Recent development in colloidal quantum dots photovoltaics

Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only ha...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Peng, Li [verfasserIn] Tang, Jiang Zhu, Mingqiang

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2012

Schlagwörter:	lead sulfide colloidal quantum dots (CQDs) solar cells multiple exciton generation (MEG) atomic ligands

Anmerkung:	© Higher Education Press and Springer-Verlag Berlin Heidelberg 2012

Übergeordnetes Werk:	Enthalten in: Frontiers of optoelectronics in China - [Beijing] : Higher Education Press, 2008, 5(2012), 4 vom: 03. Nov., Seite 358-370
Übergeordnetes Werk:	volume:5 ; year:2012 ; number:4 ; day:03 ; month:11 ; pages:358-370

Links:	Volltext

DOI / URN:	10.1007/s12200-012-0285-7

Katalog-ID:	SPR025209345

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allfields	10.1007/s12200-012-0285-7 doi (DE-627)SPR025209345 (SPR)s12200-012-0285-7-e DE-627 ger DE-627 rakwb eng Peng, Li verfasserin aut Recent development in colloidal quantum dots photovoltaics 2012 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012 Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. lead sulfide (dpeaa)DE-He213 colloidal quantum dots (CQDs) (dpeaa)DE-He213 solar cells (dpeaa)DE-He213 multiple exciton generation (MEG) (dpeaa)DE-He213 atomic ligands (dpeaa)DE-He213 Tang, Jiang aut Zhu, Mingqiang aut Enthalten in Frontiers of optoelectronics in China [Beijing] : Higher Education Press, 2008 5(2012), 4 vom: 03. Nov., Seite 358-370 (DE-627)587886420 (DE-600)2468689-X 1674-4594 nnns volume:5 year:2012 number:4 day:03 month:11 pages:358-370 https://dx.doi.org/10.1007/s12200-012-0285-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2059 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 AR 5 2012 4 03 11 358-370
spelling	10.1007/s12200-012-0285-7 doi (DE-627)SPR025209345 (SPR)s12200-012-0285-7-e DE-627 ger DE-627 rakwb eng Peng, Li verfasserin aut Recent development in colloidal quantum dots photovoltaics 2012 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012 Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. lead sulfide (dpeaa)DE-He213 colloidal quantum dots (CQDs) (dpeaa)DE-He213 solar cells (dpeaa)DE-He213 multiple exciton generation (MEG) (dpeaa)DE-He213 atomic ligands (dpeaa)DE-He213 Tang, Jiang aut Zhu, Mingqiang aut Enthalten in Frontiers of optoelectronics in China [Beijing] : Higher Education Press, 2008 5(2012), 4 vom: 03. Nov., Seite 358-370 (DE-627)587886420 (DE-600)2468689-X 1674-4594 nnns volume:5 year:2012 number:4 day:03 month:11 pages:358-370 https://dx.doi.org/10.1007/s12200-012-0285-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2059 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 AR 5 2012 4 03 11 358-370
allfields_unstemmed	10.1007/s12200-012-0285-7 doi (DE-627)SPR025209345 (SPR)s12200-012-0285-7-e DE-627 ger DE-627 rakwb eng Peng, Li verfasserin aut Recent development in colloidal quantum dots photovoltaics 2012 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012 Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. lead sulfide (dpeaa)DE-He213 colloidal quantum dots (CQDs) (dpeaa)DE-He213 solar cells (dpeaa)DE-He213 multiple exciton generation (MEG) (dpeaa)DE-He213 atomic ligands (dpeaa)DE-He213 Tang, Jiang aut Zhu, Mingqiang aut Enthalten in Frontiers of optoelectronics in China [Beijing] : Higher Education Press, 2008 5(2012), 4 vom: 03. Nov., Seite 358-370 (DE-627)587886420 (DE-600)2468689-X 1674-4594 nnns volume:5 year:2012 number:4 day:03 month:11 pages:358-370 https://dx.doi.org/10.1007/s12200-012-0285-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2059 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 AR 5 2012 4 03 11 358-370
allfieldsGer	10.1007/s12200-012-0285-7 doi (DE-627)SPR025209345 (SPR)s12200-012-0285-7-e DE-627 ger DE-627 rakwb eng Peng, Li verfasserin aut Recent development in colloidal quantum dots photovoltaics 2012 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012 Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. lead sulfide (dpeaa)DE-He213 colloidal quantum dots (CQDs) (dpeaa)DE-He213 solar cells (dpeaa)DE-He213 multiple exciton generation (MEG) (dpeaa)DE-He213 atomic ligands (dpeaa)DE-He213 Tang, Jiang aut Zhu, Mingqiang aut Enthalten in Frontiers of optoelectronics in China [Beijing] : Higher Education Press, 2008 5(2012), 4 vom: 03. Nov., Seite 358-370 (DE-627)587886420 (DE-600)2468689-X 1674-4594 nnns volume:5 year:2012 number:4 day:03 month:11 pages:358-370 https://dx.doi.org/10.1007/s12200-012-0285-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2059 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 AR 5 2012 4 03 11 358-370
allfieldsSound	10.1007/s12200-012-0285-7 doi (DE-627)SPR025209345 (SPR)s12200-012-0285-7-e DE-627 ger DE-627 rakwb eng Peng, Li verfasserin aut Recent development in colloidal quantum dots photovoltaics 2012 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012 Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. lead sulfide (dpeaa)DE-He213 colloidal quantum dots (CQDs) (dpeaa)DE-He213 solar cells (dpeaa)DE-He213 multiple exciton generation (MEG) (dpeaa)DE-He213 atomic ligands (dpeaa)DE-He213 Tang, Jiang aut Zhu, Mingqiang aut Enthalten in Frontiers of optoelectronics in China [Beijing] : Higher Education Press, 2008 5(2012), 4 vom: 03. Nov., Seite 358-370 (DE-627)587886420 (DE-600)2468689-X 1674-4594 nnns volume:5 year:2012 number:4 day:03 month:11 pages:358-370 https://dx.doi.org/10.1007/s12200-012-0285-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2059 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 AR 5 2012 4 03 11 358-370
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source	Enthalten in Frontiers of optoelectronics in China 5(2012), 4 vom: 03. Nov., Seite 358-370 volume:5 year:2012 number:4 day:03 month:11 pages:358-370
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spellingShingle	Peng, Li misc lead sulfide misc colloidal quantum dots (CQDs) misc solar cells misc multiple exciton generation (MEG) misc atomic ligands Recent development in colloidal quantum dots photovoltaics
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title_sort	recent development in colloidal quantum dots photovoltaics
title_auth	Recent development in colloidal quantum dots photovoltaics
abstract	Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012
abstractGer	Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012
abstract_unstemmed	Abstract The increasing demand for sustainable and green energy supply spurred the surging research on high-efficiency, low-cost photovoltaics. Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development. © Higher Education Press and Springer-Verlag Berlin Heidelberg 2012
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Colloidal quantum dot solar cell (CQDSC) is a new type of photovoltaic device using lead chalcogenide quantum dot film as absorber materials. It not only has a potential to break the 33% Shockley-Queisser efficiency limit for single junction solar cell, but also possesses low-temperature, high-throughput solution processing. Since its first report in 2005, CQDSCs experienced rapid progress achieving a certified 7% efficiency in 2012, an averaged 1% efficiency gain per year. In this paper, we reviewed the research progress reported in the last two years. We started with background introduction and motivation for CQDSC research. We then briefly introduced the evolution history of CQDSC development as well as multiple exciton generation effect. We further focused on the latest efforts in improving the light absorption and carrier collection efficiency, including the bulk-heterojunction structure, quantum funnel concept, band alignment optimization and quantum dot passivation. Afterwards, we discussed the tandem solar cell and device stability, and concluded this article with a perspective. Hopefully, this review paper covers the major achievement in this field in year 2011–2012 and provides readers with a concise and clear understanding of recent CQDSC development.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">lead sulfide</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">colloidal quantum dots (CQDs)</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">solar cells</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">multiple exciton generation (MEG)</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">atomic ligands</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Tang, Jiang</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Zhu, Mingqiang</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Frontiers of optoelectronics in China</subfield><subfield code="d">[Beijing] : Higher Education Press, 2008</subfield><subfield code="g">5(2012), 4 vom: 03. 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