Liquid-phase synthesis of methanol using industrial copper-zinc catalyst

Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in...
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Autor*in:	Bykov, A. V. [verfasserIn] Rubin, M. A. Sul’man, M. G. Sul’man, E. M.

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2014

Schlagwörter:	liquid-phase synthesis of methanol industrial copper-zinc catalyst

Anmerkung:	© Pleiades Publishing, Ltd. 2014

Übergeordnetes Werk:	Enthalten in: Catalysis in industry - Moscow : MAIK Nauka/Interperiodica Publ., 2009, 6(2014), 2 vom: Apr., Seite 143-149
Übergeordnetes Werk:	volume:6 ; year:2014 ; number:2 ; month:04 ; pages:143-149

Links:	Volltext

DOI / URN:	10.1134/S2070050414020020

Katalog-ID:	SPR026312751

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allfields	10.1134/S2070050414020020 doi (DE-627)SPR026312751 (SPR)S2070050414020020-e DE-627 ger DE-627 rakwb eng Bykov, A. V. verfasserin aut Liquid-phase synthesis of methanol using industrial copper-zinc catalyst 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2014 Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. liquid-phase synthesis of methanol (dpeaa)DE-He213 industrial copper-zinc catalyst (dpeaa)DE-He213 Rubin, M. A. aut Sul’man, M. G. aut Sul’man, E. M. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 6(2014), 2 vom: Apr., Seite 143-149 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:6 year:2014 number:2 month:04 pages:143-149 https://dx.doi.org/10.1134/S2070050414020020 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 6 2014 2 04 143-149
spelling	10.1134/S2070050414020020 doi (DE-627)SPR026312751 (SPR)S2070050414020020-e DE-627 ger DE-627 rakwb eng Bykov, A. V. verfasserin aut Liquid-phase synthesis of methanol using industrial copper-zinc catalyst 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2014 Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. liquid-phase synthesis of methanol (dpeaa)DE-He213 industrial copper-zinc catalyst (dpeaa)DE-He213 Rubin, M. A. aut Sul’man, M. G. aut Sul’man, E. M. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 6(2014), 2 vom: Apr., Seite 143-149 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:6 year:2014 number:2 month:04 pages:143-149 https://dx.doi.org/10.1134/S2070050414020020 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 6 2014 2 04 143-149
allfields_unstemmed	10.1134/S2070050414020020 doi (DE-627)SPR026312751 (SPR)S2070050414020020-e DE-627 ger DE-627 rakwb eng Bykov, A. V. verfasserin aut Liquid-phase synthesis of methanol using industrial copper-zinc catalyst 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2014 Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. liquid-phase synthesis of methanol (dpeaa)DE-He213 industrial copper-zinc catalyst (dpeaa)DE-He213 Rubin, M. A. aut Sul’man, M. G. aut Sul’man, E. M. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 6(2014), 2 vom: Apr., Seite 143-149 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:6 year:2014 number:2 month:04 pages:143-149 https://dx.doi.org/10.1134/S2070050414020020 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 6 2014 2 04 143-149
allfieldsGer	10.1134/S2070050414020020 doi (DE-627)SPR026312751 (SPR)S2070050414020020-e DE-627 ger DE-627 rakwb eng Bykov, A. V. verfasserin aut Liquid-phase synthesis of methanol using industrial copper-zinc catalyst 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2014 Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. liquid-phase synthesis of methanol (dpeaa)DE-He213 industrial copper-zinc catalyst (dpeaa)DE-He213 Rubin, M. A. aut Sul’man, M. G. aut Sul’man, E. M. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 6(2014), 2 vom: Apr., Seite 143-149 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:6 year:2014 number:2 month:04 pages:143-149 https://dx.doi.org/10.1134/S2070050414020020 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 6 2014 2 04 143-149
allfieldsSound	10.1134/S2070050414020020 doi (DE-627)SPR026312751 (SPR)S2070050414020020-e DE-627 ger DE-627 rakwb eng Bykov, A. V. verfasserin aut Liquid-phase synthesis of methanol using industrial copper-zinc catalyst 2014 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2014 Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. liquid-phase synthesis of methanol (dpeaa)DE-He213 industrial copper-zinc catalyst (dpeaa)DE-He213 Rubin, M. A. aut Sul’man, M. G. aut Sul’man, E. M. aut Enthalten in Catalysis in industry Moscow : MAIK Nauka/Interperiodica Publ., 2009 6(2014), 2 vom: Apr., Seite 143-149 (DE-627)606030867 (DE-600)2508015-5 2070-0555 nnns volume:6 year:2014 number:2 month:04 pages:143-149 https://dx.doi.org/10.1134/S2070050414020020 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 6 2014 2 04 143-149
language	English
source	Enthalten in Catalysis in industry 6(2014), 2 vom: Apr., Seite 143-149 volume:6 year:2014 number:2 month:04 pages:143-149
sourceStr	Enthalten in Catalysis in industry 6(2014), 2 vom: Apr., Seite 143-149 volume:6 year:2014 number:2 month:04 pages:143-149
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	liquid-phase synthesis of methanol industrial copper-zinc catalyst
isfreeaccess_bool	false
container_title	Catalysis in industry
authorswithroles_txt_mv	Bykov, A. V. @@aut@@ Rubin, M. A. @@aut@@ Sul’man, M. G. @@aut@@ Sul’man, E. M. @@aut@@
publishDateDaySort_date	2014-04-01T00:00:00Z
hierarchy_top_id	606030867
id	SPR026312751
language_de	englisch
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author	Bykov, A. V.
spellingShingle	Bykov, A. V. misc liquid-phase synthesis of methanol misc industrial copper-zinc catalyst Liquid-phase synthesis of methanol using industrial copper-zinc catalyst
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topic_title	Liquid-phase synthesis of methanol using industrial copper-zinc catalyst liquid-phase synthesis of methanol (dpeaa)DE-He213 industrial copper-zinc catalyst (dpeaa)DE-He213
topic	misc liquid-phase synthesis of methanol misc industrial copper-zinc catalyst
topic_unstemmed	misc liquid-phase synthesis of methanol misc industrial copper-zinc catalyst
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title	Liquid-phase synthesis of methanol using industrial copper-zinc catalyst
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title_full	Liquid-phase synthesis of methanol using industrial copper-zinc catalyst
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author_browse	Bykov, A. V. Rubin, M. A. Sul’man, M. G. Sul’man, E. M.
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doi_str_mv	10.1134/S2070050414020020
title_sort	liquid-phase synthesis of methanol using industrial copper-zinc catalyst
title_auth	Liquid-phase synthesis of methanol using industrial copper-zinc catalyst
abstract	Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. © Pleiades Publishing, Ltd. 2014
abstractGer	Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. © Pleiades Publishing, Ltd. 2014
abstract_unstemmed	Abstract The industrial copper-zinc catalyst MEGAMAX®-phase synthesis of methanol was tested under the conditions of a liquid-phase process while varying the pressure (0.5–7.0 MPa) and the gas mixture flow rate (40–400 $ mL_{N} $/min). The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. The results from this study indicate that the MEGAMAX® can be used in the liquid-phase synthesis of methanol. © Pleiades Publishing, Ltd. 2014
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title_short	Liquid-phase synthesis of methanol using industrial copper-zinc catalyst
url	https://dx.doi.org/10.1134/S2070050414020020
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author2	Rubin, M. A. Sul’man, M. G. Sul’man, E. M.
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doi_str	10.1134/S2070050414020020
up_date	2024-07-03T20:11:28.348Z
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The catalyst was shown to have high activity and selectivity in the synthesis of methanol. The best result (730 g(methanol)/kg(cat) $ h^{−1} $ and selectivity 99.2%) was obtained under reaction conditions of 2.0 MPa, 240°C, $ H_{2} $: CO: $ CO_{2} $: $ N_{2} $ = 70.5: 17.9: 6.5: 5.1, and reaction time 3 h. The concentration of methane by-product increased at gas mixture pressures over 3.0 MPa, lowering the selectivity of the process with respect to methanol. Trace amounts of ethane and water were found in addition to methane. Dimethyl ether, a typical by-product of methanol synthesis, was missing from the vapor-gas mixture over the range of pressures. 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Liquid-phase synthesis of methanol using industrial copper-zinc catalyst

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