Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts
Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Taran, O. P. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2011 |
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| Schlagwörter: |
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| Anmerkung: |
© Pleiades Publishing, Ltd. 2011 |
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| Übergeordnetes Werk: |
Enthalten in: Catalysis in industry - Moscow : MAIK Nauka/Interperiodica Publ., 2009, 3(2011), 2 vom: Juni, Seite 161-169 |
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| Übergeordnetes Werk: |
volume:3 ; year:2011 ; number:2 ; month:06 ; pages:161-169 |
| Links: |
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| DOI / URN: |
10.1134/S2070050411020152 |
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| Katalog-ID: |
SPR026311321 |
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| 100 | 1 | |a Taran, O. P. |e verfasserin |4 aut | |
| 245 | 1 | 0 | |a Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts |
| 264 | 1 | |c 2011 | |
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| 520 | |a Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. | ||
| 650 | 4 | |a wet peroxide oxidation |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a hydrogen peroxide |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a carbon materials. |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Polyanskaya, E. M. |4 aut | |
| 700 | 1 | |a Ogorodnikova, O. L. |4 aut | |
| 700 | 1 | |a Descorme, C. |4 aut | |
| 700 | 1 | |a Besson, M. |4 aut | |
| 700 | 1 | |a Parmon, V. N. |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Catalysis in industry |d Moscow : MAIK Nauka/Interperiodica Publ., 2009 |g 3(2011), 2 vom: Juni, Seite 161-169 |w (DE-627)606030867 |w (DE-600)2508015-5 |x 2070-0555 |7 nnns |
| 773 | 1 | 8 | |g volume:3 |g year:2011 |g number:2 |g month:06 |g pages:161-169 |
| 856 | 4 | 0 | |u https://dx.doi.org/10.1134/S2070050411020152 |z lizenzpflichtig |3 Volltext |
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10.1134/S2070050411020152 doi (DE-627)SPR026311321 (SPR)S2070050411020152-e DE-627 ger DE-627 rakwb eng Taran, O. P. verfasserin aut Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2011 Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. wet peroxide oxidation (dpeaa)DE-He213 hydrogen peroxide (dpeaa)DE-He213 carbon materials. (dpeaa)DE-He213 Polyanskaya, E. M. aut Ogorodnikova, O. L. aut Descorme, C. aut Besson, M. aut Parmon, V. N. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 3(2011), 2 vom: Juni, Seite 161-169 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:3 year:2011 number:2 month:06 pages:161-169 https://dx.doi.org/10.1134/S2070050411020152 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 3 2011 2 06 161-169 |
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10.1134/S2070050411020152 doi (DE-627)SPR026311321 (SPR)S2070050411020152-e DE-627 ger DE-627 rakwb eng Taran, O. P. verfasserin aut Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2011 Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. wet peroxide oxidation (dpeaa)DE-He213 hydrogen peroxide (dpeaa)DE-He213 carbon materials. (dpeaa)DE-He213 Polyanskaya, E. M. aut Ogorodnikova, O. L. aut Descorme, C. aut Besson, M. aut Parmon, V. N. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 3(2011), 2 vom: Juni, Seite 161-169 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:3 year:2011 number:2 month:06 pages:161-169 https://dx.doi.org/10.1134/S2070050411020152 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 3 2011 2 06 161-169 |
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10.1134/S2070050411020152 doi (DE-627)SPR026311321 (SPR)S2070050411020152-e DE-627 ger DE-627 rakwb eng Taran, O. P. verfasserin aut Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2011 Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. wet peroxide oxidation (dpeaa)DE-He213 hydrogen peroxide (dpeaa)DE-He213 carbon materials. (dpeaa)DE-He213 Polyanskaya, E. M. aut Ogorodnikova, O. L. aut Descorme, C. aut Besson, M. aut Parmon, V. N. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 3(2011), 2 vom: Juni, Seite 161-169 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:3 year:2011 number:2 month:06 pages:161-169 https://dx.doi.org/10.1134/S2070050411020152 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 3 2011 2 06 161-169 |
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10.1134/S2070050411020152 doi (DE-627)SPR026311321 (SPR)S2070050411020152-e DE-627 ger DE-627 rakwb eng Taran, O. P. verfasserin aut Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2011 Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. wet peroxide oxidation (dpeaa)DE-He213 hydrogen peroxide (dpeaa)DE-He213 carbon materials. (dpeaa)DE-He213 Polyanskaya, E. M. aut Ogorodnikova, O. L. aut Descorme, C. aut Besson, M. aut Parmon, V. N. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 3(2011), 2 vom: Juni, Seite 161-169 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:3 year:2011 number:2 month:06 pages:161-169 https://dx.doi.org/10.1134/S2070050411020152 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 3 2011 2 06 161-169 |
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10.1134/S2070050411020152 doi (DE-627)SPR026311321 (SPR)S2070050411020152-e DE-627 ger DE-627 rakwb eng Taran, O. P. verfasserin aut Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2011 Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. wet peroxide oxidation (dpeaa)DE-He213 hydrogen peroxide (dpeaa)DE-He213 carbon materials. (dpeaa)DE-He213 Polyanskaya, E. M. aut Ogorodnikova, O. L. aut Descorme, C. aut Besson, M. aut Parmon, V. N. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 3(2011), 2 vom: Juni, Seite 161-169 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:3 year:2011 number:2 month:06 pages:161-169 https://dx.doi.org/10.1134/S2070050411020152 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 3 2011 2 06 161-169 |
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Taran, O. P. @@aut@@ Polyanskaya, E. M. @@aut@@ Ogorodnikova, O. L. @@aut@@ Descorme, C. @@aut@@ Besson, M. @@aut@@ Parmon, V. N. @@aut@@ |
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| author |
Taran, O. P. |
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Taran, O. P. misc wet peroxide oxidation misc hydrogen peroxide misc carbon materials. Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts |
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Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts wet peroxide oxidation (dpeaa)DE-He213 hydrogen peroxide (dpeaa)DE-He213 carbon materials. (dpeaa)DE-He213 |
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misc wet peroxide oxidation misc hydrogen peroxide misc carbon materials. |
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misc wet peroxide oxidation misc hydrogen peroxide misc carbon materials. |
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misc wet peroxide oxidation misc hydrogen peroxide misc carbon materials. |
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Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts |
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Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts |
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Taran, O. P. |
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Catalysis in industry |
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Taran, O. P. Polyanskaya, E. M. Ogorodnikova, O. L. Descorme, C. Besson, M. Parmon, V. N. |
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Elektronische Aufsätze |
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Taran, O. P. |
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10.1134/S2070050411020152 |
| title_sort |
sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. ii: wet peroxide oxidation over oxidized carbon catalysts |
| title_auth |
Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts |
| abstract |
Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. © Pleiades Publishing, Ltd. 2011 |
| abstractGer |
Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. © Pleiades Publishing, Ltd. 2011 |
| abstract_unstemmed |
Abstract The influence of the surface chemical composition of carbon catalysts prepared by oxidative treatment on the basis of the Sibunit-4 carbon material of the Sibunit family on their catalytic properties in the liquid-phase oxidation of formic acid by hydrogen peroxide was studied for the first time. Pure carbon samples were found to be active in the destruction of hydrogen peroxide and the oxidation of an organic substrate, and their activity decreased with an increase in the number of carboxyl and lactone groups on the surface of a carbon catalyst. Nevertheless, the rates of such processes on carbon catalysts are lower than in the presence of even small amounts of homogeneous $ Fe^{3+} $. It was shown that carbon samples accelerate or (to the contrary) inhibit the $ Fe^{3+} $-catalyzed peroxide oxidation of an organic substance, depending on the quantitative ratio of surface carboxyl and lactone groups and $ Fe^{3+} $ ions in the reaction solution. Possible acceleration and inhibition mechanisms for peroxide oxidation on carbon catalysts are discussed. The established influence of the surface chemical properties of carbon catalysts must be taken into account in the development of catalysts and processes for the oxidative purification of industrial wastewater. © Pleiades Publishing, Ltd. 2011 |
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Sibunit-based catalytic materials for the deep oxidation of organic ecotoxicants in aqueous solutions. II: Wet peroxide oxidation over oxidized carbon catalysts |
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Polyanskaya, E. M. Ogorodnikova, O. L. Descorme, C. Besson, M. Parmon, V. N. |
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Polyanskaya, E. M. Ogorodnikova, O. L. Descorme, C. Besson, M. Parmon, V. N. |
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| score |
7.4013977 |