Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template
Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscop...
Ausführliche Beschreibung
Autor*in: |
Sabarish, R. [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2019 |
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Schlagwörter: |
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Anmerkung: |
© Springer Nature Switzerland AG 2019 |
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Übergeordnetes Werk: |
Enthalten in: SN applied sciences - [Cham] : Springer International Publishing, 2019, 1(2019), 9 vom: 06. Aug. |
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Übergeordnetes Werk: |
volume:1 ; year:2019 ; number:9 ; day:06 ; month:08 |
Links: |
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DOI / URN: |
10.1007/s42452-019-1036-9 |
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Katalog-ID: |
SPR038579006 |
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520 | |a Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract | ||
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10.1007/s42452-019-1036-9 doi (DE-627)SPR038579006 (SPR)s42452-019-1036-9-e DE-627 ger DE-627 rakwb eng Sabarish, R. verfasserin aut Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Nature Switzerland AG 2019 Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract Hierarchical zeolite (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Starch template (dpeaa)DE-He213 Catalytic activity (dpeaa)DE-He213 Unnikrishnan, G. aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 9 vom: 06. Aug. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:9 day:06 month:08 https://dx.doi.org/10.1007/s42452-019-1036-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 9 06 08 |
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10.1007/s42452-019-1036-9 doi (DE-627)SPR038579006 (SPR)s42452-019-1036-9-e DE-627 ger DE-627 rakwb eng Sabarish, R. verfasserin aut Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Nature Switzerland AG 2019 Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract Hierarchical zeolite (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Starch template (dpeaa)DE-He213 Catalytic activity (dpeaa)DE-He213 Unnikrishnan, G. aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 9 vom: 06. Aug. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:9 day:06 month:08 https://dx.doi.org/10.1007/s42452-019-1036-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 9 06 08 |
allfields_unstemmed |
10.1007/s42452-019-1036-9 doi (DE-627)SPR038579006 (SPR)s42452-019-1036-9-e DE-627 ger DE-627 rakwb eng Sabarish, R. verfasserin aut Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Nature Switzerland AG 2019 Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract Hierarchical zeolite (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Starch template (dpeaa)DE-He213 Catalytic activity (dpeaa)DE-He213 Unnikrishnan, G. aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 9 vom: 06. Aug. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:9 day:06 month:08 https://dx.doi.org/10.1007/s42452-019-1036-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 9 06 08 |
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10.1007/s42452-019-1036-9 doi (DE-627)SPR038579006 (SPR)s42452-019-1036-9-e DE-627 ger DE-627 rakwb eng Sabarish, R. verfasserin aut Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Nature Switzerland AG 2019 Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract Hierarchical zeolite (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Starch template (dpeaa)DE-He213 Catalytic activity (dpeaa)DE-He213 Unnikrishnan, G. aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 9 vom: 06. Aug. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:9 day:06 month:08 https://dx.doi.org/10.1007/s42452-019-1036-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 9 06 08 |
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10.1007/s42452-019-1036-9 doi (DE-627)SPR038579006 (SPR)s42452-019-1036-9-e DE-627 ger DE-627 rakwb eng Sabarish, R. verfasserin aut Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer Nature Switzerland AG 2019 Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract Hierarchical zeolite (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Starch template (dpeaa)DE-He213 Catalytic activity (dpeaa)DE-He213 Unnikrishnan, G. aut Enthalten in SN applied sciences [Cham] : Springer International Publishing, 2019 1(2019), 9 vom: 06. Aug. (DE-627)103761139X (DE-600)2947292-1 2523-3971 nnns volume:1 year:2019 number:9 day:06 month:08 https://dx.doi.org/10.1007/s42452-019-1036-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_90 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_138 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 1 2019 9 06 08 |
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Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template Hierarchical zeolite (dpeaa)DE-He213 Mesoporous (dpeaa)DE-He213 Starch template (dpeaa)DE-He213 Catalytic activity (dpeaa)DE-He213 |
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synthesis, characterization and evaluations of micro/mesoporous zsm-5 zeolite using starch as bio template |
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Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template |
abstract |
Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract © Springer Nature Switzerland AG 2019 |
abstractGer |
Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract © Springer Nature Switzerland AG 2019 |
abstract_unstemmed |
Abstract We report a simple and economical method to synthesis hierarchical ZSM-5 zeolite using a natural polymer, soluble starch, as a mesotemplate. The synthesized samples were characterized with X-ray diffraction, Fourier transform infrared spectroscopy, field emission scanning electron microscopy, transmission electron microscopy, nitrogen sorption, ammonia temperature-programmed desorption and thermogravimetric analysis. The crystallinity and Mordenite Framework Inverted structure of the samples was confirmed by X-ray diffraction and Fourier transform infrared spectroscopy analysis. Scanning electron microscopy and transmission electron microscopy images revealed the presence of mesopores in the synthesized samples. The nitrogen adsorption/desorption results of the hierarchical samples have been found to be in agreement with the scanning electron microscopy and transmission electron microscopy results and support the development of mesoporosity. The acidity of the hierarchical zeolite was studied using ammonia temperature-programmed desorption. The thermogravimetric analysis confirmed the thermal stability of the synthesized samples up to 750 °C. The catalytic activities of the modified and unmodified zeolites were specifically tested for the esterification of acetic acid with benzyl alcohol. The results indicate that the hierarchical ZSM-5 catalyst offers a better catalytic yield (76%) than the unmodified systems. Graphic abstract © Springer Nature Switzerland AG 2019 |
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Synthesis, characterization and evaluations of micro/mesoporous ZSM-5 zeolite using starch as bio template |
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