Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction

Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynt...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Fiaz, Muhammad [verfasserIn] Athar, Muhammad [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Übergeordnetes Werk:	Enthalten in: JOM - New York, NY : Springer Science + Business Media, 1989, 72(2019), 6 vom: 25. Okt., Seite 2219-2225
Übergeordnetes Werk:	volume:72 ; year:2019 ; number:6 ; day:25 ; month:10 ; pages:2219-2225

Links:	Volltext

DOI / URN:	10.1007/s11837-019-03867-0

Katalog-ID:	SPR039748111

Internformat


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520			\|a Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode.
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912			\|a GBV_ILN_70
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912			\|a GBV_ILN_90
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912			\|a GBV_ILN_170
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912			\|a GBV_ILN_250
912			\|a GBV_ILN_281
912			\|a GBV_ILN_285
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912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_636
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912			\|a GBV_ILN_2001
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912			\|a GBV_ILN_2006
912			\|a GBV_ILN_2007
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2009
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
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912			\|a GBV_ILN_2027
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912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2037
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2039
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912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2057
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2070
912			\|a GBV_ILN_2086
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912			\|a GBV_ILN_2112
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912			\|a GBV_ILN_2116
912			\|a GBV_ILN_2118
912			\|a GBV_ILN_2119
912			\|a GBV_ILN_2122
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912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2144
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912			\|a GBV_ILN_2232
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2446
912			\|a GBV_ILN_2470
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912			\|a GBV_ILN_4112
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Indexfelder

author_variant	m f mf m a ma
matchkey_str	article:15431851:2019----::aieomeprtristicroainfrniineaslndtsnnprilsno
hierarchy_sort_str	2019
bklnumber	51.00 52.70
publishDate	2019
allfields	10.1007/s11837-019-03867-0 doi (DE-627)SPR039748111 (SPR)s11837-019-03867-0-e DE-627 ger DE-627 rakwb eng 670 ASE 51.00 bkl 52.70 bkl Fiaz, Muhammad verfasserin aut Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode. Athar, Muhammad verfasserin aut Enthalten in JOM New York, NY : Springer Science + Business Media, 1989 72(2019), 6 vom: 25. Okt., Seite 2219-2225 (DE-627)31368197X (DE-600)2002726-6 1543-1851 nnns volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225 https://dx.doi.org/10.1007/s11837-019-03867-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.00 ASE 52.70 ASE AR 72 2019 6 25 10 2219-2225
spelling	10.1007/s11837-019-03867-0 doi (DE-627)SPR039748111 (SPR)s11837-019-03867-0-e DE-627 ger DE-627 rakwb eng 670 ASE 51.00 bkl 52.70 bkl Fiaz, Muhammad verfasserin aut Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode. Athar, Muhammad verfasserin aut Enthalten in JOM New York, NY : Springer Science + Business Media, 1989 72(2019), 6 vom: 25. Okt., Seite 2219-2225 (DE-627)31368197X (DE-600)2002726-6 1543-1851 nnns volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225 https://dx.doi.org/10.1007/s11837-019-03867-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.00 ASE 52.70 ASE AR 72 2019 6 25 10 2219-2225
allfields_unstemmed	10.1007/s11837-019-03867-0 doi (DE-627)SPR039748111 (SPR)s11837-019-03867-0-e DE-627 ger DE-627 rakwb eng 670 ASE 51.00 bkl 52.70 bkl Fiaz, Muhammad verfasserin aut Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode. Athar, Muhammad verfasserin aut Enthalten in JOM New York, NY : Springer Science + Business Media, 1989 72(2019), 6 vom: 25. Okt., Seite 2219-2225 (DE-627)31368197X (DE-600)2002726-6 1543-1851 nnns volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225 https://dx.doi.org/10.1007/s11837-019-03867-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.00 ASE 52.70 ASE AR 72 2019 6 25 10 2219-2225
allfieldsGer	10.1007/s11837-019-03867-0 doi (DE-627)SPR039748111 (SPR)s11837-019-03867-0-e DE-627 ger DE-627 rakwb eng 670 ASE 51.00 bkl 52.70 bkl Fiaz, Muhammad verfasserin aut Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode. Athar, Muhammad verfasserin aut Enthalten in JOM New York, NY : Springer Science + Business Media, 1989 72(2019), 6 vom: 25. Okt., Seite 2219-2225 (DE-627)31368197X (DE-600)2002726-6 1543-1851 nnns volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225 https://dx.doi.org/10.1007/s11837-019-03867-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.00 ASE 52.70 ASE AR 72 2019 6 25 10 2219-2225
allfieldsSound	10.1007/s11837-019-03867-0 doi (DE-627)SPR039748111 (SPR)s11837-019-03867-0-e DE-627 ger DE-627 rakwb eng 670 ASE 51.00 bkl 52.70 bkl Fiaz, Muhammad verfasserin aut Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode. Athar, Muhammad verfasserin aut Enthalten in JOM New York, NY : Springer Science + Business Media, 1989 72(2019), 6 vom: 25. Okt., Seite 2219-2225 (DE-627)31368197X (DE-600)2002726-6 1543-1851 nnns volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225 https://dx.doi.org/10.1007/s11837-019-03867-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.00 ASE 52.70 ASE AR 72 2019 6 25 10 2219-2225
language	English
source	Enthalten in JOM 72(2019), 6 vom: 25. Okt., Seite 2219-2225 volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225
sourceStr	Enthalten in JOM 72(2019), 6 vom: 25. Okt., Seite 2219-2225 volume:72 year:2019 number:6 day:25 month:10 pages:2219-2225
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container_title	JOM
authorswithroles_txt_mv	Fiaz, Muhammad @@aut@@ Athar, Muhammad @@aut@@
publishDateDaySort_date	2019-10-25T00:00:00Z
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In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode.</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Athar, Muhammad</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">JOM</subfield><subfield code="d">New York, NY : Springer Science + Business Media, 1989</subfield><subfield code="g">72(2019), 6 vom: 25. 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author	Fiaz, Muhammad
spellingShingle	Fiaz, Muhammad ddc 670 bkl 51.00 bkl 52.70 Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction
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topic_title	670 ASE 51.00 bkl 52.70 bkl Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction
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title	Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction
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title_full	Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction
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title_sort	facile room-temperature in situ incorporation of transition-metal selenide (tmse) nanoparticles into mof-5 for oxygen evolution reaction
title_auth	Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction
abstract	Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode.
abstractGer	Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode.
abstract_unstemmed	Abstract Development of facile, low-cost, and highly efficient oxygen evolution reaction (OER) catalysts with excellent oxygen evolution activity and stability has been a major challenge in recent years. In this work, efficient TMSeMOF-5 catalysts were synthesized by in situ incorporation of presynthesized transition-metal selenide nanoparticles (MnSe, FeSe, CoSe, NiSe, CuSe, and ZnSe) into MOF-5 at room temperature.All the synthesized composites were successfully characterized by powder x-ray diffraction analysis, Fourier-transform infrared spectroscopy, Raman spectroscopy, scanning electron microscopy, energy-dispersive x-ray spectroscopy, elemental mapping, and ultraviolet–visible spectrophotometry. Among various TMSe@MOF-5/NF working electrodes, MnSe@MOF-5/NF showed higher OER catalytic activity, requiring an overpotential of only 170 mV to achieve a current density of 10 mA $ cm^{−2} $ in alkaline medium with a Tafel slope of 61 mV $ dec^{−1} $, which is superior to many other reported OER catalysts including state-of-the-art $ RuO_{2} $ (ƞ10 = 290 mV). Itis believed that the higher OER activity of MnSe@MOF-5/NF is due to the formation of a heterojunction from Ni of the nickel foam to the MnSe@MOF-5 at the surface of the working electrode.
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container_issue	6
title_short	Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction
url	https://dx.doi.org/10.1007/s11837-019-03867-0
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author2	Athar, Muhammad
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doi_str	10.1007/s11837-019-03867-0
up_date	2024-07-04T01:23:35.613Z
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Facile Room-Temperature In Situ Incorporation of Transition-Metal Selenide (TMSe) Nanoparticles into MOF-5 for Oxygen Evolution Reaction

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