserin aut MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Korean Institute of Chemical Engineers, Seoul, Korea 2014 Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. Lithium-ion Battery (dpeaa)DE-He213 Anode (dpeaa)DE-He213 Manganese Oxide (dpeaa)DE-He213 Carbon Composite (dpeaa)DE-He213 Transition Metal Oxide (dpeaa)DE-He213 Yeom, Dae Hoon aut Kim, Jaegyeong aut Lee, Jung Kyoo aut Enthalten in The Korean journal of chemical engineering Seoul : Inst., 1984 32(2014), 1 vom: 29. Dez., Seite 178-183 (DE-627)391337246 (DE-600)2152566-3 1975-7220 nnns volume:32 year:2014 number:1 day:29 month:12 pages:178-183 https://dx.doi.org/10.1007/s11814-014-0265-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2014 1 29 12 178-183
language	English
source	Enthalten in The Korean journal of chemical engineering 32(2014), 1 vom: 29. Dez., Seite 178-183 volume:32 year:2014 number:1 day:29 month:12 pages:178-183
sourceStr	Enthalten in The Korean journal of chemical engineering 32(2014), 1 vom: 29. Dez., Seite 178-183 volume:32 year:2014 number:1 day:29 month:12 pages:178-183
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Lithium-ion Battery Anode Manganese Oxide Carbon Composite Transition Metal Oxide
isfreeaccess_bool	false
container_title	The Korean journal of chemical engineering
authorswithroles_txt_mv	Park, Hongyeol @@aut@@ Yeom, Dae Hoon @@aut@@ Kim, Jaegyeong @@aut@@ Lee, Jung Kyoo @@aut@@
publishDateDaySort_date	2014-12-29T00:00:00Z
hierarchy_top_id	391337246
id	SPR022509534
language_de	englisch
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author	Park, Hongyeol
spellingShingle	Park, Hongyeol misc Lithium-ion Battery misc Anode misc Manganese Oxide misc Carbon Composite misc Transition Metal Oxide MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
authorStr	Park, Hongyeol
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topic_title	MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes Lithium-ion Battery (dpeaa)DE-He213 Anode (dpeaa)DE-He213 Manganese Oxide (dpeaa)DE-He213 Carbon Composite (dpeaa)DE-He213 Transition Metal Oxide (dpeaa)DE-He213
topic	misc Lithium-ion Battery misc Anode misc Manganese Oxide misc Carbon Composite misc Transition Metal Oxide
topic_unstemmed	misc Lithium-ion Battery misc Anode misc Manganese Oxide misc Carbon Composite misc Transition Metal Oxide
topic_browse	misc Lithium-ion Battery misc Anode misc Manganese Oxide misc Carbon Composite misc Transition Metal Oxide
format_facet	Elektronische Aufsätze Aufsätze Elektronische Ressource
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title	MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
ctrlnum	(DE-627)SPR022509534 (SPR)s11814-014-0265-2-e
title_full	MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
author_sort	Park, Hongyeol
journal	The Korean journal of chemical engineering
journalStr	The Korean journal of chemical engineering
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container_start_page	178
author_browse	Park, Hongyeol Yeom, Dae Hoon Kim, Jaegyeong Lee, Jung Kyoo
container_volume	32
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author-letter	Park, Hongyeol
doi_str_mv	10.1007/s11814-014-0265-2
title_sort	mno/c nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
title_auth	MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
abstract	Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. © Korean Institute of Chemical Engineers, Seoul, Korea 2014
abstractGer	Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. © Korean Institute of Chemical Engineers, Seoul, Korea 2014
abstract_unstemmed	Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications. © Korean Institute of Chemical Engineers, Seoul, Korea 2014
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title_short	MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes
url	https://dx.doi.org/10.1007/s11814-014-0265-2
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author2	Yeom, Dae Hoon Kim, Jaegyeong Lee, Jung Kyoo
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doi_str	10.1007/s11814-014-0265-2
up_date	2024-07-04T03:18:04.243Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR022509534</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230520003138.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">201006s2014 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s11814-014-0265-2</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR022509534</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s11814-014-0265-2-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Park, Hongyeol</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">MnO/C nanocomposite prepared by one-pot hydrothermal reaction for high performance lithium-ion battery anodes</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2014</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© Korean Institute of Chemical Engineers, Seoul, Korea 2014</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract Among various candidates to replace the low capacity graphitic carbon anode in current lithium ion batteries (LIBs), manganese oxides possess the advantages of high lithium storage capacity, low cost, high intrinsic density, environmental friendliness and low lithium storage voltage, i.e., 0.5 V $ Li^{+} $/Li. Manganese oxides, however, have to be incorporated with conducting and porous matrix due to poor electrical conductivity and large volume expansions associated with conversion reaction upon cycling. In this study, a facile one-pot route was attempted for the synthesis of MnO/C nanocomposite for which $ Mn_{3} %$ O_{4} $ nanoparticles were grown in aqueous medium followed by carbon gel formation in a one-pot reactor. Thus obtained $ Mn_{3} %$ O_{4} $/C carbon gel was transformed into MnO/C nanocomposite by thermal annealing in an Ar flow. The MnO nanoparticles (60wt%) of 20–50 nm in diameter were well dispersed throughout the MnO/C composite. The MnO/C composite delivered reversible capacity of 541mAh $ g^{−1} $ with an excellent cycling stability over 100 cycles, while parent $ Mn_{3} %$ O_{4} $ lost most of its capacity in 10 cycles. The MnO/C composite also exhibited much higher rate capability than a commercial graphite anode. Hence, the MnO/C composite based on low cost materials and facile synthetic process could be an attractive candidate for large-scale energy storage applications.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Lithium-ion Battery</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Anode</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Manganese Oxide</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Carbon Composite</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Transition Metal Oxide</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Yeom, Dae Hoon</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Kim, Jaegyeong</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Lee, Jung Kyoo</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">The Korean journal of chemical engineering</subfield><subfield code="d">Seoul : Inst., 1984</subfield><subfield code="g">32(2014), 1 vom: 29. 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