Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles

Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant beca...
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Autor*in:	Zhu, Xiyue [verfasserIn] Rong, Hongpan Zhang, Xiaobin Di, Qiumei Shang, Huishan Bai, Bing Liu, Jiajia Liu, Jia Xu, Meng Chen, Wenxing Zhang, Jiatao

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	compressive surface strain atomic-layer Cu O precise thickness-control catalytic activity

Anmerkung:	© Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019

Übergeordnetes Werk:	Enthalten in: Nano research - [S.l.] : Tsinghua Press, 2008, 12(2019), 5 vom: 28. März, Seite 1187-1192
Übergeordnetes Werk:	volume:12 ; year:2019 ; number:5 ; day:28 ; month:03 ; pages:1187-1192

Links:	Volltext

DOI / URN:	10.1007/s12274-019-2380-1

Katalog-ID:	SPR024732966

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520			\|a Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications.
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700	1		\|a Liu, Jia \|4 aut
700	1		\|a Xu, Meng \|4 aut
700	1		\|a Chen, Wenxing \|4 aut
700	1		\|a Zhang, Jiatao \|4 aut
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912			\|a GBV_ILN_110
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912			\|a GBV_ILN_138
912			\|a GBV_ILN_150
912			\|a GBV_ILN_151
912			\|a GBV_ILN_152
912			\|a GBV_ILN_161
912			\|a GBV_ILN_170
912			\|a GBV_ILN_171
912			\|a GBV_ILN_187
912			\|a GBV_ILN_213
912			\|a GBV_ILN_224
912			\|a GBV_ILN_230
912			\|a GBV_ILN_250
912			\|a GBV_ILN_281
912			\|a GBV_ILN_285
912			\|a GBV_ILN_293
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_636
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
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912			\|a GBV_ILN_2005
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912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2031
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2037
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2039
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2057
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
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Indexfelder

author_variant	x z xz h r hr x z xz q d qd h s hs b b bb j l jl j l jl m x mx w c wc j z jz
matchkey_str	article:19980000:2019----::opesvsraetandtmcaec_on
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publishDate	2019
allfields	10.1007/s12274-019-2380-1 doi (DE-627)SPR024732966 (SPR)s12274-019-2380-1-e DE-627 ger DE-627 rakwb eng Zhu, Xiyue verfasserin aut Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. compressive surface strain (dpeaa)DE-He213 atomic-layer Cu (dpeaa)DE-He213 O (dpeaa)DE-He213 precise thickness-control (dpeaa)DE-He213 catalytic activity (dpeaa)DE-He213 Rong, Hongpan aut Zhang, Xiaobin aut Di, Qiumei aut Shang, Huishan aut Bai, Bing aut Liu, Jiajia aut Liu, Jia aut Xu, Meng aut Chen, Wenxing aut Zhang, Jiatao aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 12(2019), 5 vom: 28. März, Seite 1187-1192 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192 https://dx.doi.org/10.1007/s12274-019-2380-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2019 5 28 03 1187-1192
spelling	10.1007/s12274-019-2380-1 doi (DE-627)SPR024732966 (SPR)s12274-019-2380-1-e DE-627 ger DE-627 rakwb eng Zhu, Xiyue verfasserin aut Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. compressive surface strain (dpeaa)DE-He213 atomic-layer Cu (dpeaa)DE-He213 O (dpeaa)DE-He213 precise thickness-control (dpeaa)DE-He213 catalytic activity (dpeaa)DE-He213 Rong, Hongpan aut Zhang, Xiaobin aut Di, Qiumei aut Shang, Huishan aut Bai, Bing aut Liu, Jiajia aut Liu, Jia aut Xu, Meng aut Chen, Wenxing aut Zhang, Jiatao aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 12(2019), 5 vom: 28. März, Seite 1187-1192 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192 https://dx.doi.org/10.1007/s12274-019-2380-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2019 5 28 03 1187-1192
allfields_unstemmed	10.1007/s12274-019-2380-1 doi (DE-627)SPR024732966 (SPR)s12274-019-2380-1-e DE-627 ger DE-627 rakwb eng Zhu, Xiyue verfasserin aut Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. compressive surface strain (dpeaa)DE-He213 atomic-layer Cu (dpeaa)DE-He213 O (dpeaa)DE-He213 precise thickness-control (dpeaa)DE-He213 catalytic activity (dpeaa)DE-He213 Rong, Hongpan aut Zhang, Xiaobin aut Di, Qiumei aut Shang, Huishan aut Bai, Bing aut Liu, Jiajia aut Liu, Jia aut Xu, Meng aut Chen, Wenxing aut Zhang, Jiatao aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 12(2019), 5 vom: 28. März, Seite 1187-1192 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192 https://dx.doi.org/10.1007/s12274-019-2380-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2019 5 28 03 1187-1192
allfieldsGer	10.1007/s12274-019-2380-1 doi (DE-627)SPR024732966 (SPR)s12274-019-2380-1-e DE-627 ger DE-627 rakwb eng Zhu, Xiyue verfasserin aut Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. compressive surface strain (dpeaa)DE-He213 atomic-layer Cu (dpeaa)DE-He213 O (dpeaa)DE-He213 precise thickness-control (dpeaa)DE-He213 catalytic activity (dpeaa)DE-He213 Rong, Hongpan aut Zhang, Xiaobin aut Di, Qiumei aut Shang, Huishan aut Bai, Bing aut Liu, Jiajia aut Liu, Jia aut Xu, Meng aut Chen, Wenxing aut Zhang, Jiatao aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 12(2019), 5 vom: 28. März, Seite 1187-1192 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192 https://dx.doi.org/10.1007/s12274-019-2380-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2019 5 28 03 1187-1192
allfieldsSound	10.1007/s12274-019-2380-1 doi (DE-627)SPR024732966 (SPR)s12274-019-2380-1-e DE-627 ger DE-627 rakwb eng Zhu, Xiyue verfasserin aut Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019 Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. compressive surface strain (dpeaa)DE-He213 atomic-layer Cu (dpeaa)DE-He213 O (dpeaa)DE-He213 precise thickness-control (dpeaa)DE-He213 catalytic activity (dpeaa)DE-He213 Rong, Hongpan aut Zhang, Xiaobin aut Di, Qiumei aut Shang, Huishan aut Bai, Bing aut Liu, Jiajia aut Liu, Jia aut Xu, Meng aut Chen, Wenxing aut Zhang, Jiatao aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 12(2019), 5 vom: 28. März, Seite 1187-1192 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192 https://dx.doi.org/10.1007/s12274-019-2380-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2019 5 28 03 1187-1192
language	English
source	Enthalten in Nano research 12(2019), 5 vom: 28. März, Seite 1187-1192 volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192
sourceStr	Enthalten in Nano research 12(2019), 5 vom: 28. März, Seite 1187-1192 volume:12 year:2019 number:5 day:28 month:03 pages:1187-1192
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	compressive surface strain atomic-layer Cu O precise thickness-control catalytic activity
isfreeaccess_bool	false
container_title	Nano research
authorswithroles_txt_mv	Zhu, Xiyue @@aut@@ Rong, Hongpan @@aut@@ Zhang, Xiaobin @@aut@@ Di, Qiumei @@aut@@ Shang, Huishan @@aut@@ Bai, Bing @@aut@@ Liu, Jiajia @@aut@@ Liu, Jia @@aut@@ Xu, Meng @@aut@@ Chen, Wenxing @@aut@@ Zhang, Jiatao @@aut@@
publishDateDaySort_date	2019-03-28T00:00:00Z
hierarchy_top_id	57375361X
id	SPR024732966
language_de	englisch
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author	Zhu, Xiyue
spellingShingle	Zhu, Xiyue misc compressive surface strain misc atomic-layer Cu misc O misc precise thickness-control misc catalytic activity Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles
authorStr	Zhu, Xiyue
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topic_title	Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles compressive surface strain (dpeaa)DE-He213 atomic-layer Cu (dpeaa)DE-He213 O (dpeaa)DE-He213 precise thickness-control (dpeaa)DE-He213 catalytic activity (dpeaa)DE-He213
topic	misc compressive surface strain misc atomic-layer Cu misc O misc precise thickness-control misc catalytic activity
topic_unstemmed	misc compressive surface strain misc atomic-layer Cu misc O misc precise thickness-control misc catalytic activity
topic_browse	misc compressive surface strain misc atomic-layer Cu misc O misc precise thickness-control misc catalytic activity
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title	Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles
ctrlnum	(DE-627)SPR024732966 (SPR)s12274-019-2380-1-e
title_full	Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles
author_sort	Zhu, Xiyue
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container_start_page	1187
author_browse	Zhu, Xiyue Rong, Hongpan Zhang, Xiaobin Di, Qiumei Shang, Huishan Bai, Bing Liu, Jiajia Liu, Jia Xu, Meng Chen, Wenxing Zhang, Jiatao
container_volume	12
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author-letter	Zhu, Xiyue
doi_str_mv	10.1007/s12274-019-2380-1
title_sort	compressive surface strained atomic-layer $ cu_{2} $o on cuag nanoparticles
title_auth	Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles
abstract	Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019
abstractGer	Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019
abstract_unstemmed	Abstract Control of surface structure at the atomic level can effectively tune catalytic properties of nanomaterials. Tuning surface strain is an effective strategy for enhancing catalytic activity; however, the correlation studies between the surface strain with catalytic performance are scant because such mechanistic studies require the precise control of surface strain on catalysts. In this work, a simple strategy of precisely tuning compressive surface strain of atomic-layer $ Cu_{2} $O on CuAg (AL-$ Cu_{2} $O/Cu@Ag) nanoparticles (NPs) is demonstrated. The AL-Cu2O is synthesized by structure evolution of Cu@Ag core-shell nanoparticles, and the precise thickness-control of AL-$ Cu_{2} $O is achieved by tuning the molar ratio of Cu/Ag of the starting material. Aberration-corrected high-resolution transmission electron microscopy (AC-HRTEM) and EELS elemental mapping characterization showed that the compressive surface strain of AL-$ Cu_{2} $O along the [111] and [200] directions can be precisely tuned from 6.5% to 1.6% and 6.6% to 4.7%, respectively, by changing the number of AL-$ Cu_{2} $O layer from 3 to 6. The as-prepared AL-$ Cu_{2} $O/Cu@Ag NPs exhibited excellent catalytic property in the synthesis of azobenzene from aniline, in which the strained 4-layers $ Cu_{2} $O (4.5% along the [111] direction, 6.1% along the [200] direction) exhibits the best catalytic performance. This work may be beneficial for the design and surface engineering of catalysts toward specific applications. © Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019
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container_issue	5
title_short	Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles
url	https://dx.doi.org/10.1007/s12274-019-2380-1
remote_bool	true
author2	Rong, Hongpan Zhang, Xiaobin Di, Qiumei Shang, Huishan Bai, Bing Liu, Jiajia Liu, Jia Xu, Meng Chen, Wenxing Zhang, Jiatao
author2Str	Rong, Hongpan Zhang, Xiaobin Di, Qiumei Shang, Huishan Bai, Bing Liu, Jiajia Liu, Jia Xu, Meng Chen, Wenxing Zhang, Jiatao
ppnlink	57375361X
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doi_str	10.1007/s12274-019-2380-1
up_date	2024-07-04T02:10:33.502Z
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Compressive surface strained atomic-layer $ Cu_{2} $O on CuAg nanoparticles

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