Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin
Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is c...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Ni, Ping [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2016 |
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| Schlagwörter: |
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| Anmerkung: |
© Springer-Verlag Berlin Heidelberg 2016 |
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| Übergeordnetes Werk: |
Enthalten in: Environmental earth sciences - Berlin : Springer, 2009, 75(2016), 4 vom: 19. Feb. |
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| Übergeordnetes Werk: |
volume:75 ; year:2016 ; number:4 ; day:19 ; month:02 |
| Links: |
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| DOI / URN: |
10.1007/s12665-016-5294-1 |
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SPR026726548 |
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| 245 | 1 | 0 | |a Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin |
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| 520 | |a Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. | ||
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| 650 | 4 | |a Aquifer |7 (dpeaa)DE-He213 | |
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| 700 | 1 | |a Cao, Yongsheng |4 aut | |
| 700 | 1 | |a Jia, Yongfeng |4 aut | |
| 700 | 1 | |a Jiang, Yuxiao |4 aut | |
| 700 | 1 | |a Zhang, Di |4 aut | |
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10.1007/s12665-016-5294-1 doi (DE-627)SPR026726548 (SPR)s12665-016-5294-1-e DE-627 ger DE-627 rakwb eng Ni, Ping verfasserin aut Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. As (dpeaa)DE-He213 Aquifer (dpeaa)DE-He213 Hydraulic conductivity (dpeaa)DE-He213 Partition coefficient (dpeaa)DE-He213 Water–rock interaction (dpeaa)DE-He213 Guo, Huaming aut Cao, Yongsheng aut Jia, Yongfeng aut Jiang, Yuxiao aut Zhang, Di aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 75(2016), 4 vom: 19. Feb. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:75 year:2016 number:4 day:19 month:02 https://dx.doi.org/10.1007/s12665-016-5294-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 75 2016 4 19 02 |
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10.1007/s12665-016-5294-1 doi (DE-627)SPR026726548 (SPR)s12665-016-5294-1-e DE-627 ger DE-627 rakwb eng Ni, Ping verfasserin aut Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. As (dpeaa)DE-He213 Aquifer (dpeaa)DE-He213 Hydraulic conductivity (dpeaa)DE-He213 Partition coefficient (dpeaa)DE-He213 Water–rock interaction (dpeaa)DE-He213 Guo, Huaming aut Cao, Yongsheng aut Jia, Yongfeng aut Jiang, Yuxiao aut Zhang, Di aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 75(2016), 4 vom: 19. Feb. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:75 year:2016 number:4 day:19 month:02 https://dx.doi.org/10.1007/s12665-016-5294-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 75 2016 4 19 02 |
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10.1007/s12665-016-5294-1 doi (DE-627)SPR026726548 (SPR)s12665-016-5294-1-e DE-627 ger DE-627 rakwb eng Ni, Ping verfasserin aut Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. As (dpeaa)DE-He213 Aquifer (dpeaa)DE-He213 Hydraulic conductivity (dpeaa)DE-He213 Partition coefficient (dpeaa)DE-He213 Water–rock interaction (dpeaa)DE-He213 Guo, Huaming aut Cao, Yongsheng aut Jia, Yongfeng aut Jiang, Yuxiao aut Zhang, Di aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 75(2016), 4 vom: 19. Feb. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:75 year:2016 number:4 day:19 month:02 https://dx.doi.org/10.1007/s12665-016-5294-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 75 2016 4 19 02 |
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10.1007/s12665-016-5294-1 doi (DE-627)SPR026726548 (SPR)s12665-016-5294-1-e DE-627 ger DE-627 rakwb eng Ni, Ping verfasserin aut Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. As (dpeaa)DE-He213 Aquifer (dpeaa)DE-He213 Hydraulic conductivity (dpeaa)DE-He213 Partition coefficient (dpeaa)DE-He213 Water–rock interaction (dpeaa)DE-He213 Guo, Huaming aut Cao, Yongsheng aut Jia, Yongfeng aut Jiang, Yuxiao aut Zhang, Di aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 75(2016), 4 vom: 19. Feb. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:75 year:2016 number:4 day:19 month:02 https://dx.doi.org/10.1007/s12665-016-5294-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 75 2016 4 19 02 |
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10.1007/s12665-016-5294-1 doi (DE-627)SPR026726548 (SPR)s12665-016-5294-1-e DE-627 ger DE-627 rakwb eng Ni, Ping verfasserin aut Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin 2016 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag Berlin Heidelberg 2016 Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. As (dpeaa)DE-He213 Aquifer (dpeaa)DE-He213 Hydraulic conductivity (dpeaa)DE-He213 Partition coefficient (dpeaa)DE-He213 Water–rock interaction (dpeaa)DE-He213 Guo, Huaming aut Cao, Yongsheng aut Jia, Yongfeng aut Jiang, Yuxiao aut Zhang, Di aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 75(2016), 4 vom: 19. Feb. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:75 year:2016 number:4 day:19 month:02 https://dx.doi.org/10.1007/s12665-016-5294-1 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 75 2016 4 19 02 |
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However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. 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Ni, Ping |
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Ni, Ping misc As misc Aquifer misc Hydraulic conductivity misc Partition coefficient misc Water–rock interaction Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin |
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Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin As (dpeaa)DE-He213 Aquifer (dpeaa)DE-He213 Hydraulic conductivity (dpeaa)DE-He213 Partition coefficient (dpeaa)DE-He213 Water–rock interaction (dpeaa)DE-He213 |
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aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the hetao basin |
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Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin |
| abstract |
Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. © Springer-Verlag Berlin Heidelberg 2016 |
| abstractGer |
Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. © Springer-Verlag Berlin Heidelberg 2016 |
| abstract_unstemmed |
Abstract The consumption of groundwater containing high arsenic concentrations has caused serious public health problems in the Hetao Basin in Inner Mongolia. However, the relationship between As contents of aquifer sediments and in groundwater at the same depth under different redox conditions is currently poorly understood. In order to determine this relationship in the Hetao Basin, four multilevel wells were set up to monitor As and other physiochemical parameters in groundwater at different depths in the aquifer. Sediment samples were also collected at equivalent depths to groundwater sampling intervals during the drilling of boreholes. Results showed that groundwater As concentrations ranged between 2.26 and 583 μg $ L^{−1} $. In suboxic shallow groundwater (depths <14 m) with higher Eh values, As concentrations were generally lower than those in the reducing deep groundwater (depths >14 m) with relatively lower Eh values. The As contents of sediments had a negative correlation with the grain size of sediments, showing the high affinity of fine grained sediments to As. Positive relationships were observed between dissolved As concentrations and contents of extractable As (including S1: weakly bound As, S2: strongly bound As, and F3: Fe/Mn oxide bound As) in aquifer sediments for a set of depth-matched samples in reducing and suboxic environments. The relationships showed 263 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in reducing environment, and 9.4 µg $ L^{−1} $ dissolved As per 1 mg $ kg^{−1} $ S2-extracted As in suboxic environment. In the reducing environment, As tended to be partitioned into the liquid phase, where S2-As showed a better correlation with dissolved As than S1-As. In the suboxic environment, As tended to be fixed in the solid phase, where S1-As of aquifer sediments was closely related to concentrations of dissolved As in groundwater. © Springer-Verlag Berlin Heidelberg 2016 |
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Aqueous geochemistry and its influence on the partitioning of arsenic between aquifer sediments and groundwater: a case study in the northwest of the Hetao Basin |
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https://dx.doi.org/10.1007/s12665-016-5294-1 |
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Guo, Huaming Cao, Yongsheng Jia, Yongfeng Jiang, Yuxiao Zhang, Di |
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2024-07-03T22:24:42.668Z |
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| score |
7.3998337 |