Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction
Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
He, Xinping [verfasserIn] Ruan, Shuai [verfasserIn] Chen, Yun [verfasserIn] Zhang, Jun [verfasserIn] Liang, Chu [verfasserIn] Huang, Hui [verfasserIn] Gan, Yongping [verfasserIn] Zhang, Wenkui [verfasserIn] Xia, Yang [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Ionics - Berlin : Springer, 1995, 26(2020), 10 vom: 25. Juni, Seite 5065-5073 |
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| Übergeordnetes Werk: |
volume:26 ; year:2020 ; number:10 ; day:25 ; month:06 ; pages:5065-5073 |
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| DOI / URN: |
10.1007/s11581-020-03666-7 |
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| Katalog-ID: |
SPR040988082 |
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| 245 | 1 | 0 | |a Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction |
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| 520 | |a Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. | ||
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| 650 | 4 | |a Oxygen reduction reaction |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Fuel cells |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Ruan, Shuai |e verfasserin |4 aut | |
| 700 | 1 | |a Chen, Yun |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Jun |e verfasserin |4 aut | |
| 700 | 1 | |a Liang, Chu |e verfasserin |4 aut | |
| 700 | 1 | |a Huang, Hui |e verfasserin |4 aut | |
| 700 | 1 | |a Gan, Yongping |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Wenkui |e verfasserin |4 aut | |
| 700 | 1 | |a Xia, Yang |e verfasserin |4 aut | |
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10.1007/s11581-020-03666-7 doi (DE-627)SPR040988082 (SPR)s11581-020-03666-7-e DE-627 ger DE-627 rakwb eng 530 ASE 33.30 bkl 35.10 bkl He, Xinping verfasserin aut Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. Metal-doping (dpeaa)DE-He213 Nanocomposite (dpeaa)DE-He213 Catalyst (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Fuel cells (dpeaa)DE-He213 Ruan, Shuai verfasserin aut Chen, Yun verfasserin aut Zhang, Jun verfasserin aut Liang, Chu verfasserin aut Huang, Hui verfasserin aut Gan, Yongping verfasserin aut Zhang, Wenkui verfasserin aut Xia, Yang verfasserin aut Enthalten in Ionics Berlin : Springer, 1995 26(2020), 10 vom: 25. Juni, Seite 5065-5073 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:26 year:2020 number:10 day:25 month:06 pages:5065-5073 https://dx.doi.org/10.1007/s11581-020-03666-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.30 ASE 35.10 ASE AR 26 2020 10 25 06 5065-5073 |
| spelling |
10.1007/s11581-020-03666-7 doi (DE-627)SPR040988082 (SPR)s11581-020-03666-7-e DE-627 ger DE-627 rakwb eng 530 ASE 33.30 bkl 35.10 bkl He, Xinping verfasserin aut Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. Metal-doping (dpeaa)DE-He213 Nanocomposite (dpeaa)DE-He213 Catalyst (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Fuel cells (dpeaa)DE-He213 Ruan, Shuai verfasserin aut Chen, Yun verfasserin aut Zhang, Jun verfasserin aut Liang, Chu verfasserin aut Huang, Hui verfasserin aut Gan, Yongping verfasserin aut Zhang, Wenkui verfasserin aut Xia, Yang verfasserin aut Enthalten in Ionics Berlin : Springer, 1995 26(2020), 10 vom: 25. Juni, Seite 5065-5073 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:26 year:2020 number:10 day:25 month:06 pages:5065-5073 https://dx.doi.org/10.1007/s11581-020-03666-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.30 ASE 35.10 ASE AR 26 2020 10 25 06 5065-5073 |
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10.1007/s11581-020-03666-7 doi (DE-627)SPR040988082 (SPR)s11581-020-03666-7-e DE-627 ger DE-627 rakwb eng 530 ASE 33.30 bkl 35.10 bkl He, Xinping verfasserin aut Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. Metal-doping (dpeaa)DE-He213 Nanocomposite (dpeaa)DE-He213 Catalyst (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Fuel cells (dpeaa)DE-He213 Ruan, Shuai verfasserin aut Chen, Yun verfasserin aut Zhang, Jun verfasserin aut Liang, Chu verfasserin aut Huang, Hui verfasserin aut Gan, Yongping verfasserin aut Zhang, Wenkui verfasserin aut Xia, Yang verfasserin aut Enthalten in Ionics Berlin : Springer, 1995 26(2020), 10 vom: 25. Juni, Seite 5065-5073 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:26 year:2020 number:10 day:25 month:06 pages:5065-5073 https://dx.doi.org/10.1007/s11581-020-03666-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.30 ASE 35.10 ASE AR 26 2020 10 25 06 5065-5073 |
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10.1007/s11581-020-03666-7 doi (DE-627)SPR040988082 (SPR)s11581-020-03666-7-e DE-627 ger DE-627 rakwb eng 530 ASE 33.30 bkl 35.10 bkl He, Xinping verfasserin aut Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. Metal-doping (dpeaa)DE-He213 Nanocomposite (dpeaa)DE-He213 Catalyst (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Fuel cells (dpeaa)DE-He213 Ruan, Shuai verfasserin aut Chen, Yun verfasserin aut Zhang, Jun verfasserin aut Liang, Chu verfasserin aut Huang, Hui verfasserin aut Gan, Yongping verfasserin aut Zhang, Wenkui verfasserin aut Xia, Yang verfasserin aut Enthalten in Ionics Berlin : Springer, 1995 26(2020), 10 vom: 25. Juni, Seite 5065-5073 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:26 year:2020 number:10 day:25 month:06 pages:5065-5073 https://dx.doi.org/10.1007/s11581-020-03666-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.30 ASE 35.10 ASE AR 26 2020 10 25 06 5065-5073 |
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10.1007/s11581-020-03666-7 doi (DE-627)SPR040988082 (SPR)s11581-020-03666-7-e DE-627 ger DE-627 rakwb eng 530 ASE 33.30 bkl 35.10 bkl He, Xinping verfasserin aut Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. Metal-doping (dpeaa)DE-He213 Nanocomposite (dpeaa)DE-He213 Catalyst (dpeaa)DE-He213 Oxygen reduction reaction (dpeaa)DE-He213 Fuel cells (dpeaa)DE-He213 Ruan, Shuai verfasserin aut Chen, Yun verfasserin aut Zhang, Jun verfasserin aut Liang, Chu verfasserin aut Huang, Hui verfasserin aut Gan, Yongping verfasserin aut Zhang, Wenkui verfasserin aut Xia, Yang verfasserin aut Enthalten in Ionics Berlin : Springer, 1995 26(2020), 10 vom: 25. Juni, Seite 5065-5073 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:26 year:2020 number:10 day:25 month:06 pages:5065-5073 https://dx.doi.org/10.1007/s11581-020-03666-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.30 ASE 35.10 ASE AR 26 2020 10 25 06 5065-5073 |
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He, Xinping @@aut@@ Ruan, Shuai @@aut@@ Chen, Yun @@aut@@ Zhang, Jun @@aut@@ Liang, Chu @@aut@@ Huang, Hui @@aut@@ Gan, Yongping @@aut@@ Zhang, Wenkui @@aut@@ Xia, Yang @@aut@@ |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR040988082</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20220111080256.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">201007s2020 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s11581-020-03666-7</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR040988082</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s11581-020-03666-7-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">530</subfield><subfield code="q">ASE</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">33.30</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">35.10</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">He, Xinping</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2020</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. 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He, Xinping |
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rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction |
| title_auth |
Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction |
| abstract |
Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. |
| abstractGer |
Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. |
| abstract_unstemmed |
Abstract The key to sustainable energy application is the rational utilization of abundant materials on the earth. Fe, Co, and Cu theoretically exhibit high oxygen reduction capability close to Pt. However, their high diffusion behaviors make it difficult to homogeneously incorporate with carbon at elevated fabrication temperature. Here, polyaniline is developed an incorporated frame to realize the homodisperse of Fe, Co, or Cu. Three efficient oxygen reduction catalysts, including Fe-polyaniline/carbon (Fe-N/C), Co-N/C, and Cu-N/C are synthesized by a three-step method combining polymerization, complexation, and pyrolysis. All catalysts with metal doping reveal high catalytic activity, good cyclic stability, and the activity varies with different doping metal. The Fe-doped catalyst exhibits the best oxygen reduction ability with onset and half-wave potentials of − 104 mV and − 199.5 mV. Furthermore, the influence of complexation time and the pyrolysis temperature on the oxygen reduction activity are also studied systematically. These interesting discoveries may contribute to provide important ideas to oxygen reduction catalysts. |
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Rational design of highly efficient metal-polyaniline/carbon cloth catalyst towards enhanced oxygen reduction reaction |
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https://dx.doi.org/10.1007/s11581-020-03666-7 |
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Ruan, Shuai Chen, Yun Zhang, Jun Liang, Chu Huang, Hui Gan, Yongping Zhang, Wenkui Xia, Yang |
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Ruan, Shuai Chen, Yun Zhang, Jun Liang, Chu Huang, Hui Gan, Yongping Zhang, Wenkui Xia, Yang |
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| score |
7.4015436 |