Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California
Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's ex...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Krudysz, Margaret A. [verfasserIn] Dutton, Steven J. [verfasserIn] Brinkman, Gregory L. [verfasserIn] Hannigan, Michael P. [verfasserIn] Fine, Philip M. [verfasserIn] Sioutas, Constantinos [verfasserIn] Froines, John R. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2009 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Air quality, atmosphere and health - Dordrecht : Springer Netherlands, 2008, 2(2009), 2 vom: 09. Apr., Seite 69-88 |
|---|---|
| Übergeordnetes Werk: |
volume:2 ; year:2009 ; number:2 ; day:09 ; month:04 ; pages:69-88 |
| Links: |
|---|
| DOI / URN: |
10.1007/s11869-009-0035-1 |
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| Katalog-ID: |
SPR02342110X |
|---|
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| 100 | 1 | |a Krudysz, Margaret A. |e verfasserin |4 aut | |
| 245 | 1 | 0 | |a Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California |
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| 520 | |a Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. | ||
| 650 | 4 | |a Atmospheric aerosols |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Chemical characterization |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Coefficient of divergence |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Intra-community |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Particulate matter |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Organic speciation |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Spatial variability |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Urban emissions |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Dutton, Steven J. |e verfasserin |4 aut | |
| 700 | 1 | |a Brinkman, Gregory L. |e verfasserin |4 aut | |
| 700 | 1 | |a Hannigan, Michael P. |e verfasserin |4 aut | |
| 700 | 1 | |a Fine, Philip M. |e verfasserin |4 aut | |
| 700 | 1 | |a Sioutas, Constantinos |e verfasserin |4 aut | |
| 700 | 1 | |a Froines, John R. |e verfasserin |4 aut | |
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10.1007/s11869-009-0035-1 doi (DE-627)SPR02342110X (SPR)s11869-009-0035-1-e DE-627 ger DE-627 rakwb eng 690 ASE 43.11 bkl 44.13 bkl Krudysz, Margaret A. verfasserin aut Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. Atmospheric aerosols (dpeaa)DE-He213 Chemical characterization (dpeaa)DE-He213 Coefficient of divergence (dpeaa)DE-He213 Intra-community (dpeaa)DE-He213 Particulate matter (dpeaa)DE-He213 Organic speciation (dpeaa)DE-He213 Spatial variability (dpeaa)DE-He213 Urban emissions (dpeaa)DE-He213 Dutton, Steven J. verfasserin aut Brinkman, Gregory L. verfasserin aut Hannigan, Michael P. verfasserin aut Fine, Philip M. verfasserin aut Sioutas, Constantinos verfasserin aut Froines, John R. verfasserin aut Enthalten in Air quality, atmosphere and health Dordrecht : Springer Netherlands, 2008 2(2009), 2 vom: 09. Apr., Seite 69-88 (DE-627)565516515 (DE-600)2424084-9 1873-9326 nnns volume:2 year:2009 number:2 day:09 month:04 pages:69-88 https://dx.doi.org/10.1007/s11869-009-0035-1 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4392 GBV_ILN_4393 GBV_ILN_4700 43.11 ASE 44.13 ASE AR 2 2009 2 09 04 69-88 |
| spelling |
10.1007/s11869-009-0035-1 doi (DE-627)SPR02342110X (SPR)s11869-009-0035-1-e DE-627 ger DE-627 rakwb eng 690 ASE 43.11 bkl 44.13 bkl Krudysz, Margaret A. verfasserin aut Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. Atmospheric aerosols (dpeaa)DE-He213 Chemical characterization (dpeaa)DE-He213 Coefficient of divergence (dpeaa)DE-He213 Intra-community (dpeaa)DE-He213 Particulate matter (dpeaa)DE-He213 Organic speciation (dpeaa)DE-He213 Spatial variability (dpeaa)DE-He213 Urban emissions (dpeaa)DE-He213 Dutton, Steven J. verfasserin aut Brinkman, Gregory L. verfasserin aut Hannigan, Michael P. verfasserin aut Fine, Philip M. verfasserin aut Sioutas, Constantinos verfasserin aut Froines, John R. verfasserin aut Enthalten in Air quality, atmosphere and health Dordrecht : Springer Netherlands, 2008 2(2009), 2 vom: 09. Apr., Seite 69-88 (DE-627)565516515 (DE-600)2424084-9 1873-9326 nnns volume:2 year:2009 number:2 day:09 month:04 pages:69-88 https://dx.doi.org/10.1007/s11869-009-0035-1 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4392 GBV_ILN_4393 GBV_ILN_4700 43.11 ASE 44.13 ASE AR 2 2009 2 09 04 69-88 |
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10.1007/s11869-009-0035-1 doi (DE-627)SPR02342110X (SPR)s11869-009-0035-1-e DE-627 ger DE-627 rakwb eng 690 ASE 43.11 bkl 44.13 bkl Krudysz, Margaret A. verfasserin aut Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. Atmospheric aerosols (dpeaa)DE-He213 Chemical characterization (dpeaa)DE-He213 Coefficient of divergence (dpeaa)DE-He213 Intra-community (dpeaa)DE-He213 Particulate matter (dpeaa)DE-He213 Organic speciation (dpeaa)DE-He213 Spatial variability (dpeaa)DE-He213 Urban emissions (dpeaa)DE-He213 Dutton, Steven J. verfasserin aut Brinkman, Gregory L. verfasserin aut Hannigan, Michael P. verfasserin aut Fine, Philip M. verfasserin aut Sioutas, Constantinos verfasserin aut Froines, John R. verfasserin aut Enthalten in Air quality, atmosphere and health Dordrecht : Springer Netherlands, 2008 2(2009), 2 vom: 09. Apr., Seite 69-88 (DE-627)565516515 (DE-600)2424084-9 1873-9326 nnns volume:2 year:2009 number:2 day:09 month:04 pages:69-88 https://dx.doi.org/10.1007/s11869-009-0035-1 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4392 GBV_ILN_4393 GBV_ILN_4700 43.11 ASE 44.13 ASE AR 2 2009 2 09 04 69-88 |
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10.1007/s11869-009-0035-1 doi (DE-627)SPR02342110X (SPR)s11869-009-0035-1-e DE-627 ger DE-627 rakwb eng 690 ASE 43.11 bkl 44.13 bkl Krudysz, Margaret A. verfasserin aut Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. Atmospheric aerosols (dpeaa)DE-He213 Chemical characterization (dpeaa)DE-He213 Coefficient of divergence (dpeaa)DE-He213 Intra-community (dpeaa)DE-He213 Particulate matter (dpeaa)DE-He213 Organic speciation (dpeaa)DE-He213 Spatial variability (dpeaa)DE-He213 Urban emissions (dpeaa)DE-He213 Dutton, Steven J. verfasserin aut Brinkman, Gregory L. verfasserin aut Hannigan, Michael P. verfasserin aut Fine, Philip M. verfasserin aut Sioutas, Constantinos verfasserin aut Froines, John R. verfasserin aut Enthalten in Air quality, atmosphere and health Dordrecht : Springer Netherlands, 2008 2(2009), 2 vom: 09. Apr., Seite 69-88 (DE-627)565516515 (DE-600)2424084-9 1873-9326 nnns volume:2 year:2009 number:2 day:09 month:04 pages:69-88 https://dx.doi.org/10.1007/s11869-009-0035-1 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4392 GBV_ILN_4393 GBV_ILN_4700 43.11 ASE 44.13 ASE AR 2 2009 2 09 04 69-88 |
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10.1007/s11869-009-0035-1 doi (DE-627)SPR02342110X (SPR)s11869-009-0035-1-e DE-627 ger DE-627 rakwb eng 690 ASE 43.11 bkl 44.13 bkl Krudysz, Margaret A. verfasserin aut Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California 2009 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. Atmospheric aerosols (dpeaa)DE-He213 Chemical characterization (dpeaa)DE-He213 Coefficient of divergence (dpeaa)DE-He213 Intra-community (dpeaa)DE-He213 Particulate matter (dpeaa)DE-He213 Organic speciation (dpeaa)DE-He213 Spatial variability (dpeaa)DE-He213 Urban emissions (dpeaa)DE-He213 Dutton, Steven J. verfasserin aut Brinkman, Gregory L. verfasserin aut Hannigan, Michael P. verfasserin aut Fine, Philip M. verfasserin aut Sioutas, Constantinos verfasserin aut Froines, John R. verfasserin aut Enthalten in Air quality, atmosphere and health Dordrecht : Springer Netherlands, 2008 2(2009), 2 vom: 09. Apr., Seite 69-88 (DE-627)565516515 (DE-600)2424084-9 1873-9326 nnns volume:2 year:2009 number:2 day:09 month:04 pages:69-88 https://dx.doi.org/10.1007/s11869-009-0035-1 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4392 GBV_ILN_4393 GBV_ILN_4700 43.11 ASE 44.13 ASE AR 2 2009 2 09 04 69-88 |
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Enthalten in Air quality, atmosphere and health 2(2009), 2 vom: 09. Apr., Seite 69-88 volume:2 year:2009 number:2 day:09 month:04 pages:69-88 |
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Enthalten in Air quality, atmosphere and health 2(2009), 2 vom: 09. Apr., Seite 69-88 volume:2 year:2009 number:2 day:09 month:04 pages:69-88 |
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Atmospheric aerosols Chemical characterization Coefficient of divergence Intra-community Particulate matter Organic speciation Spatial variability Urban emissions |
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Krudysz, Margaret A. @@aut@@ Dutton, Steven J. @@aut@@ Brinkman, Gregory L. @@aut@@ Hannigan, Michael P. @@aut@@ Fine, Philip M. @@aut@@ Sioutas, Constantinos @@aut@@ Froines, John R. @@aut@@ |
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Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. 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Krudysz, Margaret A. |
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Krudysz, Margaret A. ddc 690 bkl 43.11 bkl 44.13 misc Atmospheric aerosols misc Chemical characterization misc Coefficient of divergence misc Intra-community misc Particulate matter misc Organic speciation misc Spatial variability misc Urban emissions Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California |
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690 ASE 43.11 bkl 44.13 bkl Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California Atmospheric aerosols (dpeaa)DE-He213 Chemical characterization (dpeaa)DE-He213 Coefficient of divergence (dpeaa)DE-He213 Intra-community (dpeaa)DE-He213 Particulate matter (dpeaa)DE-He213 Organic speciation (dpeaa)DE-He213 Spatial variability (dpeaa)DE-He213 Urban emissions (dpeaa)DE-He213 |
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ddc 690 bkl 43.11 bkl 44.13 misc Atmospheric aerosols misc Chemical characterization misc Coefficient of divergence misc Intra-community misc Particulate matter misc Organic speciation misc Spatial variability misc Urban emissions |
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ddc 690 bkl 43.11 bkl 44.13 misc Atmospheric aerosols misc Chemical characterization misc Coefficient of divergence misc Intra-community misc Particulate matter misc Organic speciation misc Spatial variability misc Urban emissions |
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Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California |
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Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California |
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Krudysz, Margaret A. |
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Air quality, atmosphere and health |
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Krudysz, Margaret A. Dutton, Steven J. Brinkman, Gregory L. Hannigan, Michael P. Fine, Philip M. Sioutas, Constantinos Froines, John R. |
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Krudysz, Margaret A. |
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10.1007/s11869-009-0035-1 |
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intra-community spatial variation of size-fractionated organic compounds in long beach, california |
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Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California |
| abstract |
Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. |
| abstractGer |
Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. |
| abstract_unstemmed |
Abstract Quantification of the size distributions of organic molecular markers can provide information about the origin of the carbonaceous particulate matter (PM). Organic molecular marker spatial variability studies provide data that are vital to an accurate determination of a population's exposure to PM from various sources. We have investigated the intra-community spatial variation of size-segregated PM [0–0.25 μm (ultrafine), 0.25-2.5 μm (accumulation), and 2.5-10 μm (coarse)) ] in a southern California community. The highest concentrations of individual organic compounds were found in the ultrafine fraction, followed by the accumulation and coarse size fractions. Correlations between the three size fractions were weak between compounds in the coarse and corresponding ultrafine and accumulation particles, implying that the coarse PM organic compounds were emitted by different sources than those that emit ultrafine and accumulation mode PM. Evidence of the incomplete combustion of gasoline was found in the ultrafine and accumulation size fractions, while possible diesel emissions were traced to ultrafine particles. Coefficients of divergence and coefficients of variation were investigated to determine the spatial and temporal variability of individual organic compounds. Spatial divergence in organic compounds was comparatively high, but it did not differ appreciably between size fractions or between compound classes. Elemental carbon and tracer compounds, which originate from a few sources, showed higher spatial divergence than organic carbon whose numerous sources can be local and regional. Spatial and temporal variability were not different from each other for this data set and, therefore, it is not possible to determine whether variability in concentrations between sampling sites or the length of the sampling campaign is more important for health effects studies. |
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Intra-community spatial variation of size-fractionated organic compounds in Long Beach, California |
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| score |
7.401248 |