Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry
Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigatin...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Yi, Yi [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017 |
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| Schlagwörter: |
Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) |
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| Anmerkung: |
© Springer-Verlag GmbH Germany, part of Springer Nature 2017 |
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| Übergeordnetes Werk: |
Enthalten in: Environmental earth sciences - Berlin : Springer, 2009, 76(2017), 24 vom: 16. Dez. |
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| Übergeordnetes Werk: |
volume:76 ; year:2017 ; number:24 ; day:16 ; month:12 |
| Links: |
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| DOI / URN: |
10.1007/s12665-017-7161-0 |
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SPR026738163 |
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| 520 | |a Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigating the toxicity of naphthenic acids, although other compounds may also contribute to the toxicity of oil sands process-affected water (OSPW). Here, we present a case study showing a systematic approach for profiling the organic composition of OSPW and environmental water samples by concentrating and separating dissolved organics through complementary liquid–liquid extractions followed by positive- or negative-ion mode ultrahigh resolution mass detection. Our comparative investigation shows clear differences in the composition of dissolved organics (homologues particularly) not only between OSPW samples and environmental water samples, but also differences among oil sands operators. Sulfur-containing compounds (especially the $ SO_{n} $classes) appear to have great potential to be used for evaluating the impact of OSPW, while our understanding of oxygen-only containing compounds should not be limited to $ O_{2} $ (i.e., classic naphthenic acids), but rather can be broadened to include many other compound classes (for instance $ O_{n} $, n = 1–9). Systematic profiling of water samples should be more widely implemented for monitoring the origin and transport of organics in aquatic ecosystems of the oil sands development region, northeastern Alberta, Canada. | ||
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| 650 | 4 | |a Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Oil sands |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Alberta |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Han, Jun |4 aut | |
| 700 | 1 | |a Jean Birks, S. |4 aut | |
| 700 | 1 | |a Borchers, Christoph H. |4 aut | |
| 700 | 1 | |a Gibson, John J. |4 aut | |
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10.1007/s12665-017-7161-0 doi (DE-627)SPR026738163 (SPR)s12665-017-7161-0-e DE-627 ger DE-627 rakwb eng Yi, Yi verfasserin (orcid)0000-0002-1403-9841 aut Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2017 Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigating the toxicity of naphthenic acids, although other compounds may also contribute to the toxicity of oil sands process-affected water (OSPW). Here, we present a case study showing a systematic approach for profiling the organic composition of OSPW and environmental water samples by concentrating and separating dissolved organics through complementary liquid–liquid extractions followed by positive- or negative-ion mode ultrahigh resolution mass detection. Our comparative investigation shows clear differences in the composition of dissolved organics (homologues particularly) not only between OSPW samples and environmental water samples, but also differences among oil sands operators. Sulfur-containing compounds (especially the $ SO_{n} $classes) appear to have great potential to be used for evaluating the impact of OSPW, while our understanding of oxygen-only containing compounds should not be limited to $ O_{2} $ (i.e., classic naphthenic acids), but rather can be broadened to include many other compound classes (for instance $ O_{n} $, n = 1–9). Systematic profiling of water samples should be more widely implemented for monitoring the origin and transport of organics in aquatic ecosystems of the oil sands development region, northeastern Alberta, Canada. Environmental forensics (dpeaa)DE-He213 Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) (dpeaa)DE-He213 Oil sands (dpeaa)DE-He213 Alberta (dpeaa)DE-He213 Han, Jun aut Jean Birks, S. aut Borchers, Christoph H. aut Gibson, John J. aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 76(2017), 24 vom: 16. Dez. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:76 year:2017 number:24 day:16 month:12 https://dx.doi.org/10.1007/s12665-017-7161-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 76 2017 24 16 12 |
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10.1007/s12665-017-7161-0 doi (DE-627)SPR026738163 (SPR)s12665-017-7161-0-e DE-627 ger DE-627 rakwb eng Yi, Yi verfasserin (orcid)0000-0002-1403-9841 aut Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2017 Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigating the toxicity of naphthenic acids, although other compounds may also contribute to the toxicity of oil sands process-affected water (OSPW). Here, we present a case study showing a systematic approach for profiling the organic composition of OSPW and environmental water samples by concentrating and separating dissolved organics through complementary liquid–liquid extractions followed by positive- or negative-ion mode ultrahigh resolution mass detection. Our comparative investigation shows clear differences in the composition of dissolved organics (homologues particularly) not only between OSPW samples and environmental water samples, but also differences among oil sands operators. Sulfur-containing compounds (especially the $ SO_{n} $classes) appear to have great potential to be used for evaluating the impact of OSPW, while our understanding of oxygen-only containing compounds should not be limited to $ O_{2} $ (i.e., classic naphthenic acids), but rather can be broadened to include many other compound classes (for instance $ O_{n} $, n = 1–9). Systematic profiling of water samples should be more widely implemented for monitoring the origin and transport of organics in aquatic ecosystems of the oil sands development region, northeastern Alberta, Canada. Environmental forensics (dpeaa)DE-He213 Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) (dpeaa)DE-He213 Oil sands (dpeaa)DE-He213 Alberta (dpeaa)DE-He213 Han, Jun aut Jean Birks, S. aut Borchers, Christoph H. aut Gibson, John J. aut Enthalten in Environmental earth sciences Berlin : Springer, 2009 76(2017), 24 vom: 16. Dez. (DE-627)599673451 (DE-600)2493699-6 1866-6299 nnns volume:76 year:2017 number:24 day:16 month:12 https://dx.doi.org/10.1007/s12665-017-7161-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 76 2017 24 16 12 |
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Yi, Yi |
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Yi, Yi misc Environmental forensics misc Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) misc Oil sands misc Alberta Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry |
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Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry Environmental forensics (dpeaa)DE-He213 Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) (dpeaa)DE-He213 Oil sands (dpeaa)DE-He213 Alberta (dpeaa)DE-He213 |
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profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution fourier transform mass spectrometry |
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Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry |
| abstract |
Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigating the toxicity of naphthenic acids, although other compounds may also contribute to the toxicity of oil sands process-affected water (OSPW). Here, we present a case study showing a systematic approach for profiling the organic composition of OSPW and environmental water samples by concentrating and separating dissolved organics through complementary liquid–liquid extractions followed by positive- or negative-ion mode ultrahigh resolution mass detection. Our comparative investigation shows clear differences in the composition of dissolved organics (homologues particularly) not only between OSPW samples and environmental water samples, but also differences among oil sands operators. Sulfur-containing compounds (especially the $ SO_{n} $classes) appear to have great potential to be used for evaluating the impact of OSPW, while our understanding of oxygen-only containing compounds should not be limited to $ O_{2} $ (i.e., classic naphthenic acids), but rather can be broadened to include many other compound classes (for instance $ O_{n} $, n = 1–9). Systematic profiling of water samples should be more widely implemented for monitoring the origin and transport of organics in aquatic ecosystems of the oil sands development region, northeastern Alberta, Canada. © Springer-Verlag GmbH Germany, part of Springer Nature 2017 |
| abstractGer |
Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigating the toxicity of naphthenic acids, although other compounds may also contribute to the toxicity of oil sands process-affected water (OSPW). Here, we present a case study showing a systematic approach for profiling the organic composition of OSPW and environmental water samples by concentrating and separating dissolved organics through complementary liquid–liquid extractions followed by positive- or negative-ion mode ultrahigh resolution mass detection. Our comparative investigation shows clear differences in the composition of dissolved organics (homologues particularly) not only between OSPW samples and environmental water samples, but also differences among oil sands operators. Sulfur-containing compounds (especially the $ SO_{n} $classes) appear to have great potential to be used for evaluating the impact of OSPW, while our understanding of oxygen-only containing compounds should not be limited to $ O_{2} $ (i.e., classic naphthenic acids), but rather can be broadened to include many other compound classes (for instance $ O_{n} $, n = 1–9). Systematic profiling of water samples should be more widely implemented for monitoring the origin and transport of organics in aquatic ecosystems of the oil sands development region, northeastern Alberta, Canada. © Springer-Verlag GmbH Germany, part of Springer Nature 2017 |
| abstract_unstemmed |
Abstract Understanding and characterizing organics in aquatic environments is a great challenge for environmental monitoring, especially for the oil sands industry due to the complexity and potential toxicity of dissolved organics in water. To date, significant efforts have been made in investigating the toxicity of naphthenic acids, although other compounds may also contribute to the toxicity of oil sands process-affected water (OSPW). Here, we present a case study showing a systematic approach for profiling the organic composition of OSPW and environmental water samples by concentrating and separating dissolved organics through complementary liquid–liquid extractions followed by positive- or negative-ion mode ultrahigh resolution mass detection. Our comparative investigation shows clear differences in the composition of dissolved organics (homologues particularly) not only between OSPW samples and environmental water samples, but also differences among oil sands operators. Sulfur-containing compounds (especially the $ SO_{n} $classes) appear to have great potential to be used for evaluating the impact of OSPW, while our understanding of oxygen-only containing compounds should not be limited to $ O_{2} $ (i.e., classic naphthenic acids), but rather can be broadened to include many other compound classes (for instance $ O_{n} $, n = 1–9). Systematic profiling of water samples should be more widely implemented for monitoring the origin and transport of organics in aquatic ecosystems of the oil sands development region, northeastern Alberta, Canada. © Springer-Verlag GmbH Germany, part of Springer Nature 2017 |
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Profiling of dissolved organic compounds in the oil sands region using complimentary liquid–liquid extraction and ultrahigh resolution Fourier transform mass spectrometry |
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https://dx.doi.org/10.1007/s12665-017-7161-0 |
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Han, Jun Jean Birks, S. Borchers, Christoph H. Gibson, John J. |
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| score |
7.3992643 |