Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction
Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to local...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Valério, Adriana [verfasserIn] Penacchio, Rafaela F. S. [verfasserIn] Estradiote, Maurício B. [verfasserIn] Cantarino, Marli R. [verfasserIn] Garcia, Fernando A. [verfasserIn] Morelhão, Sérgio L. [verfasserIn] Rafter, Niamh [verfasserIn] Kycia, Stefan W. [verfasserIn] Calligaris, Guilherme A. [verfasserIn] Remédios, Cláudio M. R. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020 |
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| Übergeordnetes Werk: |
Enthalten in: MRS communications - Berlin : Springer, 2011, 10(2020), 2 vom: Juni, Seite 265-271 |
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| Übergeordnetes Werk: |
volume:10 ; year:2020 ; number:2 ; month:06 ; pages:265-271 |
| Links: |
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| DOI / URN: |
10.1557/mrc.2020.37 |
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| Katalog-ID: |
SPR04244506X |
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| 245 | 1 | 0 | |a Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction |
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| 520 | |a Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. | ||
| 700 | 1 | |a Penacchio, Rafaela F. S. |e verfasserin |4 aut | |
| 700 | 1 | |a Estradiote, Maurício B. |e verfasserin |4 aut | |
| 700 | 1 | |a Cantarino, Marli R. |e verfasserin |4 aut | |
| 700 | 1 | |a Garcia, Fernando A. |e verfasserin |4 aut | |
| 700 | 1 | |a Morelhão, Sérgio L. |e verfasserin |4 aut | |
| 700 | 1 | |a Rafter, Niamh |e verfasserin |4 aut | |
| 700 | 1 | |a Kycia, Stefan W. |e verfasserin |4 aut | |
| 700 | 1 | |a Calligaris, Guilherme A. |e verfasserin |4 aut | |
| 700 | 1 | |a Remédios, Cláudio M. R. |e verfasserin |4 aut | |
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10.1557/mrc.2020.37 doi (DE-627)SPR04244506X (DE-599)SPRmrc.2020.37-e (SPR)mrc.2020.37-e DE-627 ger DE-627 rakwb eng 670 ASE Valério, Adriana verfasserin aut Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. Penacchio, Rafaela F. S. verfasserin aut Estradiote, Maurício B. verfasserin aut Cantarino, Marli R. verfasserin aut Garcia, Fernando A. verfasserin aut Morelhão, Sérgio L. verfasserin aut Rafter, Niamh verfasserin aut Kycia, Stefan W. verfasserin aut Calligaris, Guilherme A. verfasserin aut Remédios, Cláudio M. R. verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 10(2020), 2 vom: Juni, Seite 265-271 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:10 year:2020 number:2 month:06 pages:265-271 https://dx.doi.org/10.1557/mrc.2020.37 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2145 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 10 2020 2 06 265-271 |
| spelling |
10.1557/mrc.2020.37 doi (DE-627)SPR04244506X (DE-599)SPRmrc.2020.37-e (SPR)mrc.2020.37-e DE-627 ger DE-627 rakwb eng 670 ASE Valério, Adriana verfasserin aut Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. Penacchio, Rafaela F. S. verfasserin aut Estradiote, Maurício B. verfasserin aut Cantarino, Marli R. verfasserin aut Garcia, Fernando A. verfasserin aut Morelhão, Sérgio L. verfasserin aut Rafter, Niamh verfasserin aut Kycia, Stefan W. verfasserin aut Calligaris, Guilherme A. verfasserin aut Remédios, Cláudio M. R. verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 10(2020), 2 vom: Juni, Seite 265-271 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:10 year:2020 number:2 month:06 pages:265-271 https://dx.doi.org/10.1557/mrc.2020.37 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2145 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 10 2020 2 06 265-271 |
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10.1557/mrc.2020.37 doi (DE-627)SPR04244506X (DE-599)SPRmrc.2020.37-e (SPR)mrc.2020.37-e DE-627 ger DE-627 rakwb eng 670 ASE Valério, Adriana verfasserin aut Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. Penacchio, Rafaela F. S. verfasserin aut Estradiote, Maurício B. verfasserin aut Cantarino, Marli R. verfasserin aut Garcia, Fernando A. verfasserin aut Morelhão, Sérgio L. verfasserin aut Rafter, Niamh verfasserin aut Kycia, Stefan W. verfasserin aut Calligaris, Guilherme A. verfasserin aut Remédios, Cláudio M. R. verfasserin aut Enthalten in MRS communications Berlin : Springer, 2011 10(2020), 2 vom: Juni, Seite 265-271 (DE-627)683366432 (DE-600)2645443-9 2159-6867 nnns volume:10 year:2020 number:2 month:06 pages:265-271 https://dx.doi.org/10.1557/mrc.2020.37 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_647 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2036 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2088 GBV_ILN_2089 GBV_ILN_2093 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2145 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2158 GBV_ILN_2190 GBV_ILN_2193 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_2924 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4346 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 GBV_ILN_4753 AR 10 2020 2 06 265-271 |
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Valério, Adriana @@aut@@ Penacchio, Rafaela F. S. @@aut@@ Estradiote, Maurício B. @@aut@@ Cantarino, Marli R. @@aut@@ Garcia, Fernando A. @@aut@@ Morelhão, Sérgio L. @@aut@@ Rafter, Niamh @@aut@@ Kycia, Stefan W. @@aut@@ Calligaris, Guilherme A. @@aut@@ Remédios, Cláudio M. R. @@aut@@ |
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Valério, Adriana ddc 670 Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction |
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670 ASE Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction |
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Valério, Adriana Penacchio, Rafaela F. S. Estradiote, Maurício B. Cantarino, Marli R. Garcia, Fernando A. Morelhão, Sérgio L. Rafter, Niamh Kycia, Stefan W. Calligaris, Guilherme A. Remédios, Cláudio M. R. |
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Elektronische Aufsätze |
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Valério, Adriana |
| doi_str_mv |
10.1557/mrc.2020.37 |
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verfasserin |
| title_sort |
phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction |
| title_auth |
Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction |
| abstract |
Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. |
| abstractGer |
Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. |
| abstract_unstemmed |
Abstract Engineering of thermoelectric materials requires an understanding of thermal conduction by lattice and electronic degrees of freedom. Filled skutterudites denote a large family of materials suitable for thermoelectric applications where reduced lattice thermal conduction attributed to localized low-frequency vibrations (rattling) of filler cations inside large cages of the structure. In this work, a multi-wavelength method of exploiting x-ray dynamical diffraction in single crystals of CeFe4P12 is presented and applied to resolve the atomic amplitudes of vibrations. The results suggest that the vibrational dynamics of the whole filler-cage system is the actual active mechanism behind the optimization of thermoelectric properties. |
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| container_issue |
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| title_short |
Phonon scattering mechanism in thermoelectric materials revised via resonant x-ray dynamical diffraction |
| url |
https://dx.doi.org/10.1557/mrc.2020.37 |
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| author2 |
Penacchio, Rafaela F. S. Estradiote, Maurício B. Cantarino, Marli R. Garcia, Fernando A. Morelhão, Sérgio L. Rafter, Niamh Kycia, Stefan W. Calligaris, Guilherme A. Remédios, Cláudio M. R. |
| author2Str |
Penacchio, Rafaela F. S. Estradiote, Maurício B. Cantarino, Marli R. Garcia, Fernando A. Morelhão, Sérgio L. Rafter, Niamh Kycia, Stefan W. Calligaris, Guilherme A. Remédios, Cláudio M. R. |
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| doi_str |
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| up_date |
2024-07-04T02:02:52.494Z |
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1803612137713565696 |
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| score |
7.4000645 |