NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5)
Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carr...
Ausführliche Beschreibung
Autor*in: |
Shimizu, Kenji [verfasserIn] Yamaguchi, Masanori [verfasserIn] Yuan, Shujuan [verfasserIn] Cao, Shixun [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2013 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Journal of the Korean Physical Society - Berlin : Springer, 1968, 63(2013), 3 vom: Aug., Seite 636-639 |
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Übergeordnetes Werk: |
volume:63 ; year:2013 ; number:3 ; month:08 ; pages:636-639 |
Links: |
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DOI / URN: |
10.3938/jkps.63.636 |
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Katalog-ID: |
SPR032705743 |
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245 | 1 | 0 | |a NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) |
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520 | |a Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. | ||
650 | 4 | |a Manganites |7 (dpeaa)DE-He213 | |
650 | 4 | |a Phase separation |7 (dpeaa)DE-He213 | |
650 | 4 | |a Eu |7 (dpeaa)DE-He213 | |
650 | 4 | |a Sr |7 (dpeaa)DE-He213 | |
650 | 4 | |a MnO |7 (dpeaa)DE-He213 | |
650 | 4 | |a Spin-echo NMR |7 (dpeaa)DE-He213 | |
700 | 1 | |a Yamaguchi, Masanori |e verfasserin |4 aut | |
700 | 1 | |a Yuan, Shujuan |e verfasserin |4 aut | |
700 | 1 | |a Cao, Shixun |e verfasserin |4 aut | |
773 | 0 | 8 | |i Enthalten in |t Journal of the Korean Physical Society |d Berlin : Springer, 1968 |g 63(2013), 3 vom: Aug., Seite 636-639 |w (DE-627)328820865 |w (DE-600)2046361-3 |x 1976-8524 |7 nnns |
773 | 1 | 8 | |g volume:63 |g year:2013 |g number:3 |g month:08 |g pages:636-639 |
856 | 4 | 0 | |u https://dx.doi.org/10.3938/jkps.63.636 |z lizenzpflichtig |3 Volltext |
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10.3938/jkps.63.636 doi (DE-627)SPR032705743 (SPR)jkps.63.636-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Shimizu, Kenji verfasserin aut NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) 2013 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. Manganites (dpeaa)DE-He213 Phase separation (dpeaa)DE-He213 Eu (dpeaa)DE-He213 Sr (dpeaa)DE-He213 MnO (dpeaa)DE-He213 Spin-echo NMR (dpeaa)DE-He213 Yamaguchi, Masanori verfasserin aut Yuan, Shujuan verfasserin aut Cao, Shixun verfasserin aut Enthalten in Journal of the Korean Physical Society Berlin : Springer, 1968 63(2013), 3 vom: Aug., Seite 636-639 (DE-627)328820865 (DE-600)2046361-3 1976-8524 nnns volume:63 year:2013 number:3 month:08 pages:636-639 https://dx.doi.org/10.3938/jkps.63.636 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 63 2013 3 08 636-639 |
spelling |
10.3938/jkps.63.636 doi (DE-627)SPR032705743 (SPR)jkps.63.636-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Shimizu, Kenji verfasserin aut NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) 2013 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. Manganites (dpeaa)DE-He213 Phase separation (dpeaa)DE-He213 Eu (dpeaa)DE-He213 Sr (dpeaa)DE-He213 MnO (dpeaa)DE-He213 Spin-echo NMR (dpeaa)DE-He213 Yamaguchi, Masanori verfasserin aut Yuan, Shujuan verfasserin aut Cao, Shixun verfasserin aut Enthalten in Journal of the Korean Physical Society Berlin : Springer, 1968 63(2013), 3 vom: Aug., Seite 636-639 (DE-627)328820865 (DE-600)2046361-3 1976-8524 nnns volume:63 year:2013 number:3 month:08 pages:636-639 https://dx.doi.org/10.3938/jkps.63.636 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 63 2013 3 08 636-639 |
allfields_unstemmed |
10.3938/jkps.63.636 doi (DE-627)SPR032705743 (SPR)jkps.63.636-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Shimizu, Kenji verfasserin aut NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) 2013 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. Manganites (dpeaa)DE-He213 Phase separation (dpeaa)DE-He213 Eu (dpeaa)DE-He213 Sr (dpeaa)DE-He213 MnO (dpeaa)DE-He213 Spin-echo NMR (dpeaa)DE-He213 Yamaguchi, Masanori verfasserin aut Yuan, Shujuan verfasserin aut Cao, Shixun verfasserin aut Enthalten in Journal of the Korean Physical Society Berlin : Springer, 1968 63(2013), 3 vom: Aug., Seite 636-639 (DE-627)328820865 (DE-600)2046361-3 1976-8524 nnns volume:63 year:2013 number:3 month:08 pages:636-639 https://dx.doi.org/10.3938/jkps.63.636 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 63 2013 3 08 636-639 |
allfieldsGer |
10.3938/jkps.63.636 doi (DE-627)SPR032705743 (SPR)jkps.63.636-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Shimizu, Kenji verfasserin aut NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) 2013 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. Manganites (dpeaa)DE-He213 Phase separation (dpeaa)DE-He213 Eu (dpeaa)DE-He213 Sr (dpeaa)DE-He213 MnO (dpeaa)DE-He213 Spin-echo NMR (dpeaa)DE-He213 Yamaguchi, Masanori verfasserin aut Yuan, Shujuan verfasserin aut Cao, Shixun verfasserin aut Enthalten in Journal of the Korean Physical Society Berlin : Springer, 1968 63(2013), 3 vom: Aug., Seite 636-639 (DE-627)328820865 (DE-600)2046361-3 1976-8524 nnns volume:63 year:2013 number:3 month:08 pages:636-639 https://dx.doi.org/10.3938/jkps.63.636 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 63 2013 3 08 636-639 |
allfieldsSound |
10.3938/jkps.63.636 doi (DE-627)SPR032705743 (SPR)jkps.63.636-e DE-627 ger DE-627 rakwb eng 530 ASE 33.00 bkl Shimizu, Kenji verfasserin aut NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) 2013 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. Manganites (dpeaa)DE-He213 Phase separation (dpeaa)DE-He213 Eu (dpeaa)DE-He213 Sr (dpeaa)DE-He213 MnO (dpeaa)DE-He213 Spin-echo NMR (dpeaa)DE-He213 Yamaguchi, Masanori verfasserin aut Yuan, Shujuan verfasserin aut Cao, Shixun verfasserin aut Enthalten in Journal of the Korean Physical Society Berlin : Springer, 1968 63(2013), 3 vom: Aug., Seite 636-639 (DE-627)328820865 (DE-600)2046361-3 1976-8524 nnns volume:63 year:2013 number:3 month:08 pages:636-639 https://dx.doi.org/10.3938/jkps.63.636 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.00 ASE AR 63 2013 3 08 636-639 |
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Enthalten in Journal of the Korean Physical Society 63(2013), 3 vom: Aug., Seite 636-639 volume:63 year:2013 number:3 month:08 pages:636-639 |
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Enthalten in Journal of the Korean Physical Society 63(2013), 3 vom: Aug., Seite 636-639 volume:63 year:2013 number:3 month:08 pages:636-639 |
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Manganites Phase separation Eu Sr MnO Spin-echo NMR |
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Journal of the Korean Physical Society |
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Shimizu, Kenji @@aut@@ Yamaguchi, Masanori @@aut@@ Yuan, Shujuan @@aut@@ Cao, Shixun @@aut@@ |
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The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Manganites</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Phase separation</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Eu</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Sr</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">MnO</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" 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|
author |
Shimizu, Kenji |
spellingShingle |
Shimizu, Kenji ddc 530 bkl 33.00 misc Manganites misc Phase separation misc Eu misc Sr misc MnO misc Spin-echo NMR NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) |
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1976-8524 |
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530 ASE 33.00 bkl NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) Manganites (dpeaa)DE-He213 Phase separation (dpeaa)DE-He213 Eu (dpeaa)DE-He213 Sr (dpeaa)DE-He213 MnO (dpeaa)DE-He213 Spin-echo NMR (dpeaa)DE-He213 |
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ddc 530 bkl 33.00 misc Manganites misc Phase separation misc Eu misc Sr misc MnO misc Spin-echo NMR |
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ddc 530 bkl 33.00 misc Manganites misc Phase separation misc Eu misc Sr misc MnO misc Spin-echo NMR |
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NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) |
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NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) |
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Shimizu, Kenji |
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Journal of the Korean Physical Society |
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Shimizu, Kenji Yamaguchi, Masanori Yuan, Shujuan Cao, Shixun |
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530 ASE 33.00 bkl |
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Shimizu, Kenji |
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nmr study of magnetic properties of $ eu_{1−x} %$ sr_{x} %$ mno_{3} $ (0 ≤ x ≤ 0.5) |
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NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) |
abstract |
Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. |
abstractGer |
Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. |
abstract_unstemmed |
Abstract The perovskite manganite $ EuMnO_{3} $ is known to be a compound with a narrow eg-band width due to small ionic radius of $ Eu^{3+} $ compared to $ La^{3+} $. The $ Eu_{1 −x} %$ Sr_{x} %$ MnO_{3} $ compounds show complex magnetic properties, depending on the Sr concentration x. We have carried out 55Mn spin-echo nuclear magnetic resonance (NMR) measurements on polycrystalline $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x≤ 0.5) compounds at 4.2 or 1.4 K in order to clarify the microscopic local magnetic state of the Mn ions. NMR spectra have been observed in the frequency range from ∼250 MHz to ∼400 MHz. For the A-type antiferromagnetic $ EuMnO_{3} $, the resonance frequency is about 260 MHz, which is much lower than that observed for $ Mn^{3+} $ in $ La_{1−x} %$ Sr_{x} %$ MnO_{3} $. For 0.1 ≤ x ≤ 0.4, the resonance lines corresponding to $ Mn^{4+} $ and $ Mn^{3+} $ have been observed at about 315 MHz and 390 MHz, respectively. Furthermore, the spectra originating from $ Mn^{2+} $ have been observed around 590 MHz for 0.1 ≤ x ≤ 0.4. For $ Eu_{0.5} %$ Sr_{0.5} %$ MnO_{3} $, the NMR spectrum spreads widely with several distinct peaks in the frequency range from 250 MHz to 410 MHz, which shows that the compound is in an inhomogeneous state due to competition between the antiferromagnetic and the ferromagnetic states. |
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container_issue |
3 |
title_short |
NMR study of magnetic properties of $ Eu_{1−x} %$ Sr_{x} %$ MnO_{3} $ (0 ≤ x ≤ 0.5) |
url |
https://dx.doi.org/10.3938/jkps.63.636 |
remote_bool |
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author2 |
Yamaguchi, Masanori Yuan, Shujuan Cao, Shixun |
author2Str |
Yamaguchi, Masanori Yuan, Shujuan Cao, Shixun |
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hochschulschrift_bool |
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doi_str |
10.3938/jkps.63.636 |
up_date |
2024-07-03T14:18:14.297Z |
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|
score |
7.402356 |