Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications
Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Lyons, Leslie J. [verfasserIn] Beecher, Scott [verfasserIn] Cunningham, Evan [verfasserIn] Derrah, Tom [verfasserIn] Su, Shengyi [verfasserIn] Zhu, Junmian [verfasserIn] Usrey, Monica [verfasserIn] Peña-Hueso, Adrián [verfasserIn] Johnson, Tobias [verfasserIn] West, Robert [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Übergeordnetes Werk: |
Enthalten in: MRS communications - Berlin : Springer, 2011, 9(2019), 3 vom: Sept., Seite 985-991 |
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| Übergeordnetes Werk: |
volume:9 ; year:2019 ; number:3 ; month:09 ; pages:985-991 |
| Links: |
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| DOI / URN: |
10.1557/mrc.2019.112 |
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| Katalog-ID: |
SPR042404843 |
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| 520 | |a Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. | ||
| 700 | 1 | |a Beecher, Scott |e verfasserin |4 aut | |
| 700 | 1 | |a Cunningham, Evan |e verfasserin |4 aut | |
| 700 | 1 | |a Derrah, Tom |e verfasserin |4 aut | |
| 700 | 1 | |a Su, Shengyi |e verfasserin |4 aut | |
| 700 | 1 | |a Zhu, Junmian |e verfasserin |4 aut | |
| 700 | 1 | |a Usrey, Monica |e verfasserin |4 aut | |
| 700 | 1 | |a Peña-Hueso, Adrián |e verfasserin |4 aut | |
| 700 | 1 | |a Johnson, Tobias |e verfasserin |4 aut | |
| 700 | 1 | |a West, Robert |e verfasserin |4 aut | |
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10.1557/mrc.2019.112 doi (DE-627)SPR042404843 (DE-599)SPRmrc.2019.112-e (SPR)mrc.2019.112-e DE-627 ger DE-627 rakwb eng 670 ASE Lyons, Leslie J. verfasserin aut Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. Beecher, Scott verfasserin aut Cunningham, Evan verfasserin aut Derrah, Tom verfasserin aut Su, Shengyi verfasserin aut Zhu, Junmian verfasserin aut Usrey, Monica verfasserin aut Peña-Hueso, Adrián verfasserin aut Johnson, Tobias verfasserin aut West, Robert verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 9(2019), 3 vom: Sept., Seite 985-991 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:9 year:2019 number:3 month:09 pages:985-991 https://dx.doi.org/10.1557/mrc.2019.112 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2107 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2145 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 9 2019 3 09 985-991 |
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10.1557/mrc.2019.112 doi (DE-627)SPR042404843 (DE-599)SPRmrc.2019.112-e (SPR)mrc.2019.112-e DE-627 ger DE-627 rakwb eng 670 ASE Lyons, Leslie J. verfasserin aut Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. Beecher, Scott verfasserin aut Cunningham, Evan verfasserin aut Derrah, Tom verfasserin aut Su, Shengyi verfasserin aut Zhu, Junmian verfasserin aut Usrey, Monica verfasserin aut Peña-Hueso, Adrián verfasserin aut Johnson, Tobias verfasserin aut West, Robert verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 9(2019), 3 vom: Sept., Seite 985-991 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:9 year:2019 number:3 month:09 pages:985-991 https://dx.doi.org/10.1557/mrc.2019.112 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2107 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2145 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 9 2019 3 09 985-991 |
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10.1557/mrc.2019.112 doi (DE-627)SPR042404843 (DE-599)SPRmrc.2019.112-e (SPR)mrc.2019.112-e DE-627 ger DE-627 rakwb eng 670 ASE Lyons, Leslie J. verfasserin aut Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. Beecher, Scott verfasserin aut Cunningham, Evan verfasserin aut Derrah, Tom verfasserin aut Su, Shengyi verfasserin aut Zhu, Junmian verfasserin aut Usrey, Monica verfasserin aut Peña-Hueso, Adrián verfasserin aut Johnson, Tobias verfasserin aut West, Robert verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 9(2019), 3 vom: Sept., Seite 985-991 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:9 year:2019 number:3 month:09 pages:985-991 https://dx.doi.org/10.1557/mrc.2019.112 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2107 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2145 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 9 2019 3 09 985-991 |
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10.1557/mrc.2019.112 doi (DE-627)SPR042404843 (DE-599)SPRmrc.2019.112-e (SPR)mrc.2019.112-e DE-627 ger DE-627 rakwb eng 670 ASE Lyons, Leslie J. verfasserin aut Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. Beecher, Scott verfasserin aut Cunningham, Evan verfasserin aut Derrah, Tom verfasserin aut Su, Shengyi verfasserin aut Zhu, Junmian verfasserin aut Usrey, Monica verfasserin aut Peña-Hueso, Adrián verfasserin aut Johnson, Tobias verfasserin aut West, Robert verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 9(2019), 3 vom: Sept., Seite 985-991 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:9 year:2019 number:3 month:09 pages:985-991 https://dx.doi.org/10.1557/mrc.2019.112 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2107 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2145 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 9 2019 3 09 985-991 |
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10.1557/mrc.2019.112 doi (DE-627)SPR042404843 (DE-599)SPRmrc.2019.112-e (SPR)mrc.2019.112-e DE-627 ger DE-627 rakwb eng 670 ASE Lyons, Leslie J. verfasserin aut Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications 2019 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. Beecher, Scott verfasserin aut Cunningham, Evan verfasserin aut Derrah, Tom verfasserin aut Su, Shengyi verfasserin aut Zhu, Junmian verfasserin aut Usrey, Monica verfasserin aut Peña-Hueso, Adrián verfasserin aut Johnson, Tobias verfasserin aut West, Robert verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 9(2019), 3 vom: Sept., Seite 985-991 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:9 year:2019 number:3 month:09 pages:985-991 https://dx.doi.org/10.1557/mrc.2019.112 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2107 GBV_ILN_2110 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2145 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 9 2019 3 09 985-991 |
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Lyons, Leslie J. @@aut@@ Beecher, Scott @@aut@@ Cunningham, Evan @@aut@@ Derrah, Tom @@aut@@ Su, Shengyi @@aut@@ Zhu, Junmian @@aut@@ Usrey, Monica @@aut@@ Peña-Hueso, Adrián @@aut@@ Johnson, Tobias @@aut@@ West, Robert @@aut@@ |
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Lyons, Leslie J. |
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Lyons, Leslie J. ddc 670 Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
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670 ASE Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
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Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
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Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
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Lyons, Leslie J. Beecher, Scott Cunningham, Evan Derrah, Tom Su, Shengyi Zhu, Junmian Usrey, Monica Peña-Hueso, Adrián Johnson, Tobias West, Robert |
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enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
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Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
| abstract |
Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. |
| abstractGer |
Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. |
| abstract_unstemmed |
Abstract The authors report on 7Li, 19F, and 1H pulsed field gradient NMR measurements of 26 organosilyl nitrile solvent-based electrolytes of either lithium bis(trifluorosulfonyl)imide (LiTFSI) or lithium hexafluorophosphate. Lithium transport numbers (as high as 0.50) were measured and are highest in the LiTFSI electrolytes. The authors also report on solvent blend electrolytes of fluoroorganosilyl (FOS) nitrile solvent mixed with ethylene carbonate (EC) and diethyl carbonate. Solvent diffusion measurements on an electrolyte with 6% FOS suggest both the FOS and EC solvate the lithium cation. By comparing lithium transport and transference numbers, The authors find less ion pairing in FOS nitrile carbonate blend electrolytes and difluoroorganosilyl nitrile electrolytes. |
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Enhanced lithium-ion transport in organosilyl electrolytes for lithium-ion battery applications |
| url |
https://dx.doi.org/10.1557/mrc.2019.112 |
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| author2 |
Beecher, Scott Cunningham, Evan Derrah, Tom Su, Shengyi Zhu, Junmian Usrey, Monica Peña-Hueso, Adrián Johnson, Tobias West, Robert |
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Beecher, Scott Cunningham, Evan Derrah, Tom Su, Shengyi Zhu, Junmian Usrey, Monica Peña-Hueso, Adrián Johnson, Tobias West, Robert |
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| doi_str |
10.1557/mrc.2019.112 |
| up_date |
2024-07-04T01:54:48.218Z |
| _version_ |
1803611629914423296 |
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