Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams

Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of...
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Autor*in:	Biernat, Monika [verfasserIn] Dąbczyński, Paweł [verfasserIn] Biernat, Paweł [verfasserIn] Rysz, Jakub [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	PCDTBT Ternary phase diagrams Interaction parameter Swelling

Übergeordnetes Werk:	Enthalten in: Chinese Journal of Polymer Science - Chinese Chemical Society and Institute of Chemistry, CAS, 2009, 38(2020), 9 vom: 09. Juni, Seite 1025-1033
Übergeordnetes Werk:	volume:38 ; year:2020 ; number:9 ; day:09 ; month:06 ; pages:1025-1033

Links:	Volltext

DOI / URN:	10.1007/s10118-020-2424-8

Katalog-ID:	SPR040455815

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520			\|a Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams.
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allfields	10.1007/s10118-020-2424-8 doi (DE-627)SPR040455815 (SPR)s10118-020-2424-8-e DE-627 ger DE-627 rakwb eng Biernat, Monika verfasserin aut Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams. PCDTBT (dpeaa)DE-He213 Ternary phase diagrams (dpeaa)DE-He213 Interaction parameter (dpeaa)DE-He213 Swelling (dpeaa)DE-He213 Dąbczyński, Paweł verfasserin aut Biernat, Paweł verfasserin aut Rysz, Jakub verfasserin aut Enthalten in Chinese Journal of Polymer Science Chinese Chemical Society and Institute of Chemistry, CAS, 2009 38(2020), 9 vom: 09. Juni, Seite 1025-1033 (DE-627)356885143 (DE-600)2093161-X 1439-6203 nnns volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033 https://dx.doi.org/10.1007/s10118-020-2424-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 38 2020 9 09 06 1025-1033
spelling	10.1007/s10118-020-2424-8 doi (DE-627)SPR040455815 (SPR)s10118-020-2424-8-e DE-627 ger DE-627 rakwb eng Biernat, Monika verfasserin aut Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams. PCDTBT (dpeaa)DE-He213 Ternary phase diagrams (dpeaa)DE-He213 Interaction parameter (dpeaa)DE-He213 Swelling (dpeaa)DE-He213 Dąbczyński, Paweł verfasserin aut Biernat, Paweł verfasserin aut Rysz, Jakub verfasserin aut Enthalten in Chinese Journal of Polymer Science Chinese Chemical Society and Institute of Chemistry, CAS, 2009 38(2020), 9 vom: 09. Juni, Seite 1025-1033 (DE-627)356885143 (DE-600)2093161-X 1439-6203 nnns volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033 https://dx.doi.org/10.1007/s10118-020-2424-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 38 2020 9 09 06 1025-1033
allfields_unstemmed	10.1007/s10118-020-2424-8 doi (DE-627)SPR040455815 (SPR)s10118-020-2424-8-e DE-627 ger DE-627 rakwb eng Biernat, Monika verfasserin aut Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams. PCDTBT (dpeaa)DE-He213 Ternary phase diagrams (dpeaa)DE-He213 Interaction parameter (dpeaa)DE-He213 Swelling (dpeaa)DE-He213 Dąbczyński, Paweł verfasserin aut Biernat, Paweł verfasserin aut Rysz, Jakub verfasserin aut Enthalten in Chinese Journal of Polymer Science Chinese Chemical Society and Institute of Chemistry, CAS, 2009 38(2020), 9 vom: 09. Juni, Seite 1025-1033 (DE-627)356885143 (DE-600)2093161-X 1439-6203 nnns volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033 https://dx.doi.org/10.1007/s10118-020-2424-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 38 2020 9 09 06 1025-1033
allfieldsGer	10.1007/s10118-020-2424-8 doi (DE-627)SPR040455815 (SPR)s10118-020-2424-8-e DE-627 ger DE-627 rakwb eng Biernat, Monika verfasserin aut Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams. PCDTBT (dpeaa)DE-He213 Ternary phase diagrams (dpeaa)DE-He213 Interaction parameter (dpeaa)DE-He213 Swelling (dpeaa)DE-He213 Dąbczyński, Paweł verfasserin aut Biernat, Paweł verfasserin aut Rysz, Jakub verfasserin aut Enthalten in Chinese Journal of Polymer Science Chinese Chemical Society and Institute of Chemistry, CAS, 2009 38(2020), 9 vom: 09. Juni, Seite 1025-1033 (DE-627)356885143 (DE-600)2093161-X 1439-6203 nnns volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033 https://dx.doi.org/10.1007/s10118-020-2424-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 38 2020 9 09 06 1025-1033
allfieldsSound	10.1007/s10118-020-2424-8 doi (DE-627)SPR040455815 (SPR)s10118-020-2424-8-e DE-627 ger DE-627 rakwb eng Biernat, Monika verfasserin aut Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams. PCDTBT (dpeaa)DE-He213 Ternary phase diagrams (dpeaa)DE-He213 Interaction parameter (dpeaa)DE-He213 Swelling (dpeaa)DE-He213 Dąbczyński, Paweł verfasserin aut Biernat, Paweł verfasserin aut Rysz, Jakub verfasserin aut Enthalten in Chinese Journal of Polymer Science Chinese Chemical Society and Institute of Chemistry, CAS, 2009 38(2020), 9 vom: 09. Juni, Seite 1025-1033 (DE-627)356885143 (DE-600)2093161-X 1439-6203 nnns volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033 https://dx.doi.org/10.1007/s10118-020-2424-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 38 2020 9 09 06 1025-1033
language	English
source	Enthalten in Chinese Journal of Polymer Science 38(2020), 9 vom: 09. Juni, Seite 1025-1033 volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033
sourceStr	Enthalten in Chinese Journal of Polymer Science 38(2020), 9 vom: 09. Juni, Seite 1025-1033 volume:38 year:2020 number:9 day:09 month:06 pages:1025-1033
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	PCDTBT Ternary phase diagrams Interaction parameter Swelling
isfreeaccess_bool	false
container_title	Chinese Journal of Polymer Science
authorswithroles_txt_mv	Biernat, Monika @@aut@@ Dąbczyński, Paweł @@aut@@ Biernat, Paweł @@aut@@ Rysz, Jakub @@aut@@
publishDateDaySort_date	2020-06-09T00:00:00Z
hierarchy_top_id	356885143
id	SPR040455815
language_de	englisch
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author	Biernat, Monika
spellingShingle	Biernat, Monika misc PCDTBT misc Ternary phase diagrams misc Interaction parameter misc Swelling Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams
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topic_title	Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams PCDTBT (dpeaa)DE-He213 Ternary phase diagrams (dpeaa)DE-He213 Interaction parameter (dpeaa)DE-He213 Swelling (dpeaa)DE-He213
topic	misc PCDTBT misc Ternary phase diagrams misc Interaction parameter misc Swelling
topic_unstemmed	misc PCDTBT misc Ternary phase diagrams misc Interaction parameter misc Swelling
topic_browse	misc PCDTBT misc Ternary phase diagrams misc Interaction parameter misc Swelling
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title	Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams
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title_full	Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams
author_sort	Biernat, Monika
journal	Chinese Journal of Polymer Science
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author_browse	Biernat, Monika Dąbczyński, Paweł Biernat, Paweł Rysz, Jakub
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author-letter	Biernat, Monika
doi_str_mv	10.1007/s10118-020-2424-8
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title_sort	phase separation in pcdtbt:pcbm blends: from flory-huggins interaction parameters to ternary phase diagrams
title_auth	Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams
abstract	Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams.
abstractGer	Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams.
abstract_unstemmed	Abstract The substantial increase in the efficiency of organic solar cells achieved in recent years would not have been possible without work on the synthesis of new materials and understanding the relationship between the morphology and performance of organic photovoltaic devices. The structure of solvent-cast active layers is a result of phase separation in mixtures of donor and acceptor components. To a large extent, this process depends on the interactions between the components of the mixture. Here, we present a systematic analysis of the morphology of poly[N-9′-heptadecanyl-2,7-carbazole-alt-5,5-(4′,7′-di-2-thienyl-2′,1′,3′-benzothiadiazole)] (PCDTBT) and [6,6]-phenyl-$ C_{71} $-butyricacid methyl ester (PC70BM) films in terms of the ternary phase diagram. The interaction parameters between PCDTBT and four different solvents, namely chloroform, chlorobenzene, o-dichlorobenzene, and toluene, were estimated based on swelling experiments. Based on these values, ternary phase diagrams of PCDTBT:PC70BM in different solvents were calculated. The morphology of spin-coated films with different blend ratios cast from different solvents is discussed in terms of the obtained phase diagrams.
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title_short	Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams
url	https://dx.doi.org/10.1007/s10118-020-2424-8
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author2	Dąbczyński, Paweł Biernat, Paweł Rysz, Jakub
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Phase Separation in PCDTBT:PCBM Blends: from Flory-Huggins Interaction Parameters to Ternary Phase Diagrams

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