Speciation of arsenic: a case study of PM1 in Zabrze
Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V)...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Nocoń, Katarzyna [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s) 2019 |
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| Übergeordnetes Werk: |
Enthalten in: SN applied sciences - [Cham] : Springer International Publishing, 2019, 1(2019), 5 vom: 12. Apr. |
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| Übergeordnetes Werk: |
volume:1 ; year:2019 ; number:5 ; day:12 ; month:04 |
| Links: |
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| DOI / URN: |
10.1007/s42452-019-0456-x |
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| Katalog-ID: |
SPR038573059 |
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| 520 | |a Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. | ||
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10.1007/s42452-019-0456-x doi (DE-627)SPR038573059 (SPR)s42452-019-0456-x-e DE-627 ger DE-627 rakwb eng Nocoń, Katarzyna verfasserin (orcid)0000-0003-0674-3131 aut Speciation of arsenic: a case study of PM1 in Zabrze 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2019 Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. Arsenic (V) (dpeaa)DE-He213 Arsenic (III) (dpeaa)DE-He213 Water-soluble arsenic (dpeaa)DE-He213 PM1 (dpeaa)DE-He213 Rogula-Kozłowska, Wioletta aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 5 vom: 12. Apr. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:5 day:12 month:04 https://dx.doi.org/10.1007/s42452-019-0456-x kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 5 12 04 |
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10.1007/s42452-019-0456-x doi (DE-627)SPR038573059 (SPR)s42452-019-0456-x-e DE-627 ger DE-627 rakwb eng Nocoń, Katarzyna verfasserin (orcid)0000-0003-0674-3131 aut Speciation of arsenic: a case study of PM1 in Zabrze 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2019 Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. Arsenic (V) (dpeaa)DE-He213 Arsenic (III) (dpeaa)DE-He213 Water-soluble arsenic (dpeaa)DE-He213 PM1 (dpeaa)DE-He213 Rogula-Kozłowska, Wioletta aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 5 vom: 12. Apr. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:5 day:12 month:04 https://dx.doi.org/10.1007/s42452-019-0456-x kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 5 12 04 |
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10.1007/s42452-019-0456-x doi (DE-627)SPR038573059 (SPR)s42452-019-0456-x-e DE-627 ger DE-627 rakwb eng Nocoń, Katarzyna verfasserin (orcid)0000-0003-0674-3131 aut Speciation of arsenic: a case study of PM1 in Zabrze 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2019 Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. Arsenic (V) (dpeaa)DE-He213 Arsenic (III) (dpeaa)DE-He213 Water-soluble arsenic (dpeaa)DE-He213 PM1 (dpeaa)DE-He213 Rogula-Kozłowska, Wioletta aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 5 vom: 12. Apr. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:5 day:12 month:04 https://dx.doi.org/10.1007/s42452-019-0456-x kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 5 12 04 |
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10.1007/s42452-019-0456-x doi (DE-627)SPR038573059 (SPR)s42452-019-0456-x-e DE-627 ger DE-627 rakwb eng Nocoń, Katarzyna verfasserin (orcid)0000-0003-0674-3131 aut Speciation of arsenic: a case study of PM1 in Zabrze 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2019 Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. Arsenic (V) (dpeaa)DE-He213 Arsenic (III) (dpeaa)DE-He213 Water-soluble arsenic (dpeaa)DE-He213 PM1 (dpeaa)DE-He213 Rogula-Kozłowska, Wioletta aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 5 vom: 12. Apr. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:5 day:12 month:04 https://dx.doi.org/10.1007/s42452-019-0456-x kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 5 12 04 |
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10.1007/s42452-019-0456-x doi (DE-627)SPR038573059 (SPR)s42452-019-0456-x-e DE-627 ger DE-627 rakwb eng Nocoń, Katarzyna verfasserin (orcid)0000-0003-0674-3131 aut Speciation of arsenic: a case study of PM1 in Zabrze 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2019 Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. Arsenic (V) (dpeaa)DE-He213 Arsenic (III) (dpeaa)DE-He213 Water-soluble arsenic (dpeaa)DE-He213 PM1 (dpeaa)DE-He213 Rogula-Kozłowska, Wioletta aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 5 vom: 12. Apr. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:5 day:12 month:04 https://dx.doi.org/10.1007/s42452-019-0456-x kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 5 12 04 |
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Nocoń, Katarzyna |
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Nocoń, Katarzyna misc Arsenic (V) misc Arsenic (III) misc Water-soluble arsenic misc PM1 Speciation of arsenic: a case study of PM1 in Zabrze |
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Speciation of arsenic: a case study of PM1 in Zabrze Arsenic (V) (dpeaa)DE-He213 Arsenic (III) (dpeaa)DE-He213 Water-soluble arsenic (dpeaa)DE-He213 PM1 (dpeaa)DE-He213 |
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speciation of arsenic: a case study of pm1 in zabrze |
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Speciation of arsenic: a case study of PM1 in Zabrze |
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Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. © The Author(s) 2019 |
| abstractGer |
Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. © The Author(s) 2019 |
| abstract_unstemmed |
Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%. © The Author(s) 2019 |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR038573059</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230328214959.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">201007s2019 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s42452-019-0456-x</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR038573059</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s42452-019-0456-x-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Nocoń, Katarzyna</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0003-0674-3131</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Speciation of arsenic: a case study of PM1 in Zabrze</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2019</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© The Author(s) 2019</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract The aim of the study was to determine ambient concentrations of soluble, inorganic form of As ((As(III) and As(V)) in submicron atmospheric particles (PM1) in one of the most polluted region of Europe (Upper Silesia, Poland). Quantitative analyses of soluble As, soluble As (III) and As (V) after chromatographic separation and total As in digested PM1 samples were performed on the Elan 6100 DRC-e ICP-MS spectrometer. Results of analysis of the 15 randomly selected daily samples of PM1 from summer to winter season were presented. We showed that As(V) is dominating soluble, inorganic form of As in ambient air of selected city in Upper Silesia (Zabrze). Ambient concentrations of As(III) and As(V) as well as their mass percentages in water-soluble and total As changed seasonally. In winter season, when emissions from coal combustion prevailed, ambient concentration of soluble As(V) was about three times higher than in summer and accounted for 55% of total As. Ambient mass of As(III) was about 3.7% of the total As mass. During summer, when the sources of As may be more differentiated (industry, traffic, secondary emission from some surfaces, e.g., soils, roads, farmlands and dumps), soluble As(V) accounted for 23% of total As while soluble As(III) 6.7%.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Arsenic (V)</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Arsenic (III)</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Water-soluble arsenic</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">PM1</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Rogula-Kozłowska, Wioletta</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">SN applied sciences</subfield><subfield code="d">[Cham] : Springer International Publishing, 2019</subfield><subfield code="g">1(2019), 5 vom: 12. 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