Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis
Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-sup...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Yang, Shu [verfasserIn] Zhang, Lei [verfasserIn] Shao, Changlu [verfasserIn] Li, Xinghua [verfasserIn] Li, Xiaowei [verfasserIn] Liu, Shuai [verfasserIn] Tao, Ran [verfasserIn] Liu, Yichun [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of sol gel science and technology - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993, 97(2021), 3 vom: 01. Feb., Seite 610-621 |
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| Übergeordnetes Werk: |
volume:97 ; year:2021 ; number:3 ; day:01 ; month:02 ; pages:610-621 |
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| DOI / URN: |
10.1007/s10971-020-05453-2 |
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| Katalog-ID: |
SPR043443389 |
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| 520 | |a Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. | ||
| 520 | |a Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. | ||
| 650 | 4 | |a Electrospun nanofibers |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Flexibility |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a BiOCl/BiOI heterojunctions |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a In situ synthesis |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Floating photocatalysis |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Zhang, Lei |e verfasserin |4 aut | |
| 700 | 1 | |a Shao, Changlu |e verfasserin |4 aut | |
| 700 | 1 | |a Li, Xinghua |e verfasserin |4 aut | |
| 700 | 1 | |a Li, Xiaowei |e verfasserin |4 aut | |
| 700 | 1 | |a Liu, Shuai |e verfasserin |4 aut | |
| 700 | 1 | |a Tao, Ran |e verfasserin |4 aut | |
| 700 | 1 | |a Liu, Yichun |e verfasserin |4 aut | |
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10.1007/s10971-020-05453-2 doi (DE-627)SPR043443389 (DE-599)SPRs10971-020-05453-2-e (SPR)s10971-020-05453-2-e DE-627 ger DE-627 rakwb eng 600 670 ASE 35.18 bkl 51.60 bkl Yang, Shu verfasserin aut Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. Electrospun nanofibers (dpeaa)DE-He213 Flexibility (dpeaa)DE-He213 BiOCl/BiOI heterojunctions (dpeaa)DE-He213 In situ synthesis (dpeaa)DE-He213 Floating photocatalysis (dpeaa)DE-He213 Zhang, Lei verfasserin aut Shao, Changlu verfasserin aut Li, Xinghua verfasserin aut Li, Xiaowei verfasserin aut Liu, Shuai verfasserin aut Tao, Ran verfasserin aut Liu, Yichun verfasserin aut Enthalten in Journal of sol gel science and technology Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993 97(2021), 3 vom: 01. Feb., Seite 610-621 (DE-627)268757607 (DE-600)1472726-2 1573-4846 nnns volume:97 year:2021 number:3 day:01 month:02 pages:610-621 https://dx.doi.org/10.1007/s10971-020-05453-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 ASE 51.60 ASE AR 97 2021 3 01 02 610-621 |
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10.1007/s10971-020-05453-2 doi (DE-627)SPR043443389 (DE-599)SPRs10971-020-05453-2-e (SPR)s10971-020-05453-2-e DE-627 ger DE-627 rakwb eng 600 670 ASE 35.18 bkl 51.60 bkl Yang, Shu verfasserin aut Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. Electrospun nanofibers (dpeaa)DE-He213 Flexibility (dpeaa)DE-He213 BiOCl/BiOI heterojunctions (dpeaa)DE-He213 In situ synthesis (dpeaa)DE-He213 Floating photocatalysis (dpeaa)DE-He213 Zhang, Lei verfasserin aut Shao, Changlu verfasserin aut Li, Xinghua verfasserin aut Li, Xiaowei verfasserin aut Liu, Shuai verfasserin aut Tao, Ran verfasserin aut Liu, Yichun verfasserin aut Enthalten in Journal of sol gel science and technology Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993 97(2021), 3 vom: 01. Feb., Seite 610-621 (DE-627)268757607 (DE-600)1472726-2 1573-4846 nnns volume:97 year:2021 number:3 day:01 month:02 pages:610-621 https://dx.doi.org/10.1007/s10971-020-05453-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 ASE 51.60 ASE AR 97 2021 3 01 02 610-621 |
| allfields_unstemmed |
10.1007/s10971-020-05453-2 doi (DE-627)SPR043443389 (DE-599)SPRs10971-020-05453-2-e (SPR)s10971-020-05453-2-e DE-627 ger DE-627 rakwb eng 600 670 ASE 35.18 bkl 51.60 bkl Yang, Shu verfasserin aut Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. Electrospun nanofibers (dpeaa)DE-He213 Flexibility (dpeaa)DE-He213 BiOCl/BiOI heterojunctions (dpeaa)DE-He213 In situ synthesis (dpeaa)DE-He213 Floating photocatalysis (dpeaa)DE-He213 Zhang, Lei verfasserin aut Shao, Changlu verfasserin aut Li, Xinghua verfasserin aut Li, Xiaowei verfasserin aut Liu, Shuai verfasserin aut Tao, Ran verfasserin aut Liu, Yichun verfasserin aut Enthalten in Journal of sol gel science and technology Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993 97(2021), 3 vom: 01. Feb., Seite 610-621 (DE-627)268757607 (DE-600)1472726-2 1573-4846 nnns volume:97 year:2021 number:3 day:01 month:02 pages:610-621 https://dx.doi.org/10.1007/s10971-020-05453-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 ASE 51.60 ASE AR 97 2021 3 01 02 610-621 |
| allfieldsGer |
10.1007/s10971-020-05453-2 doi (DE-627)SPR043443389 (DE-599)SPRs10971-020-05453-2-e (SPR)s10971-020-05453-2-e DE-627 ger DE-627 rakwb eng 600 670 ASE 35.18 bkl 51.60 bkl Yang, Shu verfasserin aut Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. Electrospun nanofibers (dpeaa)DE-He213 Flexibility (dpeaa)DE-He213 BiOCl/BiOI heterojunctions (dpeaa)DE-He213 In situ synthesis (dpeaa)DE-He213 Floating photocatalysis (dpeaa)DE-He213 Zhang, Lei verfasserin aut Shao, Changlu verfasserin aut Li, Xinghua verfasserin aut Li, Xiaowei verfasserin aut Liu, Shuai verfasserin aut Tao, Ran verfasserin aut Liu, Yichun verfasserin aut Enthalten in Journal of sol gel science and technology Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993 97(2021), 3 vom: 01. Feb., Seite 610-621 (DE-627)268757607 (DE-600)1472726-2 1573-4846 nnns volume:97 year:2021 number:3 day:01 month:02 pages:610-621 https://dx.doi.org/10.1007/s10971-020-05453-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 ASE 51.60 ASE AR 97 2021 3 01 02 610-621 |
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10.1007/s10971-020-05453-2 doi (DE-627)SPR043443389 (DE-599)SPRs10971-020-05453-2-e (SPR)s10971-020-05453-2-e DE-627 ger DE-627 rakwb eng 600 670 ASE 35.18 bkl 51.60 bkl Yang, Shu verfasserin aut Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. Electrospun nanofibers (dpeaa)DE-He213 Flexibility (dpeaa)DE-He213 BiOCl/BiOI heterojunctions (dpeaa)DE-He213 In situ synthesis (dpeaa)DE-He213 Floating photocatalysis (dpeaa)DE-He213 Zhang, Lei verfasserin aut Shao, Changlu verfasserin aut Li, Xinghua verfasserin aut Li, Xiaowei verfasserin aut Liu, Shuai verfasserin aut Tao, Ran verfasserin aut Liu, Yichun verfasserin aut Enthalten in Journal of sol gel science and technology Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993 97(2021), 3 vom: 01. Feb., Seite 610-621 (DE-627)268757607 (DE-600)1472726-2 1573-4846 nnns volume:97 year:2021 number:3 day:01 month:02 pages:610-621 https://dx.doi.org/10.1007/s10971-020-05453-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 ASE 51.60 ASE AR 97 2021 3 01 02 610-621 |
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Enthalten in Journal of sol gel science and technology 97(2021), 3 vom: 01. Feb., Seite 610-621 volume:97 year:2021 number:3 day:01 month:02 pages:610-621 |
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Enthalten in Journal of sol gel science and technology 97(2021), 3 vom: 01. Feb., Seite 610-621 volume:97 year:2021 number:3 day:01 month:02 pages:610-621 |
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Article |
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findex.gbv.de |
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Electrospun nanofibers Flexibility BiOCl/BiOI heterojunctions In situ synthesis Floating photocatalysis |
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600 |
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false |
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Journal of sol gel science and technology |
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Yang, Shu @@aut@@ Zhang, Lei @@aut@@ Shao, Changlu @@aut@@ Li, Xinghua @@aut@@ Li, Xiaowei @@aut@@ Liu, Shuai @@aut@@ Tao, Ran @@aut@@ Liu, Yichun @@aut@@ |
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2021-02-01T00:00:00Z |
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SPR043443389 |
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|
| author |
Yang, Shu |
| spellingShingle |
Yang, Shu ddc 600 bkl 35.18 bkl 51.60 misc Electrospun nanofibers misc Flexibility misc BiOCl/BiOI heterojunctions misc In situ synthesis misc Floating photocatalysis Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis |
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Yang, Shu |
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600 - Technology 670 - Manufacturing |
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600 670 ASE 35.18 bkl 51.60 bkl Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis Electrospun nanofibers (dpeaa)DE-He213 Flexibility (dpeaa)DE-He213 BiOCl/BiOI heterojunctions (dpeaa)DE-He213 In situ synthesis (dpeaa)DE-He213 Floating photocatalysis (dpeaa)DE-He213 |
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ddc 600 bkl 35.18 bkl 51.60 misc Electrospun nanofibers misc Flexibility misc BiOCl/BiOI heterojunctions misc In situ synthesis misc Floating photocatalysis |
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ddc 600 bkl 35.18 bkl 51.60 misc Electrospun nanofibers misc Flexibility misc BiOCl/BiOI heterojunctions misc In situ synthesis misc Floating photocatalysis |
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ddc 600 bkl 35.18 bkl 51.60 misc Electrospun nanofibers misc Flexibility misc BiOCl/BiOI heterojunctions misc In situ synthesis misc Floating photocatalysis |
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Journal of sol gel science and technology |
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Journal of sol gel science and technology |
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Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis |
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(DE-627)SPR043443389 (DE-599)SPRs10971-020-05453-2-e (SPR)s10971-020-05453-2-e |
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Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis |
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Yang, Shu |
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Journal of sol gel science and technology |
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2021 |
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Yang, Shu Zhang, Lei Shao, Changlu Li, Xinghua Li, Xiaowei Liu, Shuai Tao, Ran Liu, Yichun |
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600 670 ASE 35.18 bkl 51.60 bkl |
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Yang, Shu |
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10.1007/s10971-020-05453-2 |
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600 670 |
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verfasserin |
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facile preparation of flexible polyacrylonitrile/biocl/bioi nanofibers via silar method for effective floating photocatalysis |
| title_auth |
Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis |
| abstract |
Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. |
| abstractGer |
Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. |
| abstract_unstemmed |
Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation. Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties. |
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Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis |
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https://dx.doi.org/10.1007/s10971-020-05453-2 |
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Zhang, Lei Shao, Changlu Li, Xinghua Li, Xiaowei Liu, Shuai Tao, Ran Liu, Yichun |
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Zhang, Lei Shao, Changlu Li, Xinghua Li, Xiaowei Liu, Shuai Tao, Ran Liu, Yichun |
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268757607 |
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| doi_str |
10.1007/s10971-020-05453-2 |
| up_date |
2024-07-03T18:42:14.462Z |
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1803584415427723264 |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR043443389</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20220111015740.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">210310s2021 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s10971-020-05453-2</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR043443389</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-599)SPRs10971-020-05453-2-e</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s10971-020-05453-2-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">600</subfield><subfield code="a">670</subfield><subfield code="q">ASE</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">35.18</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">51.60</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Yang, Shu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Facile preparation of flexible polyacrylonitrile/BiOCl/BiOI nanofibers via SILAR method for effective floating photocatalysis</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2021</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract Flexible and floating photocatalysts have unique advantages in water pollution treatment due to their light-harvesting and recycle performance. Here, a facile successive ionic layer adsorption and reaction (SILAR) method was used to layer by layer grow BiOCl/BiOI heterojunctions on self-supporting electrospun polyacrylonitrile (PAN) nanofiber mats at room temperature. This method enables tunable good interface contact of the heterojunctions while makes the composites maintain flexibility and floatable properties. The PAN/BiOCl/BiOI nanofibers show much better photocatalytic activity than the PAN/BiOCl and PAN/BiOI nanofibers. For removal of Rhodamine-B and Bisphenol-A, the degradation rates of PAN/BiOCl/BiOI nanofibers were about 1.68 and 1.41 times higher than PAN/BiOCl nanofibers and were 2.27 and 2.01 times higher than PAN/BiOI nanofibers, respectively. The high photocatalytic performance could be attributed to the effective interfacial charge separation of BiOCl/BiOI heterojunctions, confirmed by the enhanced photocurrent densities, and significantly decreased photoluminescence intensity. The photocatalytic activity of these composite nanofibers could be further improved by adjusting the contents of BiOCl and BiOI in the heterojunction due to the excellent controllability of the SILAR method. Furthermore, the PAN/BiOCl/BiOI nanofibers can float easily and directly reused due to their flexible and self-supporting fiber mats structures. It was expected that the PAN/BiOCl/BiOI nanofibers with high photocatalytic activity and easily separable properties would be useful for industrial wastewater remediation.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Highlights BiOI/BiOCl heterojunctions were evenly grown on PAN nanofibers at room temperature.The nanofibers show high degradation rates for Rhodamine-B and Bisphenol-A.They can be used for floating photocatalysis due to the flexible and self-supporting properties.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Electrospun nanofibers</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Flexibility</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">BiOCl/BiOI heterojunctions</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">In situ synthesis</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Floating photocatalysis</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Zhang, Lei</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Shao, Changlu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Li, Xinghua</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Li, Xiaowei</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Liu, Shuai</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Tao, Ran</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Liu, Yichun</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Journal of sol gel science and technology</subfield><subfield code="d">Dordrecht [u.a.] : Springer Science + Business Media B.V, 1993</subfield><subfield code="g">97(2021), 3 vom: 01. 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