Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes

Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK),...
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Autor*in:	Panthi, Dhruba [verfasserIn] Hedayat, Nader [verfasserIn] Du, Yanhai [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2018

Schlagwörter:	yttria-stabilized zirconia (YSZ) SOFC electrolyte densification shrinkage co-sintering

Übergeordnetes Werk:	Enthalten in: Journal of Advanced Ceramics - Berlin : SpringerOpen, 2012, 7(2018), 4 vom: 21. Nov., Seite 325-335
Übergeordnetes Werk:	volume:7 ; year:2018 ; number:4 ; day:21 ; month:11 ; pages:325-335

Links:	Volltext

DOI / URN:	10.1007/s40145-018-0282-4

Katalog-ID:	SPR03312311X

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520			\|a Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes.
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allfields	10.1007/s40145-018-0282-4 doi (DE-627)SPR03312311X (SPR)s40145-018-0282-4-e DE-627 ger DE-627 rakwb eng 660 ASE Panthi, Dhruba verfasserin aut Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes. yttria-stabilized zirconia (YSZ) (dpeaa)DE-He213 SOFC electrolyte (dpeaa)DE-He213 densification (dpeaa)DE-He213 shrinkage (dpeaa)DE-He213 co-sintering (dpeaa)DE-He213 Hedayat, Nader verfasserin aut Du, Yanhai verfasserin aut Enthalten in Journal of Advanced Ceramics Berlin : SpringerOpen, 2012 7(2018), 4 vom: 21. Nov., Seite 325-335 (DE-627)726491497 (DE-600)2682430-9 2227-8508 nnns volume:7 year:2018 number:4 day:21 month:11 pages:325-335 https://dx.doi.org/10.1007/s40145-018-0282-4 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2018 4 21 11 325-335
spelling	10.1007/s40145-018-0282-4 doi (DE-627)SPR03312311X (SPR)s40145-018-0282-4-e DE-627 ger DE-627 rakwb eng 660 ASE Panthi, Dhruba verfasserin aut Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes. yttria-stabilized zirconia (YSZ) (dpeaa)DE-He213 SOFC electrolyte (dpeaa)DE-He213 densification (dpeaa)DE-He213 shrinkage (dpeaa)DE-He213 co-sintering (dpeaa)DE-He213 Hedayat, Nader verfasserin aut Du, Yanhai verfasserin aut Enthalten in Journal of Advanced Ceramics Berlin : SpringerOpen, 2012 7(2018), 4 vom: 21. Nov., Seite 325-335 (DE-627)726491497 (DE-600)2682430-9 2227-8508 nnns volume:7 year:2018 number:4 day:21 month:11 pages:325-335 https://dx.doi.org/10.1007/s40145-018-0282-4 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2018 4 21 11 325-335
allfields_unstemmed	10.1007/s40145-018-0282-4 doi (DE-627)SPR03312311X (SPR)s40145-018-0282-4-e DE-627 ger DE-627 rakwb eng 660 ASE Panthi, Dhruba verfasserin aut Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes. yttria-stabilized zirconia (YSZ) (dpeaa)DE-He213 SOFC electrolyte (dpeaa)DE-He213 densification (dpeaa)DE-He213 shrinkage (dpeaa)DE-He213 co-sintering (dpeaa)DE-He213 Hedayat, Nader verfasserin aut Du, Yanhai verfasserin aut Enthalten in Journal of Advanced Ceramics Berlin : SpringerOpen, 2012 7(2018), 4 vom: 21. Nov., Seite 325-335 (DE-627)726491497 (DE-600)2682430-9 2227-8508 nnns volume:7 year:2018 number:4 day:21 month:11 pages:325-335 https://dx.doi.org/10.1007/s40145-018-0282-4 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2018 4 21 11 325-335
allfieldsGer	10.1007/s40145-018-0282-4 doi (DE-627)SPR03312311X (SPR)s40145-018-0282-4-e DE-627 ger DE-627 rakwb eng 660 ASE Panthi, Dhruba verfasserin aut Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes. yttria-stabilized zirconia (YSZ) (dpeaa)DE-He213 SOFC electrolyte (dpeaa)DE-He213 densification (dpeaa)DE-He213 shrinkage (dpeaa)DE-He213 co-sintering (dpeaa)DE-He213 Hedayat, Nader verfasserin aut Du, Yanhai verfasserin aut Enthalten in Journal of Advanced Ceramics Berlin : SpringerOpen, 2012 7(2018), 4 vom: 21. Nov., Seite 325-335 (DE-627)726491497 (DE-600)2682430-9 2227-8508 nnns volume:7 year:2018 number:4 day:21 month:11 pages:325-335 https://dx.doi.org/10.1007/s40145-018-0282-4 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2018 4 21 11 325-335
allfieldsSound	10.1007/s40145-018-0282-4 doi (DE-627)SPR03312311X (SPR)s40145-018-0282-4-e DE-627 ger DE-627 rakwb eng 660 ASE Panthi, Dhruba verfasserin aut Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes 2018 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes. yttria-stabilized zirconia (YSZ) (dpeaa)DE-He213 SOFC electrolyte (dpeaa)DE-He213 densification (dpeaa)DE-He213 shrinkage (dpeaa)DE-He213 co-sintering (dpeaa)DE-He213 Hedayat, Nader verfasserin aut Du, Yanhai verfasserin aut Enthalten in Journal of Advanced Ceramics Berlin : SpringerOpen, 2012 7(2018), 4 vom: 21. Nov., Seite 325-335 (DE-627)726491497 (DE-600)2682430-9 2227-8508 nnns volume:7 year:2018 number:4 day:21 month:11 pages:325-335 https://dx.doi.org/10.1007/s40145-018-0282-4 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2014 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 7 2018 4 21 11 325-335
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source	Enthalten in Journal of Advanced Ceramics 7(2018), 4 vom: 21. Nov., Seite 325-335 volume:7 year:2018 number:4 day:21 month:11 pages:325-335
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Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. 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author	Panthi, Dhruba
spellingShingle	Panthi, Dhruba ddc 660 misc yttria-stabilized zirconia (YSZ) misc SOFC electrolyte misc densification misc shrinkage misc co-sintering Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes
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topic_title	660 ASE Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes yttria-stabilized zirconia (YSZ) (dpeaa)DE-He213 SOFC electrolyte (dpeaa)DE-He213 densification (dpeaa)DE-He213 shrinkage (dpeaa)DE-He213 co-sintering (dpeaa)DE-He213
topic	ddc 660 misc yttria-stabilized zirconia (YSZ) misc SOFC electrolyte misc densification misc shrinkage misc co-sintering
topic_unstemmed	ddc 660 misc yttria-stabilized zirconia (YSZ) misc SOFC electrolyte misc densification misc shrinkage misc co-sintering
topic_browse	ddc 660 misc yttria-stabilized zirconia (YSZ) misc SOFC electrolyte misc densification misc shrinkage misc co-sintering
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title	Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes
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title_full	Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes
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title_sort	densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes
title_auth	Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes
abstract	Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes.
abstractGer	Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes.
abstract_unstemmed	Abstract Yttria-stabilized zirconia (YSZ) is the most common electrolyte material for solid oxide fuel cells. Herein, we conducted a comparative study on the densification behavior of three different kinds of commercial 8 mol% YSZ powders: (i) TZ-8Y (Tosoh, Japan), (ii) MELox 8Y (MEL Chemicals, UK), and (iii) YSZ-HT (Huatsing Power, China). The comparison was made on both the self-supporting pellets and thin-film electrolytes coated onto a NiO–YSZ anode support. For the pellets, MELox 8Y showed the highest densification at lower sintering temperatures with 93% and 96% of the theoretical density at 1250 and 1300 °C, respectively. Although YSZ-HT showed a higher sintering rate than TZ-8Y, a sintering temperature of 1350 °C was required for both the powders to reach 95% of the theoretical density. For the thin-film electrolytes, on the other hand, YSZ-HT showed the highest sintering rate with a dense microstructure at a co-sintering temperature of 1250 °C. Our results indicate that besides the average particle size, other factors such as particle size distribution and post-processing play a significant role in determining the sintering rate and densification behavior of the YSZ powders. Additionally, a close match in the sintering shrinkage of the electrolyte and anode support is important for facilitating the densification of the thin-film electrolytes.
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title_short	Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes
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up_date	2024-07-03T16:46:43.795Z
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Densification behavior of yttria-stabilized zirconia powders for solid oxide fuel cell electrolytes

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