Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes
Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vin...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Baettig, Julia [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017 |
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| Schlagwörter: |
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| Anmerkung: |
© The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 |
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| Übergeordnetes Werk: |
Enthalten in: Macromolecular research - Heidelberg : Springer, 2010, 25(2017), 11 vom: 07. Sept., Seite 1091-1099 |
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| Übergeordnetes Werk: |
volume:25 ; year:2017 ; number:11 ; day:07 ; month:09 ; pages:1091-1099 |
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| DOI / URN: |
10.1007/s13233-017-5142-5 |
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| Katalog-ID: |
SPR030968577 |
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| 100 | 1 | |a Baettig, Julia |e verfasserin |4 aut | |
| 245 | 1 | 0 | |a Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes |
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| 520 | |a Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. | ||
| 650 | 4 | |a nanoporous membranes |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a block copolymer assembly |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a nanopore size |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a nanopore chemistry |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a layer-by-layer assembly of polyelectrolytes |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a integral asymmetric membranes |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a deposition in nanopores |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Oh, Junki |4 aut | |
| 700 | 1 | |a Bang, Joona |4 aut | |
| 700 | 1 | |a Khan, Anzar |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Macromolecular research |d Heidelberg : Springer, 2010 |g 25(2017), 11 vom: 07. Sept., Seite 1091-1099 |w (DE-627)618327576 |w (DE-600)2537708-5 |x 2092-7673 |7 nnns |
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10.1007/s13233-017-5142-5 doi (DE-627)SPR030968577 (SPR)s13233-017-5142-5-e DE-627 ger DE-627 rakwb eng Baettig, Julia verfasserin aut Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. nanoporous membranes (dpeaa)DE-He213 block copolymer assembly (dpeaa)DE-He213 nanopore size (dpeaa)DE-He213 nanopore chemistry (dpeaa)DE-He213 layer-by-layer assembly of polyelectrolytes (dpeaa)DE-He213 integral asymmetric membranes (dpeaa)DE-He213 deposition in nanopores (dpeaa)DE-He213 Oh, Junki aut Bang, Joona aut Khan, Anzar aut Enthalten in Macromolecular research Heidelberg : Springer, 2010 25(2017), 11 vom: 07. Sept., Seite 1091-1099 (DE-627)618327576 (DE-600)2537708-5 2092-7673 nnns volume:25 year:2017 number:11 day:07 month:09 pages:1091-1099 https://dx.doi.org/10.1007/s13233-017-5142-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2017 11 07 09 1091-1099 |
| spelling |
10.1007/s13233-017-5142-5 doi (DE-627)SPR030968577 (SPR)s13233-017-5142-5-e DE-627 ger DE-627 rakwb eng Baettig, Julia verfasserin aut Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. nanoporous membranes (dpeaa)DE-He213 block copolymer assembly (dpeaa)DE-He213 nanopore size (dpeaa)DE-He213 nanopore chemistry (dpeaa)DE-He213 layer-by-layer assembly of polyelectrolytes (dpeaa)DE-He213 integral asymmetric membranes (dpeaa)DE-He213 deposition in nanopores (dpeaa)DE-He213 Oh, Junki aut Bang, Joona aut Khan, Anzar aut Enthalten in Macromolecular research Heidelberg : Springer, 2010 25(2017), 11 vom: 07. Sept., Seite 1091-1099 (DE-627)618327576 (DE-600)2537708-5 2092-7673 nnns volume:25 year:2017 number:11 day:07 month:09 pages:1091-1099 https://dx.doi.org/10.1007/s13233-017-5142-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2017 11 07 09 1091-1099 |
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10.1007/s13233-017-5142-5 doi (DE-627)SPR030968577 (SPR)s13233-017-5142-5-e DE-627 ger DE-627 rakwb eng Baettig, Julia verfasserin aut Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. nanoporous membranes (dpeaa)DE-He213 block copolymer assembly (dpeaa)DE-He213 nanopore size (dpeaa)DE-He213 nanopore chemistry (dpeaa)DE-He213 layer-by-layer assembly of polyelectrolytes (dpeaa)DE-He213 integral asymmetric membranes (dpeaa)DE-He213 deposition in nanopores (dpeaa)DE-He213 Oh, Junki aut Bang, Joona aut Khan, Anzar aut Enthalten in Macromolecular research Heidelberg : Springer, 2010 25(2017), 11 vom: 07. Sept., Seite 1091-1099 (DE-627)618327576 (DE-600)2537708-5 2092-7673 nnns volume:25 year:2017 number:11 day:07 month:09 pages:1091-1099 https://dx.doi.org/10.1007/s13233-017-5142-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2017 11 07 09 1091-1099 |
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10.1007/s13233-017-5142-5 doi (DE-627)SPR030968577 (SPR)s13233-017-5142-5-e DE-627 ger DE-627 rakwb eng Baettig, Julia verfasserin aut Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. nanoporous membranes (dpeaa)DE-He213 block copolymer assembly (dpeaa)DE-He213 nanopore size (dpeaa)DE-He213 nanopore chemistry (dpeaa)DE-He213 layer-by-layer assembly of polyelectrolytes (dpeaa)DE-He213 integral asymmetric membranes (dpeaa)DE-He213 deposition in nanopores (dpeaa)DE-He213 Oh, Junki aut Bang, Joona aut Khan, Anzar aut Enthalten in Macromolecular research Heidelberg : Springer, 2010 25(2017), 11 vom: 07. Sept., Seite 1091-1099 (DE-627)618327576 (DE-600)2537708-5 2092-7673 nnns volume:25 year:2017 number:11 day:07 month:09 pages:1091-1099 https://dx.doi.org/10.1007/s13233-017-5142-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2017 11 07 09 1091-1099 |
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10.1007/s13233-017-5142-5 doi (DE-627)SPR030968577 (SPR)s13233-017-5142-5-e DE-627 ger DE-627 rakwb eng Baettig, Julia verfasserin aut Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes 2017 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. nanoporous membranes (dpeaa)DE-He213 block copolymer assembly (dpeaa)DE-He213 nanopore size (dpeaa)DE-He213 nanopore chemistry (dpeaa)DE-He213 layer-by-layer assembly of polyelectrolytes (dpeaa)DE-He213 integral asymmetric membranes (dpeaa)DE-He213 deposition in nanopores (dpeaa)DE-He213 Oh, Junki aut Bang, Joona aut Khan, Anzar aut Enthalten in Macromolecular research Heidelberg : Springer, 2010 25(2017), 11 vom: 07. Sept., Seite 1091-1099 (DE-627)618327576 (DE-600)2537708-5 2092-7673 nnns volume:25 year:2017 number:11 day:07 month:09 pages:1091-1099 https://dx.doi.org/10.1007/s13233-017-5142-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 25 2017 11 07 09 1091-1099 |
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Enthalten in Macromolecular research 25(2017), 11 vom: 07. Sept., Seite 1091-1099 volume:25 year:2017 number:11 day:07 month:09 pages:1091-1099 |
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Baettig, Julia @@aut@@ Oh, Junki @@aut@@ Bang, Joona @@aut@@ Khan, Anzar @@aut@@ |
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In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. 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Baettig, Julia |
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Baettig, Julia misc nanoporous membranes misc block copolymer assembly misc nanopore size misc nanopore chemistry misc layer-by-layer assembly of polyelectrolytes misc integral asymmetric membranes misc deposition in nanopores Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes |
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Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes nanoporous membranes (dpeaa)DE-He213 block copolymer assembly (dpeaa)DE-He213 nanopore size (dpeaa)DE-He213 nanopore chemistry (dpeaa)DE-He213 layer-by-layer assembly of polyelectrolytes (dpeaa)DE-He213 integral asymmetric membranes (dpeaa)DE-He213 deposition in nanopores (dpeaa)DE-He213 |
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misc nanoporous membranes misc block copolymer assembly misc nanopore size misc nanopore chemistry misc layer-by-layer assembly of polyelectrolytes misc integral asymmetric membranes misc deposition in nanopores |
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misc nanoporous membranes misc block copolymer assembly misc nanopore size misc nanopore chemistry misc layer-by-layer assembly of polyelectrolytes misc integral asymmetric membranes misc deposition in nanopores |
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misc nanoporous membranes misc block copolymer assembly misc nanopore size misc nanopore chemistry misc layer-by-layer assembly of polyelectrolytes misc integral asymmetric membranes misc deposition in nanopores |
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Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes |
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10.1007/s13233-017-5142-5 |
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sequential coating of nanopores with charged polymers: a general approach for controlling pore properties of self-assembled block copolymer membranes |
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Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes |
| abstract |
Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 |
| abstractGer |
Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 |
| abstract_unstemmed |
Abstract A general approach is developed for controlling the pore size and pore chemistry of integral isoporous membranes derived from the assembly of polystyrene-b-poly-4-vinyl pyridine (PS-b-P4VP) diblock copolymer. In this approach, initially, the sub-50 nm pore surface, decorated with poly-4-vinyl pyridine (P4VP) polymer brush, is coated with polyacrylic acid (PAA). PAA offers a majority of anionic and a minority of neutral acid functionalities. The neutral acid groups adhere to the P4VP segments of the pore wall through hydrogen bonding interactions and the anionic sites remain free. The availability of the anionic sites sets the stage for a layer-by-layer deposition of cationic and anionic polymers, in a sequential manner, on the pore-wall surface through a continuous flow of a dilute polyelectrolyte solution through the nanoporous membrane. In this way, multiple layers, stabilized through electrostatic interactions, can be deposited leading to a continuous decrease in the pore size and a known surface charge. Due to the known facile nature of the large area isoporous asymmetric membrane formation and modular nature of the polyelectrolyte assembly, the present approach is anticipated to yield new block copolymer membranes with tailored separation, sensing, and catalytic properties. © The Polymer Society of Korea and Springer Science+Business Media B.V. 2017 |
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11 |
| title_short |
Sequential coating of nanopores with charged polymers: A general approach for controlling pore properties of self-assembled block copolymer membranes |
| url |
https://dx.doi.org/10.1007/s13233-017-5142-5 |
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| author2 |
Oh, Junki Bang, Joona Khan, Anzar |
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| doi_str |
10.1007/s13233-017-5142-5 |
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2024-07-03T21:13:12.842Z |
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| score |
7.3972797 |